Search results for "Second-Harmonic Generation"

Scanning near-field optical microscopy (SNOM) of lithium niobate aperiodically poled during growth

2007

In the present work, aperiodically poled lithium niobate (APPLN) was grown, along the a-axis, by the off-centred Czochraski method. The domain formation has been triggered by rare earth doping, using in this case Er3+ and Yb3+ ions. The growth conditions were selected in order to obtain a modulated domain distribution. SNOM measurements have been performed with a Nanonics Imaging Ltd model MultiView 200 TM working in non-contact tapping mode.

Thermal expansion, normalized thermo-optic coefficients, and condition for second harmonic generation of a Nd:YAG laser with wide temperature bandwid…

2011

Interferometric determination of thermal expansion and of normalized thermo-optic coefficients of RbTiOPO4 at four laser wavelengths are performed as a function of temperature. A suitable vectorial formalism applied to obtained data allows the establishment of the temperature dependence of refractive indices, and subsequent theoretical analysis enables one to predict that an extremum in the evolution of the phase-matching direction in the (X,Y) plane should occur near 100 °C for type II second harmonic generation of Nd:YAG lasers, with a temperature bandwidth that can be as large as 117 °C for a crystal of 10 mm in length. Such unusual behavior is observed experimentally by recording the co…

Continuous-wave, double-pass second-harmonic generation with 60% efficiency in a single MgO:PPSLT crystal

2014

We present a double-pass scheme for high-efficiency, high-power, second-harmonic generation (SHG) in a single MgO-doped periodically poled stoichiometric lithium tantalate (MgO:PPSLT) crystal. The device is pumped by a single-frequency, continuous-wave fiber amplifier laser system at a wavelength of 1091 nm. For the double-pass scheme, a conversion efficiency of 60% and a harmonic power of 12.8 W at a wavelength of 545.5 nm with a high beam quality of (M2<1.2) is achieved. Compared to single-pass SHG, a double-pass enhancement factor of more than two is observed at the highest fundamental pump power.

Amphiphilic dyes for nonlinear optics: Dependence of second harmonic generation on functional group substitution

2008

Synthesis and nonlinear optical properties of novel N,N-dihydroxyethyl-based molecular organic glasses using triaryl substitutes as amorphous phase f…

2011

In given study a new structural design of molecular NLO materials is presented where amorphous phase formation is achieved by introduction of bulky trityl and triphenylsilyl substituents. Obtained materials formed stable organic glasses with good optical quality and glass transition temperatures notably exceeding ambient. NLO activity was successfully measured in samples that underwent corona discharge poling. The comparison of both enhancer groups revealed, that trityl group increases thermal sustainability of material, while triphenylsilyl group better promotes formation and stability of amorphous phase.

Multimodal nonlinear imaging of suspended carbon nanotubes using circular polarizations

2013

In this work, multimodal nonlinear microscopy of suspended CNTs using circular polarizations (CP) was reported. Significant variations in the SHG and THG signals of the CNTs between left hand circular polarization (LHCP) and right hand circular polarization (RHCP) were observed. The variations in the nonlinear signals can be associated to the unique properties of the CNTs such as chirality.

750 mW continuous-wave solid-state deep ultraviolet laser source at the 253.7 nm transition in mercury.

2007

A high-power continuous-wave coherent light source at 253.7 nm is described. It is based on a solid-state Yb:YAG disk laser with two successive frequency doubling stages and is capable of generating stable output powers of up to 750 mW. Spectroscopy of the 6 (1)S(0)-6 (3)P(1) transition of mercury has been demonstrated.

Thermal imaging in artificial nonlinear media

1997

A method has been developed to determine the temperature distribution of ferroelectric surfaces and volumes. Based on the nonlinear optical effect of second harmonic generation (SHG) in highly nonlinear ferroelectric coating, demonstration of 2D thermosensing has been performed in the wide temperature range (77 K - 600 K). Physical concept of SHG thermal imaging, design of thermosensitive coating and experimental verification of the method has been discussed.

Affordable, ultra-broadband coherent detection of terahertz pulses via CMOS-compatible solid-state devices

2017

We demonstrate the first fully solid-state technique for the coherent detection of ultra-broadband THz pulses (0.1-10 THz), relying on the electric-field-induced second-harmonic generation attained in integrated CMOS-compatible devices.

Opto-thermally controlled beam steering in nonlinear all-dielectric metastructures

2021

Reconfigurable metasurfaces have recently gained a lot of attention in applications such as adaptive meta-lenses, hyperspectral imaging and optical modulation. This kind of metastructure can be obtained by an external control signal, enabling us to dynamically manipulate the electromagnetic radiation. Here, we theoretically propose an AlGaAs device to control the second harmonic generation (SHG) emission at nanoscale upon optimized optical heating. The asymmetric shape of the used meta-atom is selected to guarantee a predominant second harmonic (SH) emission towards the normal direction. The proposed structure is concurrently excited by a pump beam at a fundamental wavelength of 1540 nm and…