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showing 10 items of 980 documents

Modificētu enzīmu dizains proteīnu deglikācijai

2022

Fruktozila peptīdu oksidāzes, pazīstamas arī kā Amadoriāzes, ir enzīmu saime, kas katalizē fruktozilaminoskābju deglikozilāciju. Šī darba mērķis ir novērtēt termālo stabilitāti un enzimātisko aktivitāti Amadoriāzes enzīma mutantiem, C16 un D02, kurus izstrādāja ārvalstu kolēģi, izmantojot skaitļošanas metodes. Darba gaitā tika veikta veikta ekspresija E. coli šūnās un proteīnu attīrīšana, izmantojot šķīdumu hromatogrāfiju. Tika veikta proteīnu analīze, izmantojot biofizikālu un bioķīmisku analīžu metodes - termiskās nobīdes, cirkulārā dihroisma un enzimātiskās aktivitātes testus. Rezultāti uzrādīja termostabilitātes un viršas punktu palielināšanos abiem mutantiem, enzimātiskās aktivitātes u…

Amadoriaseadvanced glycation end-productsBioloģijaAGEsprotein expressiondeglycating enzyme
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Evaluation of analytical performance of gas chromatography coupled with atmospheric pressure chemical ionization Fourier transform ion cyclotron reso…

2019

Abstract A new analytical method was established and validated for the analysis of eighteen halogenated flame retardants (HFRs)in food products. Gas chromatography (GC) coupled to Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR-MS) employing atmospheric pressure chemical ionization (APCI) was used for the identification and quantitation of contaminants. Intra-laboratory validation of the method was performed with respect to recovery, repeatability, linear calibration ranges, instrumental and method limits of quantitation (i-LOQ and m-LOQ), and trueness was verified where possible by analysis of reference materials (RMs). The validation results indicated recoveries of ana…

AnalyteEnvironmental EngineeringMaterials scienceFood SafetyHalogenationHealth Toxicology and Mutagenesis0208 environmental biotechnologyAtmospheric-pressure chemical ionization02 engineering and technology010501 environmental sciences01 natural sciencesFourier transform ion cyclotron resonanceGas Chromatography-Mass SpectrometryMass SpectrometryCalibrationHalogenated Diphenyl EthersEnvironmental ChemistryHumans0105 earth and related environmental sciencesFlame RetardantsDetection limitChromatographyFourier AnalysisPublic Health Environmental and Occupational HealthGeneral MedicineGeneral ChemistryRepeatabilityCyclotronsPollution020801 environmental engineeringFoodFood productsGas chromatographyFood AnalysisChemosphere
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Multi-analyte method for the analysis of legacy and alternative brominated and chlorinated flame retardants in food products of animal origin using g…

2019

Abstract An analytical method was developed and validated for the analysis of 32 halogenated flame retardants (HFRs), including 13 polybrominated diphenyl ethers (PBDEs), 9 dechlorane-related compounds (DRCs) and 10 of the so-called alternative BFRs in food samples of animal origin. Gas chromatography (GC) coupled with magnetic sector high resolution mass spectrometry (HRMS) was used for the instrumental analysis. Intralaboratory validation of the developed method was performed in terms of recovery, repeatability, linear calibration ranges, instrumental and method limits of quantitation (i-LOQ and m-LOQ). Where possible, trueness was verified by the analysis of reference materials (RMs). Fo…

AnalyteMeatEnvironmental EngineeringEggsHealth Toxicology and Mutagenesis0208 environmental biotechnologyFood ContaminationPilot Projects02 engineering and technology010501 environmental sciences01 natural sciencesAnimal originGas Chromatography-Mass SpectrometryPolybrominated diphenyl ethersLimit of DetectionHalogenated Diphenyl EthersHydrocarbons ChlorinatedCalibrationAnimalsEnvironmental ChemistryFlame Retardants0105 earth and related environmental sciencesMulti analyteChromatographyPublic Health Environmental and Occupational HealthGeneral MedicineGeneral ChemistryRepeatabilityPollution020801 environmental engineeringMilkFood productsEnvironmental scienceGas chromatographyChemosphere
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X-ray analysis on the nanogram to microgram scale using porous complexes

2012

X-ray single-crystal diffraction (SCD) analysis has the intrinsic limitation that the target molecules must be obtained as single crystals. Here we report a protocol for SCD analysis that does not require the crystallization of the sample. In our method, tiny crystals of porous complexes are soaked in a solution of the target, such that the complexes can absorb the target molecules. Crystallographic analysis clearly determines the absorbed guest structures along with the host frameworks. Because the SCD analysis is carried out on only one tiny crystal of the complex, the required sample mass is of the nanogram–microgram order. We demonstrate that as little as about 80 nanograms of a sample …

Analytical chemistryCrystallography X-RayMass spectrometryHigh-performance liquid chromatographyAbsorptionlaw.inventionCrystallawAnimalsNanotechnologyMoleculeCrystallizationta116Biological ProductsMultidisciplinaryChemistryMicrochemistryAnalytic Sample Preparation MethodsPoriferaCharacterization (materials science)AlkynesFatty AlcoholsAbsorption (chemistry)CrystallizationPorous mediumPorosityNature
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Inhibition of tumor angiogenesis by antibodies, synthetic small molecules and natural products.

