Search results for "Sulfone"

showing 10 items of 113 documents

Novel Approach for Asymmetric Synthesis of Fluorinated β-Amino Sulfones and Allylic Amines

2003

[reaction: see text] Enantiomerically pure gamma-fluoroalkyl beta-amino sulfones are readily synthesized in three steps starting from fluorinated imidoyl chlorides and arylmethyl sulfones. A complementary two-step sequence starting from chiral fluorinated beta-amino sulfoxides has also been developed. To illustrate the application of this procedure, a new method for the synthesis of alpha-fluoroalkyl allylic amines in optically pure form involving a Julia methylenation-desulfonylation reaction is presented.

Allylic rearrangementHydrocarbons FluorinatedChemistryorganic chemicalsOrganic ChemistryEnantioselective synthesisStereoisomerismGeneral MedicineCombinatorial chemistryBiochemistryAllyl CompoundsOrganic chemistrySulfonesAminesPhysical and Theoretical ChemistryOrganic Letters
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Analysis of four parabens and bisphenols A, F, S in urine, using dilute and shoot and liquid chromatography coupled to mass spectrometry

2018

Abstract A new strategy for the analysis of 4 parabens (methylparaben, ethyl paraben, propyl paraben and butyl paraben) and 3 bisphenols (A, F and S) in human urine has been developed. Dilute and shoot and liquid chromatography coupled to mass spectrometry (LC-MS/MS) determination was employed. Procedural matched calibration, certified materials and spiked samples were used for validation. The obtained recoveries varied between 85 and 104% with a precision lower than 20% for all analytes. The LOQ was 0.20 ng mL for all analytes. Negative atmospheric pressure chemical ionization in the selected reaction monitoring mode was used for MS detection. The proposed method was successfully applied f…

AnalyteBisphenol AParabensAtmospheric-pressure chemical ionization02 engineering and technologyUrineMass spectrometry01 natural sciencesAnalytical Chemistrychemistry.chemical_compoundPhenolsTandem Mass SpectrometryHumansSulfonesBenzhydryl CompoundsChromatographyMethylparaben010401 analytical chemistrySelected reaction monitoring021001 nanoscience & nanotechnology0104 chemical sciencesParabenchemistrySpain0210 nano-technologyChromatography LiquidTalanta
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Chronic peroxisome proliferator-activated receptorβ/δ agonist GW0742 prevents hypertension, vascular inflammatory and oxidative status, and endotheli…

2015

Endothelial dysfunction plays a key role in obesity-induced risk of cardiovascular disease. The aim of the present study was to analyze the effect of chronic peroxisome proliferator-activated receptor (PPAR)β/δ agonist GW0742 treatment on endothelial function in obese mice fed a high-fat diet (HFD).Five-week-old male mice were allocated to one of the following groups: control, control-treated (GW0742, 3 mg/kg per day, by oral gavage), HFD, HFD + GW0742, HFD + GSK0660 (1 mg/kg/day, intraperitoneal) or HFD-GW0742-GSK0660 and followed for 11 or 13 weeks. GW0742 administration to mice fed HFD prevented the gain of body weight, heart and kidney hypertrophy, and fat accumulation. The increase in …

Blood GlucoseMaleAgonistmedicine.medical_specialtyNitric Oxide Synthase Type IIIEndotheliumPhysiologymedicine.drug_classCaveolin 1Peroxisome proliferator-activated receptorThiophenesDiet High-FatGW0742MiceInsulin resistanceInternal medicineInternal MedicinemedicineAnimalsObesityPPAR deltaSulfonesEndothelial dysfunctionReceptorPPAR-betaAortachemistry.chemical_classificationInterleukin-6Tumor Necrosis Factor-alphabusiness.industryGlucose Tolerance TestPeroxisomemedicine.diseaseToll-Like Receptor 4VasodilationThiazolesEndocrinologymedicine.anatomical_structureAdipose TissuechemistryHypertensionAdiponectinEndothelium VascularInsulin ResistanceReactive Oxygen SpeciesCardiology and Cardiovascular MedicinebusinessJournal of Hypertension
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Transgenerational effects on intestinal inflammation status in mice perinatally exposed to bisphenol S

