Search results for "SPONTANEOUS FISSION"
showing 10 items of 42 documents
K isomerism in Rf255 and total kinetic energy measurements for spontaneous fission of Rf255,256,258
2020
Spontaneous fission properties of the isotopes $^{255}\mathrm{Rf}$, $^{256}\mathrm{Rf}$, and $^{258}\mathrm{Rf}$ produced in the reactions $^{50}\mathrm{Ti}+^{207}\mathrm{Pb}$, $^{50}\mathrm{Ti}+^{208}\mathrm{Pb}$, and $^{50}\mathrm{Ti}+^{209}\mathrm{Bi}$ were studied. The method of time and position correlations was used to identify spontaneous fission events. The correction to the energy deficit in measured total kinetic energy (TKE) determined on the basis of a study of $^{252}\mathrm{No}$ was applied to evaluate the $\overline{\mathrm{TKE}}$ of investigated rutherfordium isotopes. A signature which we assigned tentatively to bimodal fission was observed in TKE distributions of $^{255}\m…
Spontaneous fission of rutherfordium isotopes - total kinetic energies
2019
The isotopes 255,256,258Rf were produced in the fusion-evaporation reactions 50Ti + 207,208Pb and 50Ti + 209Bi at GSI Darmstadt, using the velocity filter SHIP. Total kinetic energies of fragments from spontaneous fission for these isotopes were evaluated with a correction to pulse-height defect.
Spontaneous fission instability of the neutron-deficient No and Rf isotopes: The new isotope No249
2021
In the heaviest elements, the instability of atomic nuclei against spontaneous fission leads to ever shorter nuclear half-lives. Upon falling below a timescale of ${10}^{\ensuremath{-}14}$ s, the border of existence of isotopes is crossed because this is the timescale on which the formation of atomic shells occurs. Analysis of the experimental data on the spontaneous fission half-lives of Rf isotopes in relation with their expected single-particle orbitals hint at a potentially abrupt decrease in half-lives of unknown neutron-deficient Rf isotopes with neutron numbers $l149$, which suggests that the isotopic border is already almost reached. However, this conjecture, which cannot be explain…
Decay study of 246Fm at SHIP
2011
The decay chain of 246Fm has been investigated employing the SHIP separator at GSI Darmstadt. The 246Fm nuclei were produced via the 40Ar(208Pb, 2n)246Fm fusion-evaporation reaction. Improved values of the half-life, T 1/2 = 1.54(4) s, and of the spontaneous fission branching ratio, b SF = 0.068(6) , of 246Fm were obtained. The $ \beta^{+}_{}$ /electron capture branching ratio, b EC = 0.39(3) , of 242Cf was deduced. Possible structures of high-K states in 246Fm are discussed within the framework of a model calculation based on the Woods-Saxon potential.
The identification and confirmation of isomeric states in 254Rf and 255Rf through conversion electron detection
2020
Abstract The neutron-deficient isotopes 254,255Rf were produced in the fusion-evaporation reaction 50Ti + 206Pb at the gas-filled recoil separator TASCA. Decay properties of these nuclei were investigated by applying fast digital electronics. A search for isomeric states in both isotopes was performed by using the accompanying conversion electron emissions. Isomeric states with half-lives of 4(1) μs and >30 μs were measured for 254Rf and 255Rf, respectively, which confirm the findings at different separators. The present experimental results demonstrate the great potential of fast digital electronics for measurements of isomeric states in the heaviest nuclei, which are only producible in sm…
Neutron configurations inPd113
2014
Excited states in $^{113}\mathrm{Pd}$, populated in ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of $^{113}\mathrm{Rh}$ and in spontaneous fission of $^{248}\mathrm{Cm}$ and $^{252}\mathrm{Cf}$, have been studied by means of $\ensuremath{\gamma}$ spectroscopy at the IGISOL facility of Jyv\"askyl\"a University and using large arrays of Ge detectors (Eurogam2 and Gammasphere, respectively). The position of the ${11/2}^{\ensuremath{-}}$ yrast excitation in $^{113}\mathrm{Pd}$, proposed recently at 166.1 keV by other authors, has been corrected to 98.9 keV. The decay of this level has been discussed to explain the observed transition intensities. The ${7/2}^{\ensuremath{-}}$ member of the yras…
Microscopic description of complex nuclear decay: multimodal fission
2009
Our understanding of nuclear fission, a fundamental nuclear decay, is still incomplete due to the complexity of the process. In this paper, we describe a study of spontaneous fission using the symmetry-unrestricted nuclear density functional theory. Our results show that the observed bimodal fission can be explained in terms of pathways in multidimensional collective space corresponding to different geometries of fission products. We also predict a new phenomenon of trimodal spontaneous fission for some rutherfordium, seaborgium, and hassium isotopes.
The Role of Fission in the r-process
2007
We have developed a full set of fission rates that include spontaneous fission, neutron-induced fission, beta-delayed fission and, neutrino-induced fission, that are supplemented with realistic distributions of fission yields. Using this new input data we have carried out r-process calculations assuming adiabatic expansions that mimic the conditions achieved in the supernova neutrino driven wind. We have explored the sensitivity of the final abundances to different mass models. The resulting abundance distribution turns out to be very sensitive to the strength of the N = 82 shell gap far from stability. Mass models with a strong shell gap converge to an r-process distribution that is indepe…
Determination of the partial electron capture- and spontaneous-fission half-lives of254No
1988
The isotope254No was produced in the fusion reaction48Ca +208Pb. Using the velocity filter SHIP and radiochemical techniques it was found that the nuclide254No with a half-life of 55 s decays byα, EC, and spontaneous-fission. Deduced partial half-lives are (61±2) s forα-decay, (550−160+370) s for EC and [2.2−1.0+2.0]×104 s for spontaneous fission.
Pairing-induced speedup of nuclear spontaneous fission
2014
Collective inertia is strongly influenced at the level crossing at which quantum system changes diabatically its microscopic configuration. Pairing correlations tend to make the large-amplitude nuclear collective motion more adiabatic by reducing the effect of those configuration changes. Competition between pairing and level crossing is thus expected to have a profound impact on spontaneous fission lifetimes. To elucidate the role of nucleonic pairing on spontaneous fission, we study the dynamic fission trajectories of $^{264}$Fm and $^{240}$Pu using the state-of-the-art self-consistent framework. We employ the superfluid nuclear density functional theory with the Skyrme energy density fun…