Search results for "Nitroimidazoles"

showing 7 items of 7 documents

Hypoxia-Selective Dissociation Mechanism of a Nitroimidazole Nucleoside in a DNA Environment

2019

Photodynamic therapy is a promising approach to treat a variety of superficial tumors and other diseases. One of its major limitations arises from its dependence on molecular oxygen, which decreases the efficiency of the therapy in hypoxia conditions commonly developed by solid tumors. The present contribution reveals the molecular mechanism of a modified thymine bearing a nitroimidazole substituent, a photosensitizer able to produce highly harmful interstrand cross-links in the DNA double strand after irradiation selectively in absence of oxygen. The mechanism is resolved at a fully atomistic and electronic level relying on quantum mechanics (CASPT2, coupled-cluster, DFT, and TD-DFT method…

SubstituentMolecular Dynamics Simulation010402 general chemistry01 natural scienceschemistry.chemical_compoundMolecular dynamics[CHIM]Chemical SciencesGeneral Materials SciencePhotosensitizerA-DNAPhysical and Theoretical ChemistryComputingMilieux_MISCELLANEOUSPhotosensitizing AgentsNitroimidazole010405 organic chemistryHydrogen bondHydrogen BondingDNA0104 chemical sciencesThyminechemistryNitroimidazolesBiophysicsNucleic Acid ConformationQuantum TheoryDNAThe Journal of Physical Chemistry Letters
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New polyamine drugs as more effective antichagas agents than benznidazole in both the acute and chronic phases.

2018

Abstract Despite the continuous research effort that has been made in recent years to find ways to treat the potentially life threatening Chagas disease (CD), this remains the third most important infectious disease in Latin America. CD is an important public health problem affecting 6–7 million people. Since the need to search for new drugs for the treatment of DC persists, in this article we present a panel of new polyamines based on the tripodal structure of tris(2-aminomethyl)amine (tren) that can be prepared at low cost with high yields. Moreover, these polyamines present the characteristic of being water-soluble and resistant to the acidic pH values of stomach, which would allow their…

Chagas diseaseTrypanosoma cruziPharmacology01 natural sciencesMicrobodies03 medical and health scienceschemistry.chemical_compoundIn vivoOral administrationDrug DiscoverymedicinePolyaminesAnimalsHumansChagas DiseaseTrypanosoma cruzi030304 developmental biologyPharmacology0303 health sciencesFluorenesbiology010405 organic chemistryOrganic ChemistryGeneral Medicinemedicine.diseasebiology.organism_classificationTrypanocidal Agents0104 chemical scienceschemistrySolubilityInfectious disease (medical specialty)BenznidazoleNitroimidazolesDrug DesignToxicityAcute DiseaseChronic DiseasePolyaminemedicine.drugEuropean journal of medicinal chemistry
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Co-localisation of hypoxia and perfusion markers with parameters of glucose metabolism in human squamous cell carcinoma (hSCC) xenografts

2009

Purpose: To examine relationships between tumour hypoxia, perfusion and metabolic microenvironment at themicroregional level in three different human squamous cell carcinomas (hSCC). Materials and methods: Nude mice bearing FaDu, UT-SCC-15, and UT-SCC-5 hSCC were injected with pimonidazole hypoxia and Hoechst perfusion markers. Bioluminescence imaging was used to determine spatial distribution of glucose and lactate content in serial tumour sections. Metabolite levels were grouped in 10 concentration ranges. Images were co-registered and at each concentration range the proportion of area stained for pimonidazole and Hoechst was determinedin 11–13 tumours per tumour line. Results: The spatia…

MaleRadiation-Sensitizing AgentsPathologymedicine.medical_specialtyMetaboliteglucose metabolismTransplantation HeterologousCellMice NudeBiologyCarbohydrate metabolismperfusionbiological imagingMicechemistry.chemical_compoundhuman tumour xenograftsCell Line TumorBiomarkers TumormedicineCo localisationAnimalsHumansPimonidazoleBioluminescence imagingRadiology Nuclear Medicine and imagingLactic AcidHypoxiatumour micromilieuFluorescent DyesRadiological and Ultrasound TechnologyHypoxia (medical)Glucosemedicine.anatomical_structureMicroscopy Fluorescencechemistrypimonidazole hypoxiaNitroimidazolesCarcinoma Squamous CellBenzimidazolesFemalemedicine.symptomPerfusionNeoplasm Transplantation
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Crystal structure of 2-{[1-(2-methyl-5-nitro-1H-imidazol-1-yl)propan-2-yloxy]carbonyl}benzoic acid

2014

In the title compound, C15H15N3O6, the dihedral angle between the planes of the benzene and imidazole rings is 34.93 (10)°. An intramolecular C—H...O hydrogen bond is observed. In the crystal, O—H...N hydrogen bonds link the molecules into chains parallel to thecaxis.

