Search results for "Nanoscale"
showing 10 items of 752 documents
Quantum coherent spin-electric control in a molecular nanomagnet at clock transitions
2020
Electrical control of spins at the nanoscale offers significant architectural advantages in spintronics, because electric fields can be confined over shorter length scales than magnetic fields1–5. Thus, recent demonstrations of electric-field sensitivities in molecular spin materials6–8 are tantalizing, raising the viability of the quantum analogues of macroscopic magneto-electric devices9–15. However, the electric-field sensitivities reported so far are rather weak, prompting the question of how to design molecules with stronger spin–electric couplings. Here we show that one path is to identify an energy scale in the spin spectrum that is associated with a structural degree of freedom with…
Design of a Lambda system for population transfer in superconducting nanocircuits
2013
The implementation of a Lambda scheme in superconducting artificial atoms could allow detec- tion of stimulated Raman adiabatic passage (STIRAP) and other quantum manipulations in the microwave regime. However symmetries which on one hand protect the system against decoherence, yield selection rules which may cancel coupling to the pump external drive. The tradeoff between efficient coupling and decoherence due to broad-band colored Noise (BBCN), which is often the main source of decoherence is addressed, in the class of nanodevices based on the Cooper pair box (CPB) design. We study transfer efficiency by STIRAP, showing that substantial efficiency is achieved for off-symmetric bias only i…
Quasideterministic realization of a universal quantum gate in a single scattering process
2012
We show that a flying particle, such as an electron or a photon, scattering along a one-dimensional waveguide from a pair of static spin-1/2 centers, such as quantum dots, can implement a CZ gate (universal for quantum computation) between them. This occurs quasi-deterministically in a single scattering event, hence with no need for any post-selection or iteration, {and} without demanding the flying particle to bear any internal spin. We show that an easily matched hard-wall boundary condition along with the elastic nature of the process are key to such performances.
Quantum fluctuations and coherence in high-precision single-electron capture.
2012
The phase of a single quantum state is undefined unless the history of its creation provides a reference point. Thus quantum interference may seem hardly relevant for the design of deterministic single-electron sources which strive to isolate individual charge carriers quickly and completely. We provide a counterexample by analyzing the non-adiabatic separation of a localized quantum state from a Fermi sea due to a closing tunnel barrier. We identify the relevant energy scales and suggest ways to separate the contributions of quantum non-adiabatic excitation and backtunneling to the rare non-capture events. In the optimal regime of balanced decay and non-adiabaticity, our simple electron tr…
Geometric phases and criticality in spin chain systems
2005
A relation between geometric phases and criticality of spin chains is established. As a result, we show how geometric phases can be exploited as a tool to detect regions of criticality without having to undergo a quantum phase transition. We analytically evaluate the geometric phase that correspond to the ground and excited states of the anisotropic XY model in the presence of a transverse magnetic field when the direction of the anisotropy is adiabatically rotated. Ultra-cold atoms in optical lattices are presented as a possible physical realization.
Transition to ballistic regime for heat transport in helium II
2014
The size-dependent and flux-dependent effective thermal conductivity of narrow capillaries filled with superfluid helium is analyzed from a thermodynamic continuum perspective. The classical Landau evaluation of the effective thermal conductivity of quiescent superfluid, or the Gorter-Mellinck regime of turbulent superfluids, are extended to describe the transition to ballistic regime in narrow channels wherein the radius $R$ is comparable to (or smaller than) the phonon mean-free path $\ell$ in superfluid helium. To do so we start from an extended equation for the heat flux incorporating non-local terms, and take into consideration a heat slip flow along the walls of the tube. This leads f…
Observation and analysis of Fano-like lineshapes in the Raman spectra of molecules adsorbed at metal interfaces
2015
Surface enhanced Raman spectra from molecules (bipyridyl ethylene) adsorbed on gold dumbells are observed to become increasingly asymmetric (Fano-like) at higher incident light intensity. The electronic temperature (inferred from the anti-Stokes (AS) electronic Raman signal increases at the same time while no vibrational AS scattering is seen. These observations are analyzed by assuming that the molecule-metal coupling contains an intensity dependent contribution (resulting from light-induced charge transfer transitions as well as renormalization of the molecule metal tunneling barrier). We find that interference between vibrational and electronic inelastic scattering routes is possible in …
Phonon Cooling of Nanomechanical Beams with Tunnel Junctions
2009
We demonstrate electronic cooling of 1D phonon modes in suspended nanowires for the first time, using normal-metal-insulator-superconductor (N-I-S) tunnel junctions. Simultaneous cooling of both electrons and phonons to a common temperature was achieved. In comparison with nonsuspended devices, better cooling performance is achieved in the whole operating range of bath temperatures between 0.1-0.7 K. The observed low-temperature thermal transport characteristics are consistent with scattering of ballistic phonons at the nanowire-bulk contact as being the mechanism limiting thermal transport. At the lowest bath temperature of the experiment approximately 100 mK, both phonons and electrons in…
Nanoscale etching of III-V semiconductors in acidic hydrogen peroxide solution: GaAs and InP, a striking contrast in surface chemistry
2019
In this study of nanoscale etching for state-of-the-art device technology, the importance of surface chemistry, in particular the nature of the surface oxide, is demonstrated for two III-V materials. Striking differences in etching kinetics were found for GaAs and InP in sulphuric and hydrochloric acidic solutions containing hydrogen peroxide. Under similar conditions, etching of GaAs was much faster, while the dependence of the etch rate on pH, and on H2O2 and acid concentrations also differed markedly for the two semiconductors. Surface analysis techniques provided information on the product layer present after etching: strongly non-stoichiometric porous (hydr)oxides on GaAs and a thin st…
Current-induced domain wall motion in nanoscale ferromagnetic elements
2011
The manipulation of a magnetic domain wall (DW) by a spin polarized current in ferromagnetic nanowires has attracted tremendous interest during the last years due to fundamental questions in the fields of spin dependent transport phenomena and magnetization dynamics but also due to promising applications, such as DW based magnetic memory concepts and logic devices. We comprehensively review recent developments in the field of geometrically confined domain walls and in particular current induced DW dynamics. We focus on the influence of the magnetic and electronic transport properties of the materials on the spin transfer effect in DWs. After considering the different DW structures in ferrom…