Search results for "Reaction"
showing 10 items of 6134 documents
Comparison of electromagnetic and nuclear dissociation of Ne-17
2018
8 pags., 10 figs., 3 tabs.
Synthesis ofN=127isotones through (p,n) charge-exchange reactions induced by relativistic208Pb projectiles
2011
The production cross sections of four N=127 isotones ({sup 207}Hg, {sup 206}Au, {sup 205}Pt, and {sup 204}Ir) have been measured using (p,n) charge-exchange reactions, induced in collisions of a {sup 208}Pb primary beam at 1 A GeV with a Be target. These data allow one to investigate the use of a reaction mechanism to extend the limits of the chart of nuclides toward the important r-process nuclei in the region of the third peak of elemental abundance distribution.
Molecular dynamics simulations of elementary chemical processes in liquid water using combined density functional and molecular mechanics potentials.…
1997
A new approach to carry out molecular dynamics simulations of chemical reactions in solution using combined density functional theory/molecular mechanics potentials is presented. We focus our attention on the analysis of reactive trajectories, dynamic solvent effects and transmission coefficient rather than on the evaluation of free energy which is another important topic that will be examined elsewhere. In a previous paper we have described the generalities of this hybrid molecular dynamics method and it has been employed to investigate low energy barrier proton transfer process in water. The study of processes with activation energies larger than a few kT requires the use of specific tech…
On time-resolved approach for phonon assisted interband transitions
2015
Photoexcited dynamics of electrons and holes in two-band dielectric, with special emphasis on back reaction of phonons are developed by combining the quantum electrodynamics and Baker-Campbell-Hausdorff (BCH) canonical transformation. These methods create an explicit time-domain representation of photoinduced processes and contribute in unifying phonon-assisted description of distribution functions of electron and hole quasiparticles for the description of observable effects of photoinduced processes in dielectrics.
Quantum mechanical study of the proton exchange in the ortho-para H2 conversion reaction at low temperature
2011
Ortho-para H2 conversion reactions mediated by the exchange of a H+ proton have been investigated at very low energy for the first time by means of a time independent quantum mechanical (TIQM) approach. State-to-state probabilities and cross sections for H+ + H 2 (v = 0, j = 0,1) processes have been calculated for a collision energy, Ec, ranging between 10-6 eV and 0.1 eV. Differential cross sections (DCSs) for H+ + H2 (v = 0, j = 1) → H+ + H2 (v′ = 0, j′ = 0) for very low energies only start to develop a proper global minimum around the sideways scattering direction ( ≈ 90°) at Ec = 10-3 eV. Rate coefficients, a crucial information required for astrophysical models, are provided between 10…
The influence of the solvent's mass on the location of the dividing surface for a model Hamiltonian
2019
The Transition State dividing surface is a key concept, not only for the precise calculation of the rate constant of a reaction, but also for the proper prediction of product ratios. The correct location of this surface is defined by the requirement that reactive trajectories do not recross it. In the case of reactions in solution the solvent plays an important role in the location of the dividing surface. In this paper we show with the aid of a model Hamiltonian that the effective mass of the solvent can dramatically change the location of the dividing surface. Keywords: Dynamical systems, Dividing surface, Reactions in solution, 2019 MSC: 00-01, 99-00
Recent advances in the description of reactions involving exotic nuclei
2019
In this contribution to the proceedings of the International Nuclear Physics Conference 2019, I review recent developments made in reaction models used to analyse data measured at radioactive-ion beam facilities to study exotic nuclear structures. I focus in particular on reactions like elastic scattering and breakup, which are used to study halo nuclei. Although these peculiar nuclei challenge usual nuclear-structure models, some can now be computed ab initio. This brief review illustrates the progresses made in nuclear-reaction theory in the last few years to improve the description of the projectile within reaction models. I dedicate this contribution to the memory of Mahir Hussein, who …
The elastic scattering of 25MeV α-particles and neutron shell effects in the A = 50 TO A = 93 mass region
1982
Abstract Experimental elastic scattering angular distributions of 25 MeV α-particles scattered from 28 nuclei ranging from 50Cr to 93Nb have been measured and then analysed in terms of a regular optical model with standard Woods-Saxon geometries for both the real and imaginary potentials. The experimental distributions are well fitted over the whole angular range from 5° to 175° c.m. by the predictions, provided that a smaller than normal diffuseness is used for the imaginary potentials. The usual families of potentials with volume integrals differing by approximately 100 MeV · fm3 are found. The family with volume integral ranging from 540 to 420 MeV· fm3 over the nuclei studied has been c…
Direct measurement of the radiative tail in electron scattering from atomic nuclei
1985
We have made a direct measurement of the radiative tail of the eleastic peak from several tungsten targets. The measured data have been compared to the results expected for both internal and external bremsstrahlung contributions. Even for targets as thick as 4% of a radiation length of tungsten, agreement between the results of the experiment and the predictions of the theory has been found to be unexpectedly good.
Transfer reactions on light exotic nuclei studied with CHIMERA detector at LNS
2014
The kinematical coincidence method is used to extract angular distribution of elastic scattering and transfer reactions. The detected light particle energy spectra are used to extract the angular distribution with around 1° resolution in the Center of Mass (CM) system. Examples with 10Be beam are presented. In the case of proton scattering, γ-ray coincidences are used to discriminate excited levels population from elastic scattering. © Owned by the authors, published by EDP Sciences, 2014.