2020

International audience; Increasing evidence has highlighted the critical role of early life environment in shaping the future health outcomes of individuals in subsequent generations. Bisphenol S (BPS) has been widely used as a substitute for various plastic materials due to the limited application of Bisphenol A (BPA) which is an endocrine disruptor. However, the lack of efficient evaluation of BPS leaves doubts about the relevant substitute of BPA. Few studies of transgenerational inheritance have examined the effects of environmental exposures to endocrine disruptors on the immune system. In this study, we analyzed the transgenerational effects of BPS on intestinal inflammation and its c…

Blood GlucoseMaleBisphenol SHealth Toxicology and Mutagenesis[SDV]Life Sciences [q-bio]0208 environmental biotechnologyPhysiology02 engineering and technologyEndocrine Disruptors010501 environmental sciences01 natural sciencesFecesMicePregnancySulfonesPerinatal ExposureGeneral MedicinePollutionIntestine[SDV] Life Sciences [q-bio][SDV.TOX] Life Sciences [q-bio]/ToxicologyIntestinesEndocrine disruptorPrenatal Exposure Delayed Effects[SDV.TOX]Life Sciences [q-bio]/ToxicologyCytokinesGestationFemalemedicine.symptomhormones hormone substitutes and hormone antagonistsEnvironmental EngineeringOffspringInflammationImmune systemPhenolsmedicineAnimalsEnvironmental ChemistryWeaningEndocrine system0105 earth and related environmental sciencesInflammationbusiness.industryBody WeightPublic Health Environmental and Occupational HealthGeneral Chemistry020801 environmental engineeringPerinatal exposureMice Inbred C57BLMetabolismbusiness
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Non-steroidal Anti-inflammatory Agents, Part 19:E-2-Pyrrolizin-5-yl Acrylic Acids as Potent Dual or Selective Inhibitors of Bovine Cyclooxygenase and…

1995

The pyrrolizinyl substituted acrylic acid derivatives represent another class of dual and selective inhibitors of cyclooxygenase and 5-lipoxygenase. By modifying their substitution pattern at the phenyl moiety of C-6 the balance between the activity against cyclooxygenase and against 5-lipoxygenase can be shifted. Structure-activity relationships are discussed. Compound 6k is the most potent and well-balanced dual inhibitor of both enzymes, while the highest selectivity of lipoxygenase inhibition was found for 6j. The activity and selectivity of compounds with an additional sulfur moiety depend on the oxidation status of this atom, giving an indication of the discussed coupling between pero…

Blood PlateletsNeutrophilsStereochemistryCarboxylic acidPharmaceutical ScienceIn Vitro TechniquesSulfoneStructure-Activity Relationshipchemistry.chemical_compoundLipoxygenaseDrug DiscoveryAnimalsStructure–activity relationshipMoietyCyclooxygenase InhibitorsPyrrolesLipoxygenase Inhibitorschemistry.chemical_classificationbiologyAnti-Inflammatory Agents Non-SteroidalAcrylateschemistryEnzyme inhibitorArachidonate 5-lipoxygenasebiology.proteinCattleCyclooxygenaseArchiv der Pharmazie
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Experimental evidence of pharmacological management of anchorage in Orthodontics: A systematic review

2015

Introduction: Orthodontic anchorage is one of the most challenging aspects of Orthodontics. Preventing undesired movement of teeth could result in safer and less complicated orthodontic treatment. Recently, several reviews have been published about the effects of different molecules on bone physiology and the clinical side effects in Orthodontics. However, the effects of local application of these substances on the rate of orthodontic tooth movement have not been assessed.Objectives: The aim of this research was to analyze the scientific evidence published in the literature about the effects of different molecules on orthodontic anchorage.Methods: The literature was systematically reviewed …

Bone remodeling periodBisfosfonatosTooth Movement TechniquesMovimentação dentáriaPharmacological managementAnti-Inflammatory AgentsOsteoclastsPamidronateDentistryZoledronic AcidAntioxidantsLactonesMiceStilbenesOrthodontic Anchorage ProceduresMedicineAgentes anti-inflamatóriosSulfonesAnti-inflammatory agentsOrthodonticsDiphosphonatesOsteoprotegerinaImidazolesOrthodontic anchorage proceduresArticlesBisphosphonatesProcedimentos de ancoragem ortodônticaTooth movementInclusion and exclusion criteriaBone RemodelingTooth MobilityOral SurgeryDiclofenacMEDLINEOrthodonticsKappa indexInterferon-gammaAnimalsHumansbusiness.industryOsteoprotegerinBone physiologyIsoxazolesOrthodontic Anchorage ProceduresAcetylcysteineRatslcsh:RK1-715CelecoxibResveratrolTooth movementlcsh:DentistryClodronic Acidbusiness
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Growth of human cells on polyethersulfone (PES) hollow fiber membranes.

