Search results for "TRANES"

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Organic Polyradicals as Redox Mediators: Effect of Intramolecular Radical Interactions on Their Efficiency

2020

The spin–spin interactions between unpaired electrons in organic (poly)radicals, especially nitroxides, are largely investigated and are of crucial importance for their applications in areas such as organic magnetism, molecular charge transfer, or multiple spin labeling in structural biology. Recently, 2,2,6,6-tetramethylpiperidinyloxyl and polymers functionalized with nitroxides have been described as successful redox mediators in several electrochemical applications; however, the study of spin–spin interaction effect in such an area is absent. This communication reports the preparation of a novel family of discrete polynitroxide molecules, with the same number of radical units but differe…

Materials scienceRedox mediatorsRadical02 engineering and technology010402 general chemistryPhotochemistryElectrochemistry01 natural sciencesRedoxlaw.inventiontitanatraneslawTitanatranesnitroxidesspin−spin interactionsMoleculeSettore CHIM/01 - Chimica AnaliticaGeneral Materials SciencepolymeeritElectron paramagnetic resonanceElectrochemical potentialSpin−spin interactionsNitroxides; Redox mediators; Spin−spin interactions; TEMPO; Titanatranes; μ-oxo complexesNitroxidesSettore CHIM/06 - Chimica Organicapolymeerikemia021001 nanoscience & nanotechnologysähkökemia0104 chemical sciencesredox mediatorsμ-oxo complexesUnpaired electronIntramolecular forceorgaaninen kemiaspin-spin interactionsCondensed Matter::Strongly Correlated Electrons0210 nano-technologyTEMPOResearch ArticleACS Applied Materials & Interfaces
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Nepārtraukta starojuma lāzera ietekme uz ādas autofluorescences dzīves laiku

2015

Ar spektroskopijas metodēm (ādas autofluorescences ierosināšana un emisijas spektru novērošana) nav iespējams izšķirt spektru veidojošās komponentes. Ar laikā izšķirtu spektroskopiju iegūtos datus aproksimējot ar trīs komponentēm un apstrādājot ar metodēm TRES un TRANES, ir iespējams izšķirt spektru veidojošas komponentes un novērot nepārtraukta lāzerstarojuma ietekmi uz komponenšu dzīves laikiem. Autofluorescences dzīves laiki var mainīties – pieaugt vai samazināties - atkarībā no apstarošanai izmatotā viļņa garuma un izvēlēta diapazona. Izmantojot TRANES apstrādes metodi, pēc fotoizbalēšanas tika novērota emisijas maksimuma nobīde, kas liecina par fluoroforu sadalījuma izmaiņu fotoizbalēš…

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