Search results for "Uranium-236"
showing 3 items of 3 documents
Determination of extremely low (236)U/(238)U isotope ratios in environmental samples by sector-field inductively coupled plasma mass spectrometry usi…
2005
A method by inductively coupled plasma mass spectrometry (ICP-MS) was developed which allows the measurement of (236)U at concentration ranges down to 3 x 10(-14)g g(-1) and extremely low (236)U/(238)U isotope ratios in soil samples of 10(-7). By using the high-efficiency solution introduction system APEX in connection with a sector-field ICP-MS a sensitivity of more than 5,000 counts fg(-1) uranium was achieved. The use of an aerosol desolvating unit reduced the formation rate of uranium hydride ions UH(+)/U(+) down to a level of 10(-6). An abundance sensitivity of 3 x 10(-7) was observed for (236)U/(238)U isotope ratio measurements at mass resolution 4000. The detection limit for (236)U a…
Uranium from German Nuclear Power Projects of the 1940s— A Nuclear Forensic Investigation
2015
Here we present a nuclear forensic study of uranium from German nuclear projects which used different geometries of metallic uranium fuel. Through measurement of the (230)Th/(234)U ratio, we could determine that the material had been produced in the period from 1940 to 1943. To determine the geographical origin of the uranium, the rare-earth-element content and the (87)Sr/(86)Sr ratio were measured. The results provide evidence that the uranium was mined in the Czech Republic. Trace amounts of (236)U and (239)Pu were detected at the level of their natural abundance, which indicates that the uranium fuel was not exposed to any major neutron fluence.
Variable masses in fission and heavy-ion collisions
1972
With the use of the cranking formula, the coordinate-dependent mass parameters of the kinetic-energy operator in fission processes and heavy-ion collisions are calculated in the two-center oscillator model. It is shown that the reduced mass and also the classical moment of inertia are obtained for large separations of the fragments. For small separations, however, the mass parameter for the motion of the centers of mass of the fragments is larger than the reduced mass by an order of magnitude.