Search results for "aerosol"
showing 10 items of 722 documents
Contrast in column-integrated aerosol optical properties during heating and non-heating seasons at Urumqi — Its causes and implications
2017
Abstract Aerosol optical properties were retrieved from two years' worth of Sunphotometer measurements at Urumqi, an urban station in western China. Distinct seasonal variations of aerosol optical properties were revealed. During the heating season, mean aerosol optical depth at 550 nm (τ a ), Angstrom exponent calculated from aerosol optical depth at wavelength of 440 and 870 nm (α) as well as PM 2.5 concentration were 0.58 ± 0.33, 1.11 ± 0.34 and 79.5 ± 69.6 μg m − 3 , respectively, which contrasted their counterparts during the non-heating season of 0.32 ± 0.22, 0.79 ± 0.26, and 35.0 ± 20.1 μg m − 3 . Seasonal variations of τ a and PM 2.5 at Urumqi contrasted with corresponding values in…
Determination and analysis of in situ spectral aerosol optical properties by a multi-instrumental approach
2014
Continuous in situ measurements of aerosol optical properties were conducted from 29 June to 29 July 2012 in Granada (Spain) with a seven-wavelength Aethalometer, a Multi-Angle Absorption Photometer, and a three-wavelength integrating nephelometer. The aim of this work is to describe a methodology to obtain the absorption coefficients (babs) for the different Aethalometer wavelengths. In this way, data have been compensated using algorithms which best estimate the compensation factors needed. Two empirical factors are used to infer the absorption coefficients from the Aethalometer measurements: C – the parameter describing the enhancement of absorption by particles in the filter matrix due …
The June 2007 Saharan dust event in the central Mediterranean: Observations and radiative effects in marine, urban, and sub-urban environments
2011
Abstract A desert dust episode in June 2007 and its radiative effects on the energy budget have been studied at three Italian stations (Rome, Lecce and Lampedusa) with the aim of investigating the interactions with different conditions and aerosol types over the Mediterranean. The three sites are representative for urban (Rome), sub-urban/rural (Lecce), and marine (Lampedusa) environment, respectively in the central Mediterranean region. Measured ground-based column-averaged aerosol optical properties and aerosol extinction profiles were used to initialize the MODTRAN4 radiative transfer model. The radiative transfer model was used to estimate the shortwave aerosol radiative forcing ( ARF )…
Sources of discrepancy between aerosol optical depth obtained from AERONET and in-situ aircraft profiles
2012
Abstract. Aerosol optical properties were measured by NOAA's Airborne Aerosol Observatory over Bondville, Illinois, during more than two years using a light aircraft. Measured properties included total light scattering, backscattering, and absorption, while calculated parameters included aerosol optical depth (AOD), Ångström exponent, single-scattering albedo, hemispheric backscatter fraction, asymmetry parameter, and submicrometer mode fraction of scattering. The in-situ aircraft measurements are compared here with AERONET measurements and retrievals of the aerosol optical properties at the same location, although it is difficult to verify the AERONET retrieval algorithm at a site that is …
Aerosol influence on radiative cooling
2011
Aerosol particles have a complex index of refraction and therefore contribute to atmospheric emission and radiative cooling rates. In this paper calculations of the longwave flux divergence within the atmosphere at different heights are presented including water vapour and aerosol particles as emitters and absorbers. The spectral region covered is 5 to 100 microns divided into 23 spectral intervals. The relevant properties of the aerosol particles, the single scattering albedo and the extinction coefficient, were first calculated by Mie-theory and later by an approximation formula with a complex index of refraction given by Volz. The particle growth with relative humidity is also incorporat…
Aerosol columnar properties retrieved from CIMEL radiometers during VELETA 2002
2008
During the 2002 summer, the VELETA 2002 field campaign has been carried out at the Sierra Nevada Massif, close to Granada in South-Eastern Spain. During the campaign, CIMEL CE-318 robotic radiometer has been one of the key instruments in the characterization of the atmospheric aerosol columnar properties. This kind of radiometers have been operated at Motril, a coastal location at sea level, Pitres (1200 m a.s.l.), located in the South slope of Sierra Nevada Massif, Las Sabinas (2200m a.s.l.), located on the north slope of the mountain range, and Armilla (680m a.s.l.), located in the valley. The principal feature of the locations is that they provide a strong altitudinal gradient. This work…
Columnar aerosol properties in a Northeastern Atlantic site (Plymouth, United Kingdom) by means of ground based skyradiometer data during years 2000-…
2012
Between 2000 and 2008, columnar optical and radiative properties were measured at the Plymouth Marine Laboratory (PML), UK (50° 21.95'N, 4° 8.85'W) using an automatic Prede POM01L sun-sky photometer. The database was analyzed for aerosol optical properties using the SKYRAD radiative inversion algorithm and calibrated using the in situ SKYIL calibration method. Retrievals include aerosol optical depth, ångström wavelength exponent, aerosol volume distribution, refractive index and single scattering albedo. The results show that the Plymouth site is characterized by low values of aerosol optical depth with low variability (0.18 ± 0.08 at 500 nm) and a mean annual ångström exponent of 1.03 ± 0…
Sensitivity of tropospheric chemical composition to halogen-radical chemistry using a fully coupled size-resolved multiphase chemistry–global climate…
2014
Observations and model calculations indicate that highly non-linear multiphase atmospheric processes involving inorganic Cl and Br significantly impact tropospheric chemistry and composition, aerosol evolution, and radiative transfer. The sensitivity of global atmospheric chemistry to the production of marine aerosol and the associated activation and cycling of inorganic Cl and Br was investigated using a size-resolved multiphase coupled chemistry–global climate model (National Center for Atmospheric Research's Community Atmosphere Model (CAM) v3.6.33). Simulated results revealed strong meridional and vertical gradients in Cl and Br species. They also point to possible physicochemical mecha…
Improvements of organic aerosol representations and their effects in large-scale atmospheric models
2012
Organics dominate the composition of the atmospheric aerosol, especially in the fine mode, influencing some of its characteristics such as the hygroscopicity, which is of climatic relevance for the Earth system. This study targets an improvement in the description of organic aerosols suitable for large-scale modelling, making use of recent developments based on laboratory and field measurements. In addition to the organic mass and particle number distribution, the proposed method keeps track of the oxidation state of the aerosol based on the OH exposure time, describing some of its chemical characteristics. This study presents the application of the method in a global chemistry climate mode…
Bioaerosols in the Earth system: Climate, health, and ecosystem interactions
2016
Abstract Aerosols of biological origin play a vital role in the Earth system, particularly in the interactions between atmosphere, biosphere, climate, and public health. Airborne bacteria, fungal spores, pollen, and other bioparticles are essential for the reproduction and spread of organisms across various ecosystems, and they can cause or enhance human, animal, and plant diseases. Moreover, they can serve as nuclei for cloud droplets, ice crystals, and precipitation, thus influencing the hydrological cycle and climate. The sources, abundance, composition, and effects of biological aerosols and the atmospheric microbiome are, however, not yet well characterized and constitute a large gap i…