crystal structureCrystal structurepharmaceuticalsDihedral angleBioinformaticsMedicinal chemistrynitro­imidazolesCrystalchemistry.chemical_compoundImidazoleGeneral Materials SciencePhysics::Chemical PhysicsO—H⋯N hydrogen bondsBenzeneBenzoic acidQuantitative Biology::BiomoleculesnitroimidazolesCrystallographyHydrogen bondGeneral ChemistryCondensed Matter PhysicsData ReportsO—H...N hydrogen bondschemistryQD901-999NitroActa Crystallographica Section E Structure Reports Online
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Treatment of Vaginal Trichomoniasis with a Single Dose of Tinidazole

1974

SummaryTwenty-two patients with proven vaginal trichomoniasis were treated with a single dose of 2 g. tinidazole. Twenty-one patients were cured, at both the early and the late follow-up visits. No side-effects were noted and no abnormalities of the clinical laboratory parameters were found in the trial. A historical comparison with published works was carried out and the results compared favourably with those found in the literature for tinidazole as well as for other agents used in a similar fashion.

AdultGynecologymedicine.medical_specialtyDose-Response Relationship Drugbusiness.industryVaginal trichomoniasisAdministration OralAntitrichomonal AgentsGeneral MedicineMiddle AgedTrichomonal VaginitisDermatologyTinidazoleAntitrichomonal agentchemistry.chemical_compoundchemistryNitroimidazolesmedicineHumansFemaleTrichomonas Vaginitisbusinessmedicine.drugCurrent Medical Research and Opinion
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Pimonidazole labelling and response to fractionated irradiation of five human squamous cell carcinoma (hSCC) lines in nude mice: The need for a multi…

2006

To investigate the influence on local control after fractionated radiotherapy of hypoxia measured in unirradiated tumours using the hypoxic marker Pimonidazole, using multivariate approaches.Five human squamous cell carcinoma lines (FaDu, UT-SCC-15, UT-SCC-14, XF354, and UT-SCC-5) were transplanted subcutaneously into the right hind-leg of NMRI nude mice. Histological material was collected from 60 unirradiated tumours after injection of Pimonidazole. The relative hypoxic area within the viable tumour area (Pimonidazole hypoxic fraction, pHF) was determined in seven serial 10 microm cross-sections per tumour by fluorescence microscopy and computerized image analysis. Local tumour control wa…

MaleMultivariate statisticsPathologymedicine.medical_specialtyMice NudeMiceImaging Three-DimensionalCell Line TumorLabellingBiomarkers TumorCarcinomamedicineAnimalsHumansPimonidazoleRadiology Nuclear Medicine and imagingProportional hazards modelbusiness.industryDose fractionationHematologyHypoxia (medical)Prognosismedicine.diseaseXenograft Model Antitumor AssaysCell HypoxiaTreatment OutcomeOncologyNitroimidazolesCarcinoma Squamous CellBiomarker (medicine)FemaleDose Fractionation Radiationmedicine.symptombusinessRadiotherapy and Oncology
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Inhibition of tumor lactate oxidation: consequences for the tumor microenvironment.

2011

Abstract Background and purpose Tumor cells are recognized as being highly glycolytic. However, recently it was suggested that lactate produced in hypoxic tumor areas may be taken up by the monocarboxylate transporter MCT1 and oxidized in well-oxygenated tumor parts. Furthermore, it was shown that inhibition of lactate oxidation using the MCT1 inhibitor α-cyano-hydroxycinnamate (CHC) can radio-sensitize tumors possibly by forcing a switch from lactate oxidization to glycolysis in oxygenated cells, which in turn improves tumor oxygenation and indirectly kills radio-resistant hypoxic tumor cells from glucose starvation. Material and methods To provide direct evidence for the existence of a ta…

Monocarboxylic Acid TransportersPasteur effectMice NudeUterine Cervical NeoplasmsImmunoenzyme Techniques03 medical and health sciencesMice0302 clinical medicineLactate oxidationFluorodeoxyglucose F18Cell Line TumorTumor MicroenvironmentPimonidazoleAnimalsRadiology Nuclear Medicine and imaging030304 developmental biologyMonocarboxylate transporter0303 health sciencesTumor microenvironmentbiologySymportersChemistryGlucose analogHematologyTumor OxygenationWarburg effectCell Hypoxia3. Good healthGlucoseOncologyCinnamatesHead and Neck NeoplasmsNitroimidazoles030220 oncology & carcinogenesisImmunologyLuminescent Measurementsbiology.proteinCancer researchCarcinoma Squamous CellLactatesLinear ModelsAutoradiographyFemaleGlycolysisOxidation-ReductionRadiotherapy and oncology : journal of the European Society for Therapeutic Radiology and Oncology
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