Search results for "Troposphere"
showing 10 items of 206 documents
Overview of aerosol properties associated with air masses sampled by the ATR-42 during the EUCAARI campaign (2008)
2013
Abstract. Within the frame of the European Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) project the Météo-France aircraft ATR-42 performed 22 research flights, over central Europe and the North Sea during the intensive observation period in May 2008. For the campaign, the ATR-42 was equipped in order to study aerosol physical, chemical and optical properties, as well as cloud microphysics. During the campaign, continental air masses from Eastern and Western Europe were encountered, along with polar and Scandinavian air masses. For the 22 research flights, retroplume analyses along the flight tracks were performed with FLEXPART in order to classify air masses into five sector…
Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere: insights into the transport pathways and t…
2021
We report on measurements of total bromine (Brtot) in the upper troposphere and lower stratosphere taken during 15 flights with the German High Altitude and LOng range research aircraft (HALO). The research campaign WISE (Wave-driven ISentropic Exchange) included regions over the North Atlantic, Norwegian Sea, and northwestern Europe in fall 2017. Brtot is calculated from measured total organic bromine (Brorg) added to inorganic bromine (Bryinorg), evaluated from measured BrO and photochemical modeling. Combining these data, the weighted mean [Brtot] is 19.2±1.2 ppt in the northern hemispheric lower stratosphere (LS), in agreement with expectations for Brtot in the middle stratosphere (Enge…
Seasonal variations in aerosol particle composition at the puy-de-Dôme research station in France
2011
Detailed investigations of the chemical and microphysical properties of atmospheric aerosol particles were performed at the puy-de-Dôme (pdD) research station (1465 m) in autumn (September and October 2008), winter (February and March 2009), and summer (June 2010) using a compact Time-of-Flight Aerosol Mass Spectrometer (cToF-AMS). Over the three campaigns, the average mass concentrations of the non-refractory submicron particles ranged from 10 μg m<sup>&minus;3</sup> up to 27 μg m<sup>&minus;3</sup>. Highest nitrate and ammonium mass concentrations were measured during the winter and during periods when marine modified airmasses were arriving at the site, wh…
The Asian tropopause aerosol layer within the 2017 monsoon anticyclone: microphysical properties derived from aircraft-borne in situ measurements
2021
The Asian summer monsoon is an effective pathway for aerosol particles and precursors from the planetary boundary layer over Central, South, and East Asia into the upper troposphere and lower stratosphere. An enhancement of aerosol particles within the Asian monsoon anticyclone (AMA), called the Asian tropopause aerosol layer (ATAL), has been observed by satellites. We discuss airborne in situ and remote sensing observations of aerosol microphysical properties conducted during the 2017 StratoClim field campaign within the AMA region. The aerosol particle measurements aboard the high-altitude research aircraft M55 Geophysica (maximum altitude reached of ∼20.5 km) were conducted with a modifi…
Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N
2021
We analyse aerosol particle composition measurements from five research missions between 2014 and 2018 to assess the meridional extent of particles containing meteoric material in the upper troposphere and lower stratosphere (UTLS). Measurements from the Jungfraujoch mountaintop site and a low-altitude aircraft mission show that meteoric material is also present within middle- and lower-tropospheric aerosol but within only a very small proportion of particles. For both the UTLS campaigns and the lower- and mid-troposphere observations, the measurements were conducted with single-particle laser ablation mass spectrometers with bipolar-ion detection, which enabled us to measure the chemical c…
Airborne measurements of dust layer properties, particle size distribution and mixing state of Saharan dust during SAMUM 2006
2009
The Saharan Mineral Dust Experiment (SAMUM) was conducted in May/June 2006 in southern Morocco. As part of SAMUM, airborne in situ measurements of the particle size distribution in the diameter range 4 nm < Dp < 100 μm were conducted. The aerosol mixing state was determined below Dp < 2.5 μm. Furthermore, the vertical structure of the dust layers was investigated with a nadir-looking high spectral resolution lidar (HSRL). The desert dust aerosol exhibited two size regimes of different mixing states: below 0.5 μm, the particles had a non-volatile core and a volatile coating; larger particles above 0.5 μm consisted of non-volatile components and contained light absorbing material. In…
Regional Saharan dust modelling during the SAMUM 2006 campaign
2011
The regional dust model system LM-MUSCAT-DES was developed in the framework of the SAMUM project. Using the unique comprehensive data set of near-source dust properties during the 2006 SAMUM field campaign, the performance of the model system is evaluated for two time periods in May and June 2006. Dust optical thicknesses, number size distributions and the position of the maximum dust extinction in the vertical profiles agree well with the observations. However, the spatio-temporal evolution of the dust plumes is not always reproduced due to inaccuracies in the dust source placement by the model. While simulated winds and dust distributions are well matched for dust events caused by dry syn…
Quantifying transport into the lowermost stratosphere using simultaneous in-situ measurements of SF&lt;sub&gt;6&lt;/sub&gt; and CO&am…
2009
Abstract. The seasonality of transport and mixing of air into the lowermost stratosphere (LMS) is studied using distributions of mean age of air and a mass balance approach, based on in-situ observations of SF6 and CO2 during the SPURT (Spurenstofftransport in der Tropopausenregion, trace gas transport in the tropopause region) aircraft campaigns. Combining the information of the mean age of air and the water vapour distributions we demonstrate that the tropospheric air transported into the LMS above the extratropical tropopause layer (ExTL) originates predominantly from the tropical tropopause layer (TTL). The concept of our mass balance is based on simultaneous measurements of the two pas…
Synoptic-scale variability of the polar and subpolar tropopause: Data analysis and idealized PV inversions
2002
The synoptic-scale variability of the polar and subpolar tropopause is investigated based on radiosonde and European Centre for Medium-Range Weather Forecasts Reanalysis data in combination with idealized potential vorticity (PV) inversions. A regression analysis is performed to examine the relationship between the relative vorticity at tropopause level, the tropopause displacement, the static stability above the tropopause, and the anomalies of tropopause temperature and potential temperature. The results are compared with regression coefficients computed from a large number of PV inversions. Generally, a cyclonically influenced tropopause is lower, warmer and potentially colder than avera…
Evidence for heterogeneous chlorine activation in the tropical UTLS
2011
Airborne in-situ observations of ClO in the tropics were made during the TROCCINOX (Aracatuba, Brazil, February 2005) and SCOUT-O<sub>3</sub> (Darwin, Australia, November/December 2005) field campaigns. While during most flights significant amounts of ClO (≈10–20 parts per trillion, ppt) were present only in aged stratospheric air, instances of enhanced ClO mixing ratios of up to 40 ppt – significantly exceeding those expected from gas phase chemistry – were observed in air masses of a more tropospheric character. Most of these observations are associated with low temperatures or with the presence of cirrus clouds (often both), suggesting that cirrus ice particles and/or liquid …