Search results for "Nonlinear optics"
showing 10 items of 482 documents
Very narrow-bandwidth tunable infrared difference frequency generation with injection-locked dye lasers
1989
Two flashlamp pumped dye lasers of very high spectral quality are mixed in a LiIO3 crystal to generate a tunable infrared beam through the difference frequency mixing. Thanks to the injection-locking process of the pulsed dye lasers leading to a linewidth of 6 MHz with peak powers of about 10 kW, we obtain an IR beam tunable from 3.5 to 5.9 μm with a peak power of 40 W and a linewidth of 9 MHz. As an application we present a spectrum of N2O obtained by differential absorption near 1880 cm−1. The lines of thisQ-branch are Doppler limited at the working pressure (102 Pa).
Forward-backward equations for nonlinear propagation in axially invariant optical systems
2004
We present a novel general framework to deal with forward and backward components of the electromagnetic field in axially-invariant nonlinear optical systems, which include those having any type of linear or nonlinear transverse inhomogeneities. With a minimum amount of approximations, we obtain a system of two first-order equations for forward and backward components explicitly showing the nonlinear couplings among them. The modal approach used allows for an effective reduction of the dimensionality of the original problem from 3+1 (three spatial dimensions plus one time dimension) to 1+1 (one spatial dimension plus one frequency dimension). The new equations can be written in a spinor Dir…
Linear and nonlinear optical properties of a series of Ni-dithiolene derivatives
2009
Some linear and nonlinear optical (NLO) properties of Ni(SCH)4 and several of its derivatives have been computed by employing a series of basis sets and a hierarchy of methods (e.g., HF, DFT, coupled cluster, and multiconfigurational techniques). The electronic structure of Ni(SCH)4 has been also analyzed by using CASSCF/CASPT2, ab initio valence bond, and DFT methods. In particular we discuss how the diradicaloid character (DC) of Ni(SCH)4 significantly affects its NLO properties. The quasidegeneracy of the two lowest-energy singlet states 1 mathg and 1 math1u, the clear DC nature of the former, and the very large number of low-lying states enhance the NLO properties values. These particul…
Deep Non-Line-of-Sight Reconstruction
2020
The recent years have seen a surge of interest in methods for imaging beyond the direct line of sight. The most prominent techniques rely on time-resolved optical impulse responses, obtained by illuminating a diffuse wall with an ultrashort light pulse and observing multi-bounce indirect reflections with an ultrafast time-resolved imager. Reconstruction of geometry from such data, however, is a complex non-linear inverse problem that comes with substantial computational demands. In this paper, we employ convolutional feed-forward networks for solving the reconstruction problem efficiently while maintaining good reconstruction quality. Specifically, we devise a tailored autoencoder architect…
Directional Second Harmonic Generation Controlled by Sub-wavelength Facets of an Organic Mesowire
2018
Directional harmonic generation is an important property characterizing the ability of nonlinear optical antennas to diffuse the signal in well-defined region of space. Herein, we show how sub-wavelength facets of an organic molecular mesowire crystal can be utilized to systematically vary the directionality of second harmonic generation (SHG) in the forward scattering geometry. We demonstrate this capability on crystalline diamonoanthraquinone (DAAQ) mesowires with subwavelength facets. We observed that the radial angles of the SHG emission can be tuned over a range of 130 degrees. This angular variation arises due to spatially distributed nonlinear dipoles in the focal volume of the excit…
Fabrication of polarizing photonic crystal fibres and photonic crystal fibre tapers: Applications
2007
We report the fabrication of an anisotropic photonic crystal fibre with polarization properties and photonic crystal fibre tapers for supercontinuum generation. The anisotropy of the fibre was created by enlarging four airholes next to the silica core. Different polarization regimes as a function of the geometric parameters, including polarizing behaviour at 1.55 mum, were obtained. In the second part of the paper, we report the fabrication of photonic crystal fibre tapers. We present experimental results on supercontinuum generation in photonic crystal fibre tapers using quasi-continuous pump pulses of 7 ns duration at 532 nm and at 1064 nm.
Nonlinear Characterisation of an AsSe Chalcogenide Holey Fiber
2009
oral session TuA " Highly Nonlinear Fibers " [TuA1]; International audience; We report the nonlinear characterization of a chalcogenide holey fiber, based on the AsSe glass composition. A nonlinear coefficient as high as 15 000 W-1 km-1 has been measured.
Coherent control in single plasmonic nanostructures
2015
Coherent control in plasmonic nanostructures is a door to space-time confinement of optical excitation and femtosecond super-resolution spectroscopy. Towards this goal, here we demonstrate femtosecond pulse-shaping of single gold nanostructure and local phase compensation.
All-fiber processing of terahertz-bandwidth signals based on cascaded tapered fibers
2013
Tapered single-mode fibers are employed to perform dynamic pulse shaping in a bandwidth of several terahertz. The transfer function of cascaded biconical tapers is controlled by introducing a phase shift into one of them through mechanical stretching. It is a simple and low-cost technique with potential to process signals with bandwidths as large as those allocated by standard optical fiber while introducing little degradation. Femtosecond pulses are shaped to prove the concept. (C) 2013 Optical Society of America
Towards CEP stable, single-cycle pulse compression with bulk material
2010
We demonstrate both experimentally and numerically that self-steepening during propagation in a hollow-fiber followed by linear propagation through glass in the anomalous dispersion enables pulse compression down to 1.6 cycles at 1.8 µm wavelength.