Search results for "Second-harmonic generation"
showing 10 items of 116 documents
Guided-wave frequency doubling in surface periodically poled lithium niobate: competing effects
2007
We carried out second-harmonic generation in quasi-phase-matched ? -phase lithium niobate channel waveguides realized by proton exchange and surface periodic poling. Owing to a limited ferroelectric domain depth, we could observe the interplay between second-harmonic generation and self-phase modulation due to cascading and cubic effects, resulting in a nonlinear resonance shift. Data reduction allowed us to evaluate both the quadratic nonlinearity in the near infrared as well as the depth of the uninverted domains. © 2007 Optical
Towards CEP stable sub two cycle IR pulse compression with bulk material
2010
We demonstrate both experimentally and numerically that self-steepening during propagation in a hollow-fiber followed by linear propagation through glass in the anomalous dispersion enables pulse compression down to 1.9 cycles at 1.8 micron wavelength.
Backward frequency doubling of near infrared picosecond pulses.
2014
We report on backward second-harmonic generation using ps laser pulses in congruent lithium niobate with 3.2 µm periodic poling. Three resonant peaks were measured between 1530 and 1730 nm, corresponding to 16th, 17th and 18th quasi-phase-matching orders in the backward configuration, with a conversion efficiency of 4.75 x 10(-5%)/W for the 16th order. We could also discriminate the contributions from inverted domains randomized in duty-cycle.
Grating-assisted third-harmonic generation in photonic crystal fibers using a pulse pump
2011
We demonstrate that quasi-phase-matching of the third-harmonic generation process can be obtained for a pulse pump in the photonic crystal fiber with a refractive-index grating. Conversion efficiency is calculated numerically using a system of coupled generalized nonlinear Schrodinger equations. We propose a special design of the microstructured fiber for the third-harmonic generation and analyze different phenomena limiting the maximum efficiency for short (femtosecond) and long (picosecond) pump pulses. Moreover, we show that a certain level of a group-velocity mismatch between the pump and the third harmonic can increase the maximum efficiency in the long pulse regime.
Soft proton exchanged channel waveguides in congruent lithium tantalate for frequency doubling
2010
We report on stable optical waveguides fabricated by soft-proton exchange in periodically-poled congruent lithium tantalate in the a-phase. The channel waveguides are characterized in the telecom wavelength range in terms of both linear properties and frequency doubling. The measurements yield a nonlinear coefficient of about 9.5pm/V, demonstrating that the nonlinear optical properties of lithium tantalate are left nearly unaltered by the process. (C) 2010 Optical Society of America
Triple excitation effects in coupled-cluster calculations of frequency-dependent hyperpolarizabilities
1998
Abstract We describe an implementation of an analytic scheme for the calculation of static and dynamical first hyperpolarizabilities at the CC3 level in the framework of coupled-cluster response theory. Calculations are reported for the static, the second harmonic generation, and the optical rectification hyperpolarizabilities of FH. The results indicate the importance of triple excitation effects for accurate theoretical predictions of hyperpolarizabilities and lend further support to previous contentions that an experimental value for the second harmonic generation hyperpolarizabilities of FH should be reconsidered.
Measurement of optical second-harmonic generation from an individual single-walled carbon nanotube
2013
We show that optical second-harmonic generation (SHG) can be observed from individual single-walled carbon nanotubes (SWCNTs) and, furthermore, allows imaging of individual tubes. Detailed analysis of our results suggests that the structural noncentrosymmetry, as required for SHG, arises from the non-zero chiral angle of the SWCNT. SHG thus has potential as a fast, non-destructive, and simple method for imaging of individual nanomolecules and for probing their chiral properties. Even more, it opens the possibility to optically determine the handedness of individual SWCNTs.
Bi-color spatial solitons in linearly uncoupled planar waveguides
2004
We report on the observation of spatial optical simultons in a novel geometry consisting of two partially overlapped, linearly uncoupled planar waveguides in lithium niobate obtained by reverse proton exchange. Two orthogonally polarized modes are coupled through an off-diagonal tensor element of the quadratic nonlinearity, giving rise to second harmonic generation and mutual trapping via cascading. This phenomenon demonstrates a balance between diffraction and self-focusing for two orthogonal modes of different waveguides, and occurs at room temperature in longitudinally uniform waveguides.
Counter-propagating difference-frequency generation in diamond with terahertz fields
2013
The nonlinear interaction of terahertz (THz) pulses with optical fields in Kerr, gaseous media is a key ingredient for broadband THz detection schemes [1]. Terahertz field-induced second harmonic generation in solid-state media has also been considered for THz detection and as a tool e.g. for liquid dynamics investigations [2,3], while four-wave mixing has been addressed as a possible mechanism for THz generation [4,5]. © 2013 IEEE.
Second harmonic generation in multimode graded-index fibers: spatial beam cleaning and multiple harmonic sideband generation
2017
We study experimentally and numerically the spectral and spatial dynamics of second harmonic generation in an all-optically poled multimode graded-index fiber. In contrast with poled single-mode fibers, in a multimode graded-index fiber a pump can generate a series of sharp sidebands around its second harmonic (SH) that originate from the sub-millimetric periodic evolution of the intensity at the fundamental frequency. The mutual interaction between the fundamental and its SH may also strongly affect the spatial distribution of guided light for both colors: when increasing the pump power, both fundamental and SH output beams evolve from disordered multimode speckles into two bell-shaped bea…