Search results for "Second-harmonic generation"
showing 10 items of 116 documents
Nanotechnology in lithium niobate for integrated optic frequency conversion in the UV
2017
In the domain of Earth Explorer satellites nanoengineered nonlinear crystals can optimize UV tunable solid-state laser converters. Lightweight sources can be based on Lithium Niobate (LN) domain engineering by electric field poling and guided wave interactions. In this Communication we report the preliminary experimental results and the very first demonstration of UltraViolet second-harmonic generation by first-order quasi-phase-matching in a surface-periodically-poled proton-exchanged LN waveguide. The pump source was a Ti-Sapphire laser with a tunability range of 700- 980 nm and a 40 GHz linewidth. We have measured UV continuous-wave light at 390 nm by means of a lock-in amplifier and of …
Background-Free Second-Harmonic Generation Microscopy of Individual Carbon Nanotubes
2015
We use polarized second-harmonic generation (SHG) microscopy to investigate pristine air-suspended carbon nanotubes (CNT). We show that SHG originates from CNT chirality, allowing also different response for the two circular polarizations of fundamental light.
Second harmonic generation in selenium-metal structures
2009
The article examines the processes of second harmonic generation (SHG) when selenium-metal (Cu) film structures are illuminated by femtosecond radiation (180 fs, 80 MHz) at wavelength 800 – 1000 nm. Selenium-copper structures were obtained by successive thermal evaporation of selenium and copper onto the glass substrate in vacuum. Microanalysis of the film composition was performed to determine amount of copper in thin films. The as-evaporated selenium-copper structures were crystallised by annealing in inert atmosphere at temperature 85°C. Just evaporated as well as annealed thin films were explored. The experiment was performed by confocal microscope [1] where the femtosecond radiation fr…
Novel second-order nonlinear optical polymer materials containing indandione derivativatives as a chromophore
2006
Second order non linear optical (NLO) properties of sPMMA based host-guest systems containing eight dimethylaminobenzylidene -1, 3 - indandione (DMABI) related chromophores have been investigated by means of quantum chemical calculations and SHG experimental characterization. Ab initio calculations with basis set 6-31G were used for molecular geometry determination as well as in the calculations of molecular hyperpolarizability by FF approach. Influence of the chromophore concentration on the host-guest film NLO performance was obtained by SHG Maker fringe experiments. The highest value of d53233 =80 pm/V (frequency corrected value d033 =12 pm/V) at chromophore concentration 15 %wt have bee…
Second harmonic generation and beam cleaning in optically poled multimode graded-index fibers
2017
Recent experimental results have confirmed that nonlinear effects in multimode graded-index (MM-GRIN) fibers lead to a wealth of observable spatiotemporal effects. In spite of the large number of modes supported by the fiber, by increasing the input power the transverse profile evolves in a clean bell-shaped beam [1, 2]. Next, the input laser line experiences a strong spectral broadening and Geometric Parametric Instability (GPl) peaks are observed [3].
Spatial beam cleaning in quadratic nonlinear medium
2018
We show experimentally that a laser beam scrambled by propagation in a short segment of multimode fiber may be cleaned by the nonlinear propagation in KTP cristal with type-II second-harmonic generation.
Second- and third-harmonic generation as a local probe for nanocrystal-doped polymer materials with a suppressed optical breakdown threshold
2003
Abstract Second- and third-harmonic generation processes are shown to allow the detection of absorptive agglomerates of nanocrystals in transparent materials and the visualization of optical breakdown in nanocomposite materials. Correlations between laser-induced breakdown and the behavior of the second- and third-harmonic signals produced in SiC/PMMA nanocomposite films are studied. The potential of second- and third-harmonic generation for the on-line visualization of laser breakdown in nanocomposite polymer materials is revealed, with the ablative material removal being monitored by the decay of the second- and third-harmonic signals. The second and third harmonics generated around the o…
Optical characterization of YCa4O(BO3)3 and Nd:YCa4O(BO3)3 crystals
2007
International audience; We report a complete optical characterization of YCa4O(BO3)3 and Nd:YCa4O(BO3)3 crystals. We studied the relative orientation between the dielectric and the crystallographic frames as a function of the wavelength and performed accurate phase-matching angles measurements for second harmonic generation, using a single crystal cut as a sphere. We also recorded polarized luminescence spectra of Nd:YCOB along the principal axes of the dielectric frame. For both crystals, we measured the gray-tracking and the thermo-optic properties as a function of temperature and wavelength using oriented slabs. Finally, we measured all their dielectric and electro-optic coefficients, as…
Nanopatterned ferroelectric crystals for parametric generation
2006
We report on recent results by surface periodic poling on lithium niobate and lithium tantalate. Such approach allows periodic inversion of the second order susceptibility with nanoscale features using insulating masks. We achieved a world-best 200 nm feature size, as well as good compatibility with alpha-phase proton exchanged channel waveguides in lithium niobate. Preliminary results of surface periodic poling in lithium tantalate also show similar characteristics. Surface poling is best suited for integrated optics devices in technologically-demanding configurations such as backward second harmonic generation and counter propagating optical parametric amplification
GENERAZIONE DI SECONDA ARMONICA RETRO-PROPAGANTE IN NIOBATO DI LITIO CON POLING PERIODICO
2010
We report on backward second-harmonic-generation in bulk periodically poled congruent lithium niobate with a 3.2 micron period. A tunable continuous-wave Ti:Sapphire laser allowed us exciting two resonant quasi-phase-matched orders. Resonances were also resolved by temperature tuning.