Search results for "atomic physics"

showing 10 items of 5530 documents

The electron affinity of astatine

2020

One of the most important properties influencing the chemical behavior of an element is the electron affinity (EA). Among the remaining elements with unknown EA is astatine, where one of its isotopes, 211At, is remarkably well suited for targeted radionuclide therapy of cancer. With the At− anion being involved in many aspects of current astatine labeling protocols, the knowledge of the electron affinity of this element is of prime importance. Here we report the measured value of the EA of astatine to be 2.41578(7) eV. This result is compared to state-of-the-art relativistic quantum mechanical calculations that incorporate both the Breit and the quantum electrodynamics (QED) corrections and…

Atomic Physics (physics.atom-ph)ENERGIESGeneral Physics and AstronomyElectron01 natural sciences7. Clean energyPhysics - Atomic PhysicsElectronegativityastatiinielectron affinityPhysics::Atomic Physicslcsh:SciencePhysicsMultidisciplinary010304 chemical physicsIsotopeQELECTRONEGATIVITYMultidisciplinary SciencesHalogenScience & Technology - Other Topicsddc:500Atomic physicsBASIS-SET CONVERGENCE[CHIM.RADIO]Chemical Sciences/RadiochemistryRadioactive decayChemical physicsAstrophysics::High Energy Astrophysical PhenomenaScienceComputer Science::Neural and Evolutionary ComputationOther Fields of PhysicsPOTENTIALSFOS: Physical scienceschemistry.chemical_elementphysics.atom-phGeneral Biochemistry Genetics and Molecular BiologyArticleIonElectron affinity0103 physical sciences[CHIM]Chemical Sciences010306 general physicsAstatineDETECTORScience & TechnologySTABILITYRadiochemistry500General Chemistrychemistrylcsh:Qastatine
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Rydberg excitation of cold atoms inside a hollow core fiber

2017

We report on a versatile, highly controllable hybrid cold Rydberg atom fiber interface, based on laser cooled atoms transported into a hollow core Kagom\'{e} crystal fiber. Our experiments are the first to demonstrate the feasibility of exciting cold Rydberg atoms inside a hollow core fiber and we study the influence of the fiber on Rydberg electromagnetically induced transparency (EIT) signals. Using a temporally resolved detection method to distinguish between excitation and loss, we observe two different regimes of the Rydberg excitations: one EIT regime and one regime dominated by atom loss. These results are a substantial advancement towards future use of our system for quantum simulat…

Atomic Physics (physics.atom-ph)Electromagnetically induced transparencyFOS: Physical sciencesPhysics::Optics02 engineering and technology01 natural scienceslaw.inventionPhysics - Atomic Physicssymbols.namesakelaw0103 physical sciencesAtomRydberg matterFiberPhysics::Atomic Physics010306 general physicsPhysicsQuantum Physics021001 nanoscience & nanotechnologyLaserRydberg atomRydberg formulasymbolsAtomic physicsQuantum Physics (quant-ph)0210 nano-technologyExcitation
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Quantum localization and bound state formation in Bose-Einstein condensates

2010

We discuss the possibility of exponential quantum localization in systems of ultracold bosonic atoms with repulsive interactions in open optical lattices without disorder. We show that exponential localization occurs in the maximally excited state of the lowest energy band. We establish the conditions under which the presence of the upper energy bands can be neglected, determine the successive stages and the quantum phase boundaries at which localization occurs, and discuss schemes to detect it experimentally by visibility measurements. The discussed mechanism is a particular type of quantum localization that is intuitively understood in terms of the interplay between nonlinearity and a bou…

Atomic Physics (physics.atom-ph)FOS: Physical sciences01 natural sciencesSpectral linelocalization010305 fluids & plasmaslaw.inventionPhysics - Atomic PhysicslawQuantum mechanics0103 physical sciencesBound state010306 general physicsElectronic band structureQuantumPhysicsQuantum PhysicsAtomic and Molecular Physics and Optics3. Good healthExponential functionWeak localizationQuantum Gases (cond-mat.quant-gas)Excited stateQuantum electrodynamicsQuantum Physics (quant-ph)Condensed Matter - Quantum GasesBose–Einstein condensate
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Orientation and Alignment Echoes

2015

We present one of the simplest classical systems featuring the echo phenomenon---a collection of randomly oriented free rotors with dispersed rotational velocities. Following excitation by a pair of time-delayed impulsive kicks, the mean orientation or alignment of the ensemble exhibits multiple echoes and fractional echoes. We elucidate the mechanism of the echo formation by the kick-induced filamentation of phase space, and provide the first experimental demonstration of classical alignment echoes in a thermal gas of ${\mathrm{CO}}_{2}$ molecules excited by a pair of femtosecond laser pulses.