2004

A novel material of porous hollow fibers made of polyethersulfone (PES) was examined for its ability to support the growth of human cells. This material was made in the absence of solvents and had pore diameters smaller than 100 microm. Human cell lines of different tissue and cell types (endothelial, epithelial, fibroblast, glial, keratinocyte, osteoblast) were investigated for adherence, growth, spread and survival on PES by confocal laser microscopy after staining of the cells with Calcein-AM. Endothelial cell attachment and growth required pre-coating PES with either fibronectin or gelatin. The other cell types exhibited little difference in growth, spread or survival on coated or uncoa…

Cell typeMaterials scienceBiocompatibilityPolymersSurface PropertiesConfocalBiophysicsCell Culture TechniquesBioengineeringNanotechnologyBiocompatible MaterialsCell LineBiomaterialsTissue engineeringCell MovementMaterials TestingmedicineCell AdhesionHumansSulfonesCell ProliferationTissue EngineeringOsteoblastMembranes Artificialbody regionsEndothelial stem cellMembranemedicine.anatomical_structureMechanics of MaterialsCell cultureCeramics and CompositesBiophysicshuman activitiesPorosityBiomaterials
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Self-adjuvanting C18 lipid vinil sulfone-PP2A vaccine: study of the induced immunomodulation against

2017

Despite the importance of the adjuvant in the immunization process, very few adjuvants merge with the antigens in vaccines. A synthetic self-adjuvant oleic-vinyl sulfone (OVS) linked to the catalytic region of recombinant serine/threonine phosphatase 2A from the nematode Angiostrongylus costaricensis (rPP2A) was used for intranasal immunization in mice previously infected with Trichuris muris. The animal intranasal immunization with rPP2A-OVS showed a reduction of 99.01% in the number of the nematode eggs and 97.90% in adult. The immunohistochemical analysis of the intestinal sections showed that in immunized animals with lipopeptide the mucus was significantly higher than in the other expe…

Chemokine CCL111001Gene Expressionchemical and pharmacologic phenomenachemokines199LipopeptidesMiceMice Inbred AKRAdjuvants ImmunologicAnimalsAmino Acid SequenceProtein Phosphatase 2SulfonesTrichuriasisIntestinal Mucosalipid vinyl sulfoneParasite Egg CountAdministration IntranasalChemokine CCL20Vaccines Conjugate31InterleukinsResearchHelminth Proteins200Recombinant ProteinsTrichuris muris vaccinationcytokinesTrichurisTh17 CellsFemaleSequence AlignmentResearch Articleself-assembling lipopeptide rPP2AOpen biology
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Liquid chromatographic determination of planar aromatic sulphur compounds in crude oil

1989

Oxydation des dibenzothiophenes en sulfones et analyse par chromatographie liquide haute performance

ChromatographyChemistryOrganic Chemistrychemistry.chemical_elementGeneral MedicineCrude oilBiochemistrySulfurThin-layer chromatographyAnalytical ChemistrySulfonechemistry.chemical_compoundDibenzothiopheneOrganic chemistryJournal of Chromatography A
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Preferential solvation of a dicyanate ester monomer and poly(sulfone) in different organic solvents by size-exclusion chromatography.

2002

Preferential solvation parameters A in the ternary systems solvent (1) -monomer (2) -polymer (3) were determined as a tool to measure the compatibility between the cyanate ester monomer Arocy B10 and poly(sulfone), PSF, in the presence of three organic solvents: tetrahydrofuran, dimethylformamide and dicloromethane. The A parameter was measured by size-exclusion chromatography at different monomer-to-polymer ratios. The quantitative evaluation was rigorously made at polymer-diluted conditions. PSF was found to be preferentially solvated by the monomer. Concerning the solvent used, systems containing tetrahydrofuran showed the strongest solvation, the lowest A values being those obtained in …

ChromatographyPolymersViscosityIntrinsic viscosityOrganic ChemistrySize-exclusion chromatographySolvationGeneral MedicineBiochemistryAnalytical ChemistrySolventGel permeation chromatographychemistry.chemical_compoundMonomerchemistrySolubilityPolymer chemistryChromatography GelSolventsDimethylformamideSulfonesTetrahydrofuranCyanatesJournal of chromatography. A
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