2011

Cancer remains one of the major causes of death worldwide. The switch to pathological angiogenesis is a key process in the promotion of cancer and consequently provides several new and promising targets to anticancer therapy. Thus, antagonizing angiogenesis cuts off the tumor's oxygen and nutrition supply. This review focuses on angiogenesis inhibitors as option for cancer treatment. Modes of action, adverse effects, mechanisms of resistance as well as new developments are highlighted. One approach in angiogenesis inhibition is intermitting the further VEGF (vascular endothelial growth factor) signal pathway with monoclonal antibodies. Bevacizumab is a highly specific recombinant humanized …

Angiogenesismedicine.drug_classGenisteinAngiogenesis InhibitorsAntineoplastic AgentsBiologyPharmacologyMonoclonal antibodyBiochemistryReceptor tyrosine kinaseNeovascularizationSmall Molecule Librarieschemistry.chemical_compoundGrowth factor receptorNeoplasmsDrug DiscoverymedicineAnimalsHumansPharmacologyBiological ProductsNeovascularization PathologicVascular Endothelial Growth FactorsOrganic ChemistryCancerAntibodies Monoclonalmedicine.diseaseAntineoplastic Agents PhytogenicVascular endothelial growth factorchemistrybiology.proteinMolecular Medicinemedicine.symptomCurrent medicinal chemistry
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Protection by extra virgin olive oil against oxidative stress in vitro and in vivo. Chemical and biological studies on the health benefits due to a m…

2017

Abstract We report the results of in vivo studies in Caenorhabditis elegans nematodes in which addition of extra virgin olive oil (EVOO) to their diet significantly increased their life span with respect to the control group. Furthermore, when nematodes were exposed to the pesticide paraquat, they started to die after two days, but after the addition of EVOO to their diet, both survival percentage and lifespans of paraquat-exposed nematodes increased. Since paraquat is associated with superoxide radical production, a test for scavenging this radical was performed using cyclovoltammetry and the EVOO efficiently scavenged the superoxide. Thus, a linear correlation (y = -0.0838x +19.73, regres…

Animals; Caenorhabditis elegans; Cell Cycle; Cell Line; Electron Spin Resonance Spectroscopy; Humans; In Vitro Techniques; Olive Oil; Oxidative Stress; Paraquat; Rats; Reactive Oxygen Species; Diet Mediterranean0301 basic medicineAntioxidantmedicine.medical_treatmentlcsh:MedicineMediterraneanmedicine.disease_causeDiet MediterraneanBiochemistryAntioxidantsMonocytesMyoblastschemistry.chemical_compoundWhite Blood Cells0302 clinical medicineParaquatGalvinoxylSuperoxidesAnimal CellsPlant ProductsMedicine and Health SciencesElectrochemistryFood sciencelcsh:Sciencechemistry.chemical_classificationMultidisciplinarySuperoxideStem CellsCell CycleAgricultureOxidesLipidsPeroxidesHydroperoxideChemistry030220 oncology & carcinogenesisPhysical SciencesCellular TypesResearch ArticleParaquatImmune CellsImmunologyIn Vitro TechniquesSettore BIO/09Vegetable OilsCell Line03 medical and health sciencesmedicineAnimalsHumansSettore BIO/10Caenorhabditis elegansOlive OilReactive oxygen speciesBlood CellsElectrode Potentialslcsh:RElectron Spin Resonance SpectroscopyChemical CompoundsBiology and Life SciencesCell BiologyAgronomyDietRatsTyrosolOxidative Stress030104 developmental biologychemistryHydroxytyrosollcsh:QReactive Oxygen SpeciesOilsOxidative stressCrop Science
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Chemical Constituents and Pharmacological Properties ofPoria cocos

2011

Poria cocos (Polyporaceae) is a saprophytic fungus that grows in diverse species of Pinus. Its sclerotium, called fu-ling or hoelen, is used in traditional Chinese and Japanese medicine for its diuretic, sedative, and tonic effects. Various studies of this fungus have demonstrated its marked anti-inflammatory activity in different experimental models of acute and chronic inflammation. It is widely used as a constituent of many preparations in Asian medicine, but the number of research papers on its clinical properties is insufficient for establishing its efficacy and safety from a scientific point of view. In this review, we have compiled all the published data concerning the chemistry, pha…

Anti-Inflammatory AgentsPharmaceutical ScienceAntineoplastic AgentsInflammationBiologyPharmacognosyAnalytical ChemistryImmune systemJapanPolysaccharidesPsoriasisDrug DiscoverymedicineHumansImmunologic FactorsSecretionMedicine Chinese TraditionalPolyporaceaePharmacologyBiological ProductsTraditional medicineOrganic ChemistryPoriamedicine.diseasebiology.organism_classificationTriterpenesPolyporusComplementary and alternative medicinePhytochemicalMolecular Medicinemedicine.symptomPlanta Medica
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Polycerasoidol, a Natural Prenylated Benzopyran with a Dual PPARα/PPARγ Agonist Activity and Anti-inflammatory Effect

