Search results for "Troposphere"

Physicochemistry of the Atmosphere

2016

2020

Abstract. The vertical distribution and seasonal variation of water vapour volume mixing ratio (H2O VMR), of relative humidity with respect to ice (RHice) and particularly of regions with ice-supersaturated air masses (ISSRs) in the extratropical upper troposphere and lowermost stratosphere are investigated at northern mid-latitudes over the eastern North American, North Atlantic and European regions for the period 1995 to 2010. Observation data originate from regular and continuous long-term measurements on board instrumented passenger aircraft in the framework of the European research programme MOZAIC (1994–2010), which continues as the European research infrastructure IAGOS (from 2011). …

Aircraft-based observations of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX-SOA) in the tropical upper troposphere over the Amazon reg…

2018

During the ACRIDICON-CHUVA field project (September–October 2014; based in Manaus, Brazil) aircraft-based in situ measurements of aerosol chemical composition were conducted in the tropical troposphere over the Amazon using the High Altitude and Long Range Research Aircraft (HALO), covering altitudes from the boundary layer (BL) height up to 14.4 km. The submicron non-refractory aerosol was characterized by flash-vaporization/electron impact-ionization aerosol particle mass spectrometry. The results show that significant secondary organic aerosol (SOA) formation by isoprene oxidation products occurs in the upper troposphere (UT), leading to increased organic aerosol mass concentratio…

Impact of the Asian monsoon on the extratropical lower stratosphere: trace gas observations during TACTS over Europe 2012

2016

Abstract. The transport of air masses originating from the Asian monsoon anticyclone into the extratropical upper troposphere and lower stratosphere (Ex-UTLS) above potential temperatures Θ =  380 K was identified during the HALO aircraft mission TACTS in August and September 2012. In situ measurements of CO, O3 and N2O during TACTS flight 2 on 30 August 2012 show the irreversible mixing of aged stratospheric air masses with younger (recently transported from the troposphere) ones within the Ex-UTLS. Backward trajectories calculated with the trajectory module of CLaMS indicate that these tropospherically affected air masses originate from the Asian monsoon anticyclone. These air masses are …

2019

Abstract. The evolution of the tropopause inversion layer (TIL) during cyclogenesis in the North Atlantic storm track is investigated using operational meteorological analysis data (Integrated Forecast System from the European Centre for Medium-Range Weather Forecasts). For this a total of 130 cyclones have been analysed during the months August through October between 2010 and 2014 over the North Atlantic. Their paths of migration along with associated flow features in the upper troposphere and lower stratosphere (UTLS) have been tracked based on the mean sea level pressure field. Subsets of the 130 cyclones have been used for composite analysis using minimum sea level pressure to filter t…

Characterization of transport regimes and the polar dome during Arctic spring and summer using in situ aircraft measurements

2019

The springtime composition of the Arctic lower troposphere is to a large extent controlled by the transport of midlatitude air masses into the Arctic. In contrast, precipitation and natural sources play the most important role during summer. Within the Arctic region sloping isentropes create a barrier to horizontal transport, known as the polar dome. The polar dome varies in space and time and exhibits a strong influence on the transport of air masses from midlatitudes, enhancing transport during winter and inhibiting transport during summer. We analyzed aircraft-based trace gas measurements in the Arctic from two NETCARE airborne field campaigns (July 2014 and April 2015) with the Alfred W…

SOUTHTRAC-GW: An airborne field campaign to explore gravity wave dynamics at the world’s strongest hotspot

2021

The southern part of South America and the Antarctic peninsula are known as the world’s strongest hotspot region of stratospheric gravity wave (GW) activity. Large tropospheric winds are deflected by the Andes and the Antarctic Peninsula and excite GWs that might propagate into the upper mesosphere. Satellite observations show large stratospheric GW activity above the mountains, the Drake Passage, and in a belt centered along 60°S. This scientifically highly interesting region for studying GW dynamics was the focus of the Southern Hemisphere Transport, Dynamics, and Chemistry–Gravity Waves (SOUTHTRAC-GW) mission. The German High Altitude and Long Range Research Aircraft (HALO) was deployed …

Cold cloud microphysical process rates in a global chemistry–climate model

2021

Microphysical processes in cold clouds which act as sources or sinks of hydrometeors below 0 ∘C control the ice crystal number concentrations (ICNCs) and in turn the cloud radiative effects. Estimating the relative importance of the cold cloud microphysical process rates is of fundamental importance to underpin the development of cloud parameterizations for weather, atmospheric chemistry, and climate models and to compare the output with observations at different temporal resolutions. This study quantifies and investigates the ICNC rates of cold cloud microphysical processes by means of the chemistry–climate model EMAC (ECHAM/MESSy Atmospheric Chemistry) and defines the hierarchy of sources…

2021

Abstract. Warm conveyor belts (WCBs) are important airstreams in extratropical cyclones, often leading to the formation of intense precipitation and the amplification of upper-level ridges. This study presents a case study that involves aircraft, lidar and radar observations in a WCB ascending from western Europe towards the Baltic Sea during the Hydrological Cycle in the Mediterranean Experiment (HyMeX) and T-NAWDEX-Falcon in October 2012, a preparatory campaign for the THORPEX North Atlantic Waveguide and Downstream Impact Experiment (T-NAWDEX). Trajectories were used to link different observations along the WCB, that is, to establish so-called Lagrangian matches between observations. To …

A convolution of observational and model data to estimate age of air spectra in the northern hemispheric lower stratosphere

2020

Abstract. Derivation of mean age of air (AoA) and age spectra from atmospheric measurements remains a challenge and often requires data from atmospheric models. This study tries to minimize the direct influence of model data and presents an extension and application of a previously established inversion method to derive age spectra from mixing ratios of long- and short-lived trace gases. For a precise description of cross-tropopause transport processes, the inverse method is extended to incorporate air entrainment into the stratosphere across the tropical and extratropical tropopause. We first use simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) to provide a genera…