Search results for "OPTICS"
showing 10 items of 10033 documents
Isotope-shift measurements of stable and short-lived lithium isotopes for nuclear-charge-radii determination
2010
Changes in the mean-square nuclear charge radii along the lithium isotopic chain were determined using a combination of precise isotope shift measurements and theoretical atomic structure calculations. Nuclear charge radii of light elements are of high interest due to the appearance of the nuclear halo phenomenon in this region of the nuclear chart. During the past years we have developed a new laser spectroscopic approach to determine the charge radii of lithium isotopes which combines high sensitivity, speed, and accuracy to measure the extremely small field shift of an 8 ms lifetime isotope with production rates on the order of only 10,000 atoms/s. The method was applied to all bound iso…
Ab initio angle- and energy-resolved photoelectron spectroscopy with time-dependent density-functional theory
2012
We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that efficiently gives access to photoelectron spectroscopy in time-dependent density-functional calculations. By using a geometrical approach, we provide a simple description of momentum-resolved photoemission including multiphoton effects. The approach is validated by comparison with results in the literature and exact calculations. Furthermore, we present numerical photoelectron angular distributions for randomly oriented nitrogen molecules in a short near-infrared…
Broadening and intensity redistribution in the Na($3p$) hyperfine excitation spectra due to optical pumping in the weak excitation limit
2008
Detailed analysis of spectral line broadening and variations in relative intensities of hyperfine spectral components due to optical pumping is presented. Hyperfine levels of sodium $3p_{1/2}$ and $3p_{3/2}$ levels are selectively excited in a supersonic beam at various laser intensities under the conditions when optical pumping time is shorter than transit time of atoms through the laser beam. The excitation spectra exhibit significant line broadening at laser intensities well below the saturation intensity, and redistribution of intensities of hyperfine spectral components is observed, which in some cases is contradicting with intuitive expectations. Theoretical analysis of the dynamics o…
Polarization-driven spin precession of mesospheric sodium atoms
2018
We report experimental results on the first on-sky observation of atomic spin precession of mesospheric sodium driven by polarization modulation of a continuous-wave laser. The magnetic resonance was remotely detected from the ground by observing the enhancement of induced fluorescence when the driving frequency approached the precession frequency of sodium in the mesosphere, between 85 km and 100 km altitude. The experiment was performed at La Palma, and the uncertainty in the measured Larmor frequency ($\approx$260 kHz) corresponded to an error in the geomagnetic field of 0.4 mG. The results are consistent with geomagnetic field models and with the theory of light-atom interaction in the …
Integration of fuzzy logic and image analysis for the detection of gullies in the Calhoun Critical Zone Observatory using airborne LiDAR data
2017
Abstract The entire Piedmont of the Southeastern United States, where the Calhoun Critical Zone Observatory (CCZO) is located, experienced one of the most severe erosive events of the last two centuries. Forested areas were cleared to cultivate cotton, tobacco, and other crops during the nineteenth and early twentieth century and these land use changes, together with intense rainfalls, initiated deep gullying. An accurate mapping of these landforms is important since, despite some gully stabilization and reforestation efforts, gullies are still major contributors of sediment to streams. Mapping gullies in the CCZO area is hindered by the presence of dense canopy, which precludes the identif…
Argon broadening of the 13CO R(0) and R(7) transitions in the fundamental band at temperatures between 80 and 297K: comparison between experiment and…
2003
We present measurements of Ar-broadening parameters for the R(0) and R(7) lines in the fundamental band of13CO at eight temperatures from 80 to 297 K. The broadening parameters are determined by simultaneous least-squares fitting of spectra recorded using a frequency stabilized diode laser spectrometer. The comparison of the broadening parameter values for R(7) derived at room temperature and different pressures from different line profiles shows that an empirical line profile, which takes into account narrowing effects (Dicke narrowing and absorber speed dependence) but neglects any correlation between collisions, is able to describe the observed lines with constant values of the narrowing…
Investigation by raman spectroscopy of the decomposition process of HKUST-1 upon exposure to air
2016
We report an experimental investigation by Raman spectroscopy of the decomposition process of Metal-Organic Framework (MOF) HKUST-1 upon exposure to air moisture (T=300 K, 70% relative humidity). The data collected here are compared with the indications obtained from a model of the process of decomposition of this material proposed in literature. In agreement with that model, the reported Raman measurements indicate that for exposure times longer than 20 days relevant irreversible processes take place, which are related to the occurrence of the hydrolysis of Cu-O bonds. These processes induce small but detectable variations of the peak positions and intensities of the main Raman bands of th…
Coherence and entanglement dynamics of vibrating qubits
2017
We investigate the dynamics of coherence and entanglement of vibrating qubits. Firstly, we consider a single trapped ion qubit inside a perfect cavity and successively we use it to construct a bipartite system made of two of such subsystems, taken identical and noninteracting. As a general result, we find that qubit vibration can lead to prolonging initial coherence in both single-qubit and two-qubit system. However, despite of this coherence preservation, we show that the decay of the entanglement between the two qubits is sped up by the vibrational motion of the qubits. Furthermore, we highlight how the dynamics of photon-phonon correlations between cavity mode and vibrational mode, which…
Deconvolution procedure of the UV-vis spectra. A powerful tool for the estimation of the binding of a model drug to specific solubilisation loci of b…
2015
UV-vis-spectra evolution of Nile Red loaded into Tween 20 micelles with pH and [Tween 20] have been analysed in a non-conventional manner by exploiting the deconvolution method. The number of buried sub-bands has been found to depend on both pH and bio-surfactant concentration, whose positions have been associated to Nile Red confined in aqueous solution and in the three micellar solubilisation sites. For the first time, by using an extended classical two-pseudo-phases-model, the robust treatment of the spectrophotometric data allows the estimation of Nile Red binding constant to the available loci. Hosting capability towards Nile Red is exalted by the pH enhancement. Comparison between bin…
The Athena X-ray Integral Field Unit (X-IFU)
2018
著者人数: 23名