2019

Dual peroxisome proliferator-activated receptor-α/γ (PPARα/γ) agonists regulate both lipid and glucose homeostasis under different metabolic conditions and can exert anti-inflammatory activity. We investigated the potential dual PPARα/γ agonism of prenylated benzopyrans polycerasoidol (1) and polycerasoidin (2) and their derivatives for novel drug development. Nine semisynthetic derivatives were prepared from the natural polycerasoidol (1) and polycerasoidin (2), which were evaluated for PPARα, -γ, -δ and retinoid X receptor-α activity in transactivation assays. Polycerasoidol (1) exhibited potent dual PPARα/γ agonism and low cytotoxicity. Structure–activity relationship studies revealed th…

Anti-Inflammatory AgentsRXRα/PPARγPharmaceutical ScienceRetinoid X receptorPharmacology01 natural sciencesAnalytical ChemistryStructure-Activity Relationshipchemistry.chemical_compoundTransactivationPrenylationPOLYCERASOIDOLDrug DiscoveryHumansStructure–activity relationshipGlucose homeostasisBenzopyransPPAR alphaMOLECULAR MODELINGCytotoxicityPrenylationPharmacologyMolecular Structure010405 organic chemistryChemistry[CHIM.ORGA]Chemical Sciences/Organic chemistryOrganic ChemistryCiencias QuímicasNATARUL PRODUCTSPeroxisome0104 chemical sciencesBenzopyranPPAR gamma010404 medicinal & biomolecular chemistryQuímica OrgánicaComplementary and alternative medicineMolecular MedicineCIENCIAS NATURALES Y EXACTAS
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Characterization of the interaction of the antifungal and cytotoxic cyclic glycolipopeptide hassallidin with sterol-containing lipid membranes.

2019

Hassallidins are cyclic glycolipopeptides produced by cyanobacteria and other prokaryotes. The hassallidin structure consists of a peptide ring of eight amino acids where a fatty acid chain, additional amino acids, and sugar moieties are attached. Hassallidins show antifungal activity against several opportunistic human pathogenic fungi, but does not harbor antibacterial effects. However, they have not been studied on mammalian cells, and the mechanism of action is unknown. We purified hassallidin D from cultured cyanobacterium Anabaena sp. UHCC 0258 and characterized its effect on mammalian and fungal cells. Ultrastructural analysis showed that hassallidin D disrupts cell membranes, causin…

Antifungal AgentskolesteroliPeptideLipopeptide01 natural sciencesBiochemistrychemistry.chemical_compoundSTRUCTURE ELUCIDATIONCandida albicansMARINE CYANOBACTERIAmammalian cellsmembrane1183 Plant biology microbiology virologychemistry.chemical_classification0303 health sciencesCell DeathMembraneGlycopeptidesLipopeptideHERBICOLIN-ADEHYDROPEPTIDE LACTONEAmino acidSterolsCholesterolMembraneBiochemistrysolunsalpaajatMitochondrial Membranesmedicine.symptomBacterial outer membraneBiophysicsmechanismAntineoplastic Agentssaponin digitoninMolecular dynamicsCyanobacteriaITURIN-A03 medical and health sciencesLipopeptidesMembrane LipidsNATURAL-PRODUCTSCell Line TumormedicineHumansPropidium iodidesyanobakteerit030304 developmental biologyantimikrobiset yhdisteet010405 organic chemistryMAJOR COMPONENTCell BiologyluonnonaineetAnabaenaSterol0104 chemical sciencesMechanism of actionchemistrylipopeptidepeptiditMOLECULAR-DYNAMICS1182 Biochemistry cell and molecular biologyDrug Screening Assays AntitumorGlycolipidsBiochimica et biophysica acta. Biomembranes
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Isolation, Identification and Investigation of Fermentative Bacteria from Sea Bass (Dicentrarchus labrax): Evaluation of Antifungal Activity of Ferme…

2020

During fish production processes, great amounts of by-products are generated, representing &asymp

Antifungal activity; By-products; Fermentative process; Lactic acid bacteria; Sea bassHealth (social science)Plant Sciencelcsh:Chemical technologyHealth Professions (miscellaneous)MicrobiologyArticle03 medical and health sciencesMinimum inhibitory concentrationchemistry.chemical_compound0404 agricultural biotechnologyLactobacilluslcsh:TP1-1185Food scienceSea bassby-productsFermented fishfermentative process0303 health sciencesbiology030306 microbiologyantifungal activityAmbientalefood and beverages04 agricultural and veterinary sciencesbiology.organism_classification040401 food scienceLactic acidlactic acid bacteriachemistryPenicilliumFermentationsea bassBacteriaFood ScienceFoods
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