Search results for "Liquid water"
showing 10 items of 61 documents
Clouds and aerosols in Puerto Rico - a new evaluation
2007
The influence of aerosols, both natural and anthropogenic, remains a major area of uncertainty when predicting the properties and behaviour of clouds and their influence on climate. In an attempt to better understand warm cloud formation in a tropical marine environment, a period of intensive measurements took place in December 2004 in Puerto Rico, using some of the latest developments in online instrumentation such as aerosol mass spectrometers, cloud condensation nuclei counters and a hygroscopicity tandem differential mobility analyser. Simultaneous online measurements of aerosol size distributions, composition, hygroscopicity and optical properties were made near the lighthouse of Cape …
A Theoretical Study of the Wet Removal of Atmospheric Pollutants. Part V: The Uptake, Redistribution, and Deposition of (NM4)4SO4by a Convective Clou…
1995
Abstract The effects of an ice phase on the wet deposition of aerosol particles was studied by means of the authors’ 2D cloud dynamics model with spectral microphysics applied to the Cooperative Convective Precipitation Experiment in Miles City, Montana, on 19 July 1981. The cloud macrostructure as well as the cloud microstructure simulated by the model was found to agree well with observations. Although no on-site observations were available with respect to the chemical composition of the cloud and rain water, the values predicted by the model compared well with typical nearby measurements. The following conclusions can be derived from the model computations: (1) In confirmation of the aut…
A numerical model of the cloud-topped planetary boundary-layer: chemistry in marine stratus and the effects on aerosol particles
1999
Abstract In a numerical study the effect of stratiform clouds on aerosol particles is investigated. This is done with the one-dimensional chemical microphysical stratus model CHEMISTRA. In the microphysical part of the model special emphasis is layed on a detailed description of cloud microphysical processes by means of a joint two-dimensional particle distribution for aerosols and cloud droplets. In the chemical part of the model the particle spectrum is subdivided into three categories referring to unactivated aerosols, small and large cloud droplets. Aqueous-phase chemical reactions are separately treated in the two droplet size classes. Numerical results show that within the boundary-la…
Arctic low-level boundary layer clouds: in situ measurements and simulations of mono- and bimodal supercooled droplet size distributions at the top l…
2015
Abstract. Aircraft borne optical in situ size distribution measurements were performed within Arctic boundary layer clouds with a special emphasis on the cloud top layer during the VERtical Distribution of Ice in Arctic clouds (VERDI) campaign in April and May 2012. An instrumented Basler BT-67 research aircraft operated out of Inuvik over the Mackenzie River delta and the Beaufort Sea in the Northwest Territories of Canada. Besides the cloud particle and hydrometeor size spectrometers the aircraft was equipped with instrumentation for aerosol, radiation and other parameters. Inside the cloud, droplet size distributions with monomodal shapes were observed for predominantly liquid-phase Arct…
The effects of different radiation parametrizations on cloud evolution
1997
With the use of the microphysical stratus model (MISTRA), investigations into the effects of variations in the radiative-transfer parametrizations on cloud development have been undertaken. Two radiative-transfer schemes were coupled with the microphysical-thermodynamical section of MISTRA, one based on the exponential sumfitting method and the other based on the correlated k-distribution method of determining gaseous absorption properties. Model runs were initiated with parameter values in accordance with measurements made over the North Sea and comparisons made between model runs where only the radiation schemes were altered. Results indicated that differences between the two schemes had …
Comparison of ERA40 cloud top phase with POLDER-1 observations
2008
[1] A detailed grid-point-based comparison of the cloud top phase derived from the 40-year reanalyses (ERA40) of the European Centre for Medium-Range Weather Forecasts (ECMWF) with satellite measurements is presented. For this purpose an algorithm is implemented to extract a two-dimensional “satellite-like” field of the cloud top phase from ERA40 data. This field is compared with cloud top phase data from the Polarization and Directionality of the Earth Reflectances (POLDER-1) instrument which was in orbit from November 1996 to June 1997. The thermodynamic cloud phase in ERA40 data is parameterized as a function of temperature with pure liquid clouds above 0°C, pure ice clouds below −23°C a…
Reproducing cloud microphysical and irradiance measurements using three 3D cloud generators
2007
Using three cloud generators, three-dimensional (3D) cloud fields are reproduced from microphysical cloud data measured in situ by aircraft. The generated cloud fields are used as input to a 3D radiative transfer model to calculate the corresponding fields of downward and upward irradiance, which are then compared with airborne and ground-based radiation measurements. One overcast stratocumulus scene and one broken cumulus scene were selected from the European INSPECTRO field experiment, which was held in Norwich, UK, in September 2002. With these data, the characteristics of the three different cloud reproduction techniques are assessed. Besides vertical profiles and histograms of measured…
Effects of 20–100 nm particles on liquid clouds in the clean summertime Arctic
2016
Abstract. Observations addressing effects of aerosol particles on summertime Arctic clouds are limited. An airborne study, carried out during July 2014 from Resolute Bay, Nunavut, Canada, as part of the Canadian NETCARE project, provides a comprehensive in situ look into some effects of aerosol particles on liquid clouds in the clean environment of the Arctic summer. Median cloud droplet number concentrations (CDNC) from 62 cloud samples are 10 cm−3 for low-altitude cloud (clouds topped below 200 m) and 101 cm−3 for higher-altitude cloud (clouds based above 200 m). The lower activation size of aerosol particles is ≤ 50 nm diameter in about 40 % of the cases. Particles as small as 20 nm ac…
Control of solute concentrations in cloud and fog water by liquid water content
2000
We measured the concentrations of Cl^−, NO_3^−, and SO_4^(2−) in atmospheric cloudwater collected with a passive collector from a remote marine site and the concentrations of Cl^−, NO_3^−, SO_4^(2−), Na^+ and NH_4^+ in cloudwater from a continental site. At the continental site, an active rotating arm collector was employed for cloudwater collection. At both locations, we observed an inverse relationship between the measured ion concentrations and the liquid water content of the clouds. The product of the observed concentrations and the liquid water content, the cloudwater loading, was found to be nearly constant. A study of published cloudwater data showed that at the majority of the exami…
Airborne investigation of the aerosols–cloud interactions in the vicinity and within a marine stratocumulus over the North Sea during EUCAARI (2008)
2013
Abstract Within the European Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) project, the Meteo France research aircraft ATR-42 was operated from Rotterdam (Netherlands) airport during May 2008, to perform scientific flights dedicated to the investigation of aerosol–cloud interactions. The objective of this study is to illustrate the impact of cloud processing on the aerosol particle physical and chemical properties. The presented results are retrieved from measurements during flight operation with two consecutive flights, first from Rotterdam to Newcastle (United Kingdom) and subsequently reverse along the same waypoints back to Rotterdam using data measured with compact Time …