Search results for "Second harmonic generation"
showing 10 items of 20 documents
Contrôle de nano-antennes optiques par une commande électrique : tuner plasmonique et transduction
2011
Optical nano-antennae are the new class of components to control light/matterinteraction at the nanoscale. These devices are operating in the visible to near infraredpart of the spectrum. The properties of these nano objects are controlled by theform, the size and the material.In the radio frequency domain, the tuner changes dynamically the operatingwavelength of the antenna. In this thesis work, we search to transfer this conceptto the nanoscale. The principle is to change the load impedance of the antenna, i.e.changing the optical index of the dielectric medium around the nano-object. Forthat we used anisotropic liquid cristal molecules. The value of the optical index iscontrolled by appl…
Optical characterization of YCa4O(BO3)3 and Nd:YCa4O(BO3)3 crystals
2007
International audience; We report a complete optical characterization of YCa4O(BO3)3 and Nd:YCa4O(BO3)3 crystals. We studied the relative orientation between the dielectric and the crystallographic frames as a function of the wavelength and performed accurate phase-matching angles measurements for second harmonic generation, using a single crystal cut as a sphere. We also recorded polarized luminescence spectra of Nd:YCOB along the principal axes of the dielectric frame. For both crystals, we measured the gray-tracking and the thermo-optic properties as a function of temperature and wavelength using oriented slabs. Finally, we measured all their dielectric and electro-optic coefficients, as…
Orientation dependence of high-order harmonic generation in molecules
2003
We present two- and three-dimensional model calculations of high-order harmonic generation in ${\mathrm{H}}_{2}^{+}.$ The harmonic spectra exhibit clear signatures of intramolecular interference. An interference minimum appears at a harmonic order that depends on the molecular orientation. Harmonic generation in three-center molecules is studied on the basis of two-dimensional calculations for a ${\mathrm{H}}_{3}^{2+}$ model system. From analytical considerations, the orientation dependence of the harmonic intensities in three-center molecules exhibits a double minimum due to intramolecular interference. In the numerical results, the double minimum is broadened into a single wide minimum. T…
Second harmonic generation by an isolated spin
1970
Abstract The second harmonic generation at microwave frequency by a spin S = 1 2 in a cavity has been studied as a function of the external magnetic field using a resolvent technique, and the average transition rates to states with an increased number of double-frequency photons has been calculated. In spite of the crudeness of the model, a good qualitative agreement has been found between the predictions of the present theory and recent experimental results on non-linear behaviour of paramagnetic spin systems in a microwave field.
Parametric self-trapping in the presence of randomized quasi phase matching
2010
We report on experimental evidence of parametric spatial solitons in a quadratic crystal with randomized periodic ferroelectric poling. Two-color self-focusing via quadratic cascading overcomes the diffractive nature of both fundamental and frequency-doubled beams.
Second Harmonic Generation via Random Quasi-phase Matching in a Periodically Poled Lithium Tantalate Waveguide
2011
We observe second harmonic generation via random quasi phase matching in a 1.5μm periodically poled lithium tantalate. The presence of a slab waveguide allows the comparison between bulk and guided wave configurations.
Self-Assembled Molecular Rafts at Liquid|Liquid Interfaces for Four-Electron Oxygen Reduction
2011
The self-assembly of the oppositely charged water-soluble porphyrins, cobalt tetramethylpyridinium porphyrin (CoTMPyP(4+)) and cobalt tetrasulphonatophenyl porphyrin (CoTPPS(4-)), at the interface with an organic solvent to form molecular "rafts", provides an excellent catalyst to perform the interfacial four-electron reduction of oxygen by lipophilic electron donors such as tetrathiafulvalene (TTF). The catalytic activity and selectivity of the self-assembled catalyst toward the four-electron pathway was found to be as good as that of the Pacman type cofacial cobalt porphyrins. The assembly has been characterized by UV-visible spectroscopy, Surface Second Harmonic Generation, and Scanning …
Second order nonlinear optics in AlGaAs metasurfaces
2023
Recently, nonlinear optics at the nanoscale level has emerged as a promising branch of nanophotonics. In this work, we focus our attention on Aluminum Gallium Arsenide (AlGaAs) nanoantennas and metasurfaces for efficient and controlled second harmonic photon emission. After a brief introduction concerning the main studies in this field, we present the latest results achieved in AlGaAs platforms both in the lossless and absorption regimes.
Second Harmonic Emission From Dielectric Nanoresonators in the Absorption Regime
2023
We study second harmonic generation in dielectric nanocylinders as a function of the wavelength of the incident field and geometrical dimensions. Uncommonly, we consider a spectral range in which the emitted nonlinear signal is partially absorbed by the dielectric. Surprisingly, we reveal that the second harmonic efficiency does not decrease as the imaginary part of the complex dielectric refractive index increases. Indeed, the presence of higher order multipoles supported by the resonators at the fundamental wavelength can significantly boost the generated second harmonic signal even in the dielectric absorption spectral region achieving nonlinear efficiency of the same order of magnitude …
Quasi Phase Matched UV Second Harmonic Generation in Lithium Tantalate soft PE Waveguides
2008
We report on first experimental results on UltraViolet second-harmonic generation by first-order quasiphase-matching in a surface periodically poled proton exchanged Lithium Tantalate waveguide. We have achieved a good compatibility with alpha phase proton exchanged channel waveguides in Lithium Tantalate. We held the sample in a temperature controlled oven kept at a constant temperature of 250 °C, to reduce photorefractive damage. The pump source was a Ti-Sapphire laser with a tunability range of 700 - 980 nm and a 40-GHz linewidth. Continuous wave UV light at 365.4 nm was produced with a conversion efficiency of 6.6% W-1cm-2.