Search results for "Nonlinear optic"
showing 10 items of 530 documents
W-shaped, bright and kink solitons in the quadratic-cubic nonlinear Schrödinger equation with time and space modulated nonlinearities and potentials
2017
An extended non-linear Schrodinger equation (NLSE) combining quadratic and cubic Non-linearities, which appears as an approximate model of a relatively dense quasi-one-dimensional Bose–Einstein con...
Observation of the condensation of classical waves
2010
We report a theoretical, numerical and experimental study of condensation of classical optical waves. The condensation of observed directly, as a function of nonlinearity and wave kinetic energy, in a self-defocusing photorefractive crystal.
Collective behavior ofMbosonic modes interacting with a single two-level atom
1988
The Hamiltonian describing, without the rotating-wave approximation (RWA), the linear interaction between M bosonic modes with an Einstein spectrum and a single two-level atom is exactly and canonically transformed introducing M suitable collective independent field modes, in such a way that only one among them is coupled to the atom. Some physical consequences of this fact are analyzed and, in particular, the existence of radiation-trapping phenomena together with the possibility of atomic absorption suppression is established. The applicability of the RWA to this system is discussed and the importance of the effective-field statistics for the time evolution of the system is pointed out.
Supersolid Behavior of Light
2008
We will show how light can form stationary structures on dielectric periodic media such that their dynamics present simultaneous features of spatial long range order and superfluidity. This phenomenon is normally referred to as supersolidity.
Dynamics of thermally induced optical nonlinearity in GaSe thin slabs
1996
A study of the nonlinear effects shown by thin slabs of GaSe metaled with Au is presented.
Nonlinear pulse deceleration using photorefractive four-wave mixing
2009
We investigate the possibilities of the backward four-wave coupling based on the nonlocal photorefractive response for the nonlinear deceleration of light pulses. The presence of an additional external variable parameter—the pump intensity ratio—allows to improve the output characteristics of the decelerated pulses compared to those typical of the two-wave coupling. In particular, large delay times of the output pulses can be achieved without their strong amplification. This positive distinctive feature of the pulse deceleration occurs far from threshold of the mirrorless optical oscillation.
Strategies for structure solution and refinement of small organic molecules from electron diffraction data and limitations of the simulation approach
1999
In recent years, a series of non-linear optically active bis(benzylidene) ketones have been synthesized and investigated by electron crystallography. In most cases, structure refinement was possible by combining electron diffraction analysis and quantum-mechanical calculations with maximum-entropy methods. However, when the torsional angles between the phenyl rings and the C=C double bonds are strongly affected by the crystal field, this method fails because packing-energy calculations are not sufficiently sensitive. This problem can be solved by refining the approximate model with SHELXL, if the data set is sufficiently accurate and the model close to the correct structure. Here it is show…
Structure determination to calculate nonlinear optical coefficients in a class of organic material
1999
A class of molecules with intramolecular two-dimensional charge transfer upon excitation has been synthesized. It is expected that these materials should be prospective candidates for nonlinear optical (NLO) applications such as second harmonic (SHG) generation. In order to optimize the macroscopic NLO properties of the compounds, it is necessary to relate their first hyperpolarizability tensors at a molecular level to those at a crystal bulk level. This requires a complete structure determination and refinement. However, the growth of sufficiently large single crystals, which are needed for structural analysis and refinement by x-ray methods, is a time-consuming and sometimes impossible ta…
Quadratic Nonlinear Behaviour of Various Langmuir-Blodgett Molecules
1989
The Langmuir-Blodgett (L-B) technique is well known as a method of building-up ordered arrays of organic molecules, and especially as a means of imposing a noncentrosymmetric structure from molecules that crystallize in a centrosymmetric space group(1–3). L-B films for use in quadratic nonlinear optics can be ordered in a statistically noncentrosymmetric lattice. The method involves the compression of a mono-layer of the organic molecule, spread on top of a water surface, into a two-dimensional solid, followed by the repeated dipping of the substrate to be coated into and out of the subphase. Monolayers may be deposited onto the substrate both on immersion and withdrawal, resulting in a cen…
Relationship between microscopic and macroscopic structures of organic thin films for SHG
1993
The experiments described in this paper were undertaken in order to obtain information about the relationship between the structure and non-linear optical properties (second-harmonic generation) of organic thin films. For this purpose, two closely related dyes, diones and tetrones, were compared, both of which are shown to have large hyperpolarisabilities. Their microscopic properties are investigated by conformational analysis and electron diffraction. It could be shown that detailed knowledge about the structure and the adjacent neighbour packing can be obtained from conformational analysis and electron diffraction in order to understand the non-linear optical properties of the two dyes.