Search results for "POLARITON"
showing 10 items of 162 documents
Designed surface modes propagating along hyperbolic metamaterials
2013
We report on surface-wave propagation (SWP) that occurs in semi-infinite hyperbolic metamaterials whose optical axis is set in the interface plane. In practice it is implemented by a multi-layered metal-dielectric nanostructure that is cut normally to the layers. Our theoretical analysis shows that various conditions can be designed enabling distinct regimes of SWP. We concluded that hybridization of SWP polarization leads to tighter confinement near the interface as compared with conventional surface plasmon polaritons. By using the finite-element method (FEM), we demonstrate that the fields are enhanced on the walls of metallic films, and thus minimizing significantly its presence inside …
Near-field beam displacement at surface plasmon resonance
2011
International audience; A finite-size beam exciting a surface plasmon polariton (SPP) in a prism coupling configuration experiences an in-plane displacement that can be used for the characterization of plasmonic components by means of near-field optical microscopy. We first demonstrate experimentally the existence of this displacement by taking near-field images of finite-width metal strips. Next, the properties of this shift are analyzed in detail. We investigate the dynamic of the near-field shift for an incident Gaussian beam as a function of illumination conditions. For beams with a narrow spectrum, we propose a straightforward derivation showing that the displacement depends on the ave…
Coherent Light Harvesting through Strong Coupling to Confined Light
2018
When photoactive molecules interact strongly with confined light modes, new hybrid light–matter states may form: the polaritons. These polaritons are coherent superpositions of excitations of the molecules and of the cavity photon. Recently, polaritons were shown to mediate energy transfer between chromophores at distances beyond the Forster limit. Here we explore the potential of strong coupling for light-harvesting applications by means of atomistic molecular dynamics simulations of mixtures of photoreactive and non-photo-reactive molecules strongly coupled to a single confined light mode. These molecules are spatially separated and present at different concentrations. Our simulations sug…
Absence of mutual polariton scattering for strongly coupled surface plasmon polaritons and dye molecules with a large Stokes shift
2013
The understanding and control of the dynamics of hybrid modes consisting of strongly coupled surface plasmon polaritons and molecular excitations of dye molecules is of great timely interest, as it allows one to tailor interactions between optical signals as needed for active all-optical devices. Here we utilize dye molecules with an especially large Stokes shift to demonstrate the absence of mutual scatterings among the strongly coupled hybrid modes. We employ a quantum mechanical three-level model and show that the hybrid modes decay via dephasing and internal relaxation of the molecules to a fluorescing state of the dye, which can be used as a measure for the decay. Our results provide e…
Room-temperature polariton luminescence from a bulk GaN microcavity
2006
We report strong exciton-photon coupling at room temperature in a hybrid high quality bulk 3 lambda/2 GaN cavity with a bottom lattice-matched AlInN/AlGaN distributed Bragg reflector through angle-resolved polarized photoluminescence (PL). Coupling of the optically active free excitons (X-A, X-B, and X-C) to the cavity mode is demonstrated, with their contribution to the PL spectra varying with polarization. Under TE polarization, exciton oscillator strengths for X-A and X-B are about one order of magnitude larger than in bulk GaAs. Photoluminescence exhibits a strong bottleneck effect despite its thermal lineshape.
Phonon-induced polariton superlattices
2006
We show that the coherent interaction between microcavity polaritons and externally stimulated acoustic phonons forms a tunable polariton superlattice with a folded energy dispersion determined by the phonon population and wavelength. Under high phonon concentration, the strong confinement of the optical and excitonic polariton components in the phonon potential creates weakly coupled polariton wires with a virtually flat energy dispersion.
Quantum plasmonics with multi-emitters: application to stimulated Raman adiabatic passage
2018
We construct a mode-selective effective model describing the interaction of the localised surface plasmon polaritons (LSPs) supported by a spherical metal nanoparticle (MNP) with N quantum emitters (QEs) in an arbitrary geometric arrangement. Simplifying previously presented procedures, we develop a formulation in which the field response in the presence of the MNP can be decomposed into orthogonal modes, expanding the Green tensor of the system in the spherical vector harmonics basis and using the generalized global Löwdin orthogonalization algorithm. We investigate the possibility of using the LSPs as mediators of an efficient control of population transfer between two QEs. We show that a…
Molecular quenching and relaxation in a plasmonic tunable system
2008
Molecular fluorescence decay is significantly modified when the emitting molecule is located near a plasmonic structure. When the lateral sizes of such structures are reduced to nanometer-scale cross sections, they can be used to accurately control and amplify the emission rate. In this Rapid Communication, we extend Green's dyadic method to quantitatively investigate both radiative and nonradiative decay channels experienced by a single fluorescent molecule confined in an adjustable dielectric-metal nanogap. The technique produces data in excellent agreement with current experimental work.
Optimization of surface plasmons launching from subwavelength hole arrays: modelling and experiments
2009
International audience; The launching of surface plasmons by micro-gratings of subwavelength apertures milled in a thick metal film is important for the development of surface plasmon based circuits. By comparing the near-field optical images of such surface plasmon sources with the results of a Huygens-Fresnel principle based scattering model, we show that the properties of the locally launched SP beams such as divergence or uniformity can be tuned by adjusting the shape of the micro-gratings. This allows us to propose an optimized source array well adapted for providing a narrow, collimated and uniform beam. (c) 2007 Optical Society of America.
Ridge-enhanced optical transmission through a continuous metal film
2004
Optical transmission through a continuous (without holes) metal film with a periodic structure of metal or dielectric ridges on one or both interfaces was numerically studied. The dependencies of the transmission on the ridge width and height as well as the ridge arrangements on the opposite interfaces were investigated in weak- and strong-coupling regimes. The transmission enhancement was shown to depend on the relative position of the ridge gratings on the opposite interfaces of a film, confirming the role of resonant tunneling processes involving states of the surface polariton Bloch modes.