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General overview: European Integrated project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI)-integrating aerosol research from nano …
2011
In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan…
The Fifth International Workshop on Ice Nucleation phase 2 (FIN-02): Laboratory intercomparison of ice nucleation measurements
2018
The second phase of the Fifth International Ice Nucleation Workshop (FIN-02) involved the gathering of a large number of researchers at the Karlsruhe Institute of Technology's Aerosol Interactions and Dynamics of the Atmosphere (AIDA) facility to promote characterization and understanding of ice nucleation measurements made by a variety of methods used worldwide. Compared to the previous workshop in 2007, participation was doubled, reflecting a vibrant research area. Experimental methods involved sampling of aerosol particles by direct processing ice nucleation measuring systems from the same volume of air in separate experiments using different ice nucleating particle (INP) types, and coll…
New investigations on homogeneous ice nucleation: the effects of water activity and water saturation formulations
2022
Laboratory measurements at the AIDA cloud chamber and airborne in-situ observations suggest that the homogeneous freezing thresholds at low temperatures are possibly higher than expected from the so-called “Koop-line”. This finding is of importance, because the ice onset relative humidity affects the cirrus cloud coverage and, at the very low temperatures of the tropical tropopause layer, together with the number of ice crystals also the transport of water vapor into the stratosphere. Both, the appearance of cirrus clouds and the amount of stratospheric water feed back to the radiative budget of the atmosphere. In order to explore the enhanced ice onset humidities, we re-examine…
A New Look at Homogeneous Ice Nucleation in Supercooled Water Drops
1995
Abstract The classical theory for homogeneous ice nucleation in supercooled water is investigated in the light of recent data published in various physico-chemical journal on the physical properties of supercooled water and in the light of recent evidence that the cooperative nature of the hydrogen bonds between water molecules is responsible for a singularity behavior of pure supercooled water at −45°C. Recent rates for homogeneous ice nucleation in supercooled water drops field from field experiments at the cirrus cloud level and from cloud chamber studies were shown to be quantitatively in agreement with the laboratory-derived lowest temperatures to which ultrapure water drops of a given…
Variation of H2O/CO2and CO2/SO2ratios of volcanic gases discharged by continuous degassing of Mount Etna volcano, Italy
2008
[1] We applied the Multi-GAS technique to measure compositions of the volcanic plumes continuously discharged from summit craters of Voragine, Northeast and Bocca Nuova at Mount Etna, in an attempt to estimate compositions of the source volcanic gases. The estimated CO2/SO2 and H2O/CO2 ratios of the volcanic gases show a large variation ranging from 0.6 to 30 and from 1 to 18, respectively. This variability overlaps with the compositional range of dissolved volatiles in melt inclusions and their coexisting bubbles in a magma chamber and can be caused by the low-pressure degassing of a magma with variable bubble content ranging from 0.3 to 15 wt.%. The variable bubble content in the magma is…
Application of an O-ring pinch device as a constant-pressure inlet (CPI) for airborne sampling
2020
We present a novel and compact design of a constant-pressure inlet (CPI) developed for use in airborne aerosol mass spectrometry. In particular, the inlet system is optimized for aerodynamic lenses commonly used in aerosol mass spectrometers, in which efficient focusing of aerosol particles into a vacuum chamber requires a precisely controlled lens pressure, typically of a few hectopascals. The CPI device can also be used in condensation particle counters (CPCs), cloud condensation nucleus counters (CCNCs), and gas-phase sampling instruments across a wide range of altitudes and inlet pressures. The constant pressure is achieved by changing the inner diameter of a properly scaled O-ring that…
Evidence of deep magma degassing and ascent by geochemistry of peripheral gas emissions at Mount Etna (Italy): Assessment of the magmatic reservoir p…
2003
[1] Five gas discharges in the area of Mount Etna volcano (Italy) and in the near Hyblean plateau have been monitored since 1996. All the emissions displayed low contributions from crustal fluids, whereas magmatic gases were the main component. Selective dissolution of these gases into hydrothermal aquifers has been recognized and modeled, allowing us to calculate the original composition of the magma-released gases. The inferred composition of the magmatic gases exhibits synchronous variations of He/Ne and He/CO2 ratios, which are coherent with the magma degassing process. On the basis of numerical simulations of volatile degassing from Etnean basalts we have computed the initial and final…
Lower Cretaceous tholeiitic dyke swarms from the Ponta Grossa Arch (southeast Brazil): Petrology, Sr-Nd isotopes and genetic relationships with the P…
1990
The Lower Cretaceous dykes of the Ponta Grossa Arch, the most important dyke swarms in Brazil, are associated with the flood basalts and rare acid flows of the northern Parana basin. The Ponta Grossa (PG) dykes are formed by two-pyroxene tholeiites and rare acid rocks. The basaltic dykes may be distinguished into two main groups: a dominant, high-TiO2 (> 2 wt.%; HTi) group and a subordinate, low-TiO2 (< 2 wt.%; LTi) group, characterized, for similar MgO content, by high and low incompatible-element contents, respectively. Most PG dykes do not show chemical and isotope evidence supporting important crustal contamination. PG dykes with (87Sr86Sr)0 < 0.7060 plot in the mantle array (ϵSr ≈ + 17…
Lever Press Duration as a Measure of Frustration Motivated Response Variation in Rat Self-administration to Investigate the Effects of Frustration on…
2023
In human studies, frustration has been identified as a potential risk factor for substance use disorders. Currently, there is little research into the role of frustration in substance use disorders despite research showing that frustration tolerance in humans is associated with a lower likelihood of developing substance use problems, better outcomes in recovery, and fewer relapses. To address this need, our studies use rat self-administration models to focus on frustration-related behavior in natural reward and addiction-related behavioral procedures. First, to study frustration in operant responding, there is a need to establish a real-time objective measure and validate its use in predict…
Ocular biometry with swept-source optical coherence tomography
2020
This study aimed to summarize the outcomes reported when swept-source optical coherence tomography (SS-OCT) is used for ocular biometry. A literature search was performed to identify publications reporting clinical outcomes of patients measured with commercial SS-OCT. Twenty-nine studies were included in this review. A comprehensive analysis of the available data was performed, focusing on parameters used for intraocular lens (IOL) power calculation in cataract surgery, including keratometry, central corneal thickness, white-to-white distance, anterior chamber depth, lens thickness, axial length, IOL power, and pupil diameter. Different metrics for repeatability, reproducibility, and agreem…