Search results for "Physics::Optics"
showing 10 items of 1958 documents
ChemInform Abstract: Electron Crystallography and Organic Materials with Non-Linear Optical Properties
2010
Results of electron microscopic studies of crystal structures of a number of bis-benzylidene cyclohexanones are presented. It is shown that some of these compounds are efficient crystalline non-linear optically active (NLO) chromophores with second harmonic generation (SHG) properties. Appropriately functionalized chromophores of this type can be used as a polycondensation comonomer to produce partly crystalline main-chain NLO-active polymers. Electron diffraction crystal structural data, obtained for very small crystals, allowed us to get reasonable estimations of macroscopic crystal NLO-coefficients, relating quantum-chemically calculated molecular first hyperpolarizability components to …
Relationship between microscopic and macroscopic structures of organic thin films for SHG
1993
The experiments described in this paper were undertaken in order to obtain information about the relationship between the structure and non-linear optical properties (second-harmonic generation) of organic thin films. For this purpose, two closely related dyes, diones and tetrones, were compared, both of which are shown to have large hyperpolarisabilities. Their microscopic properties are investigated by conformational analysis and electron diffraction. It could be shown that detailed knowledge about the structure and the adjacent neighbour packing can be obtained from conformational analysis and electron diffraction in order to understand the non-linear optical properties of the two dyes.
Cylindrical Cuvette Light Refraction Measurements Technology to Analyse Biomedical Liquids
2015
Compact device of high sensitivity for measurement of the refractive indices for both stationary and flowing liquids has been developed. This device can be used to analyse a variety of biomedical liquids: urine, serum protein. The refractive index (RI) is determined by measuring the deviation of a laser beam passing through a cylindrical cuvette containing the test liquid. In order to significantly improve the resolution and stability of RI measurements, the repeated reflections and refractions of the light beam travelling through the cylindrical cuvette are employed.
All-Optical Fiber Hanbury Brown & Twiss Interferometer to study 1300 nm single photon emission of a metamorphic InAs Quantum Dot
2016
[EN] New optical fiber based spectroscopic tools open the possibility to develop more robust and efficient characterization experiments. Spectral filtering and light reflection have been used to produce compact and versatile fiber based optical cavities and sensors. Moreover, these technologies would be also suitable to study N-photon correlations, where high collection efficiency and frequency tunability is desirable. We demonstrated single photon emission of a single quantum dot emitting at 1300 nm, using a Fiber Bragg Grating for wavelength filtering and InGaAs Avalanche Photodiodes operated in Geiger mode for single photon detection. As we do not observe any significant fine structure s…
Ultrafast Optical Demagnetization manipulates Nanoscale Spin Structure in Domain Walls
2012
During ultrafast demagnetization of a magnetically ordered solid, angular momentum has to be transferred between the spins, electrons, and phonons in the system on femto- and picosecond timescales. Although the intrinsic spin-transfer mechanisms are intensely debated, additional extrinsic mechanisms arising due to nanoscale heterogeneity have only recently entered the discussion. Here we use femtosecond X-ray pulses from a free-electron laser to study thin film samples with magnetic domain patterns. We observe an infrared-pump-induced change of the spin structure within the domain walls on the sub-picosecond timescale. This domain-topography-dependent contribution connects the intrinsic dem…
Polarization-domain-wall complexes in fiber lasers
2013
To study the possible build-up of polarization-domain-walls (PDWs) in fiber laser cavities, an erbium-doped fiber ring laser was used and a wide range of vector polarization dynamics that can be selected at a given pump power, by using the degrees of freedom of two intracavity polarization controllers (PC) was investigated. A simple theoretical model that explains polarization switching in fiber ring lasers featuring a normally dispersive cavity with a typical, moderate, level of birefringence is presented. Such polarization dynamics, based on a special class of polarization-domain-wall structures, agrees qualitatively well with experimental observations. The paper stresses on the complex a…
Hamiltonian tools for the analysis of optical polarization control
2011
Import JabRef; International audience; The study of the polarization dynamics of two counterpropagating beams in optical fibers has recently been the subject of a growing renewed interest, from both the theoretical and experimental points of view. This system exhibits a phenomenon of polarization attraction, which can be used to achieve a complete polarization of an initially unpolarized signal beam, almost without any loss of energy. Along the same way, an arbitrary polarization state of the signal beam can be controlled and converted into any other desired state of polarization, by adjusting the polarization state of the counterpropagating pump beam. These properties have been demonstrate…
Nanorod orientation control by swift heavy ion irradiation
2022
Highly energetic ions have been previously used to modify the shape of metal nanoparticles embedded in an insulating matrix. In this work, we demonstrate that under suitable conditions, energetic ions can be used not only for shape modification but also for manipulation of nanorod orientation. This observation is made by imaging the same nanorod before and after swift heavy ion irradiation using a transmission electron microscope. Atomistic simulations reveal a complex mechanism of nanorod re-orientation by an incremental change in its shape from a rod to a spheroid and further back into a rod aligned with the beam. Highly energetic ions have been previously used to modify the shape of meta…
Enhanced nanoscopy of individual CsPbBr3 perovskite nanocrystals using dielectric sub-micrometric antennas
2020
We demonstrate an efficient, simple, and low-cost approach for enhanced nanoscopy in individual green emitting perovskite (CsPbBr3) nanocrystals via TiO2 dielectric nanoantenna. The observed three- to five-fold emission enhancement is attributed to near-field effects and emission steering promoted by the coupling between the perovskite nanocrystals and the dielectric sub-micrometric antennas. The dark-field scattering configuration is then exploited for surface-enhanced absorption measurements, showing a large increase in detection sensitivity, leading to the detection of individual nanocrystals. Due to the broadband spectral response of the Mie sub-micrometric antennas, the method can be e…
Femtosecond laser induced breakdown spectroscopy of air–methane mixtures
2013
Abstract Femtosecond laser pulses are used in order to induce dielectric breakdown in gaseous mixtures, namely in some reactive air–methane mixtures. The light emitted from the laser induced plasma was analyzed while the main emission features are identified and assigned. From the analysis of the emission spectra, a linear relationship was found to hold between the intensity of some spectral features and methane content. Finally, the use of femtosecond laser induced breakdown as a tool for the in situ determination of the composition of gaseous mixtures (e.g., equivalence ratio) is also discussed.