Atomic Physics (physics.atom-ph)FOS: Physical sciencesGeneral Physics and AstronomyPhysics - Classical PhysicsPhysics - Atomic Physicslaw.inventionOpticsFilamentationlawPhysics - Chemical PhysicsChemical Physics (physics.chem-ph)Physics[PHYS.PHYS.PHYS-OPTICS]Physics [physics]/Physics [physics]/Optics [physics.optics][PHYS.PHYS.PHYS-ATOM-PH]Physics [physics]/Physics [physics]/Atomic Physics [physics.atom-ph]business.industry[PHYS.PHYS.PHYS-ATM-PH]Physics [physics]/Physics [physics]/Atomic and Molecular Clusters [physics.atm-clus]Echo (computing)Classical Physics (physics.class-ph)LaserOrientation (vector space)Phase spaceExcited stateFemtosecondAtomic physicsbusinessExcitationPhysics - OpticsOptics (physics.optics)Physical Review Letters
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Heading-Error-Free Optical Atomic Magnetometry in the Earth-Field Range

2023

Alkali-metal atomic magnetometry is widely used due to its high sensitivity and cryogen-free operation. However, when operating in geomagnetic field, it suffers from heading errors originating from nonlinear Zeeman (NLZ) splittings and magnetic resonance asymmetries, which lead to difficulties in mobile-platform measurements. We demonstrate an alignment based $^{87}$Rb magnetometer, which, with only a single magnetic resonance peak and well-separated hyperfine transition frequencies, is insensitive or even immune to NLZ-related heading errors. It is shown that the magnetometer can be implemented for practical measurements in the geomagnetic environments and the photon-shot-noise-limited sen…

Atomic Physics (physics.atom-ph)FOS: Physical sciencesGeneral Physics and AstronomyPhysics::Atomic PhysicsPhysics - Atomic PhysicsPhysical Review Letters
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BASE-STEP: A transportable antiproton reservoir for fundamental interaction studies

2023

Currently, the only worldwide source of low-energy antiprotons is the AD/ELENA facility located at CERN. To date, all precision measurements on single antiprotons have been conducted at this facility and provide stringent tests of the fundamental interactions and their symmetries. However, the magnetic field fluctuations from the facility operation limit the precision of upcoming measurements. To overcome this limitation, we have designed the transportable antiproton trap system BASE-STEP to relocate antiprotons to laboratories with a calm magnetic environment. We anticipate that the transportable antiproton trap will facilitate enhanced tests of CPT invariance with antiprotons, and provide…

Atomic Physics (physics.atom-ph)FOS: Physical sciencesInstrumentation and Detectors (physics.ins-det)
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Resonance ionization spectroscopy of thorium isotopestowards a laser spectroscopic identification of the low-lying 7.6 eV isomer of 229Th

2011

International audience; In-source resonance ionization spectroscopy was used to identify an efficient and selective three step excitation/ionization scheme of thorium, suitable for titanium:sapphire (Ti:sa) lasers. The measurements were carried out in preparation of laser spectroscopic investigations for an identification of the low-lying 229 m Th isomer predicted at 7.6 ± 0.5 eV above the nuclear ground state. Using a sample of 232 Th, a multitude of optical transitions leading to over 20 previously unknown intermediate states of even parity as well as numerous high-lying odd parity auto-ionizing states were identified. Level energies were determined with an accuracy of 0.06 cm −1 for inte…

Atomic Physics (physics.atom-ph)FOS: Physical sciencesMass spectrometry01 natural sciences7. Clean energyIonlaw.inventionPhysics - Atomic PhysicslawIonization0103 physical sciences32.80.Zb42.62.Fi010306 general physicsSpectroscopyPhysics010308 nuclear & particles physics32.80.RmCondensed Matter PhysicsLaserAtomic and Molecular Physics and Optics32.30.-rAtomic physicsGround stateIsotopes of thoriumExcitation
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First-principles nonequilibrium Green's-function approach to transient photoabsorption: Application to atoms

2015

We put forward a first-principle NonEquilibrium Green's Function (NEGF) approach to calculate the transient photoabsorption spectrum of optically thin samples. The method can deal with pump fields of arbitrary strength, frequency and duration as well as for overlapping and nonoverlapping pump and probe pulses. The electron-electron repulsion is accounted for by the correlation self-energy, and the resulting numerical scheme deals with matrices that scale quadratically with the system size. Two recent experiments, the first on helium and the second on krypton, are addressed. For the first experiment we explain the bending of the Autler-Townes absorption peaks with increasing the pump-probe d…

Atomic Physics (physics.atom-ph)FOS: Physical sciencesNon-equilibrium thermodynamicschemistry.chemical_elementPhysics - Atomic PhysicsSettore FIS/03 - Fisica della MateriaIonsymbols.namesakeAtomic and Molecular Physics; OpticsAb initio quantum chemistry methodsAtomic and Molecular PhysicsMesoscale and Nanoscale Physics (cond-mat.mes-hall)nonequilibrium Green's-functionAbsorption (electromagnetic radiation)HeliumPhysicsta114Condensed Matter - Mesoscale and Nanoscale PhysicsKryptonOpticsFunction (mathematics)Atomic and Molecular Physics and OpticsphotoabsorptionchemistryGreen's functionsymbolsAtomic physicsPhysical Review A
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Reversed Dark Resonance in Rb Atom Excited by a Diode Laser

2000

Origin of recently discovered reversed (opposite sign) dark resonances was explained theoretically and verified experimentally. It is shown that the reason for these resonances is a specific optical pumping of ground state level in a transition when ground state angular momentum is smaller than the excited state momentum.

Atomic Physics (physics.atom-ph)FOS: Physical sciencesOptics (physics.optics)Physics - Atomic PhysicsPhysics - Optics
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Energy transfer reaction K(4s) + K(7s) \rightarrow K(4s) + K(5f), theory compared with experiment

2017

A comparison between theory and experiment, concerning the K(4s)+K(7s)\rightarrow K(4s)+K(5f) reaction of energy transfer in thermal collisions, is presented. Relevant cross sections are calculated for the potassium vapour temperatures in the range of 310-1000 K. They are based on the theoretical adiabatic K_2 potential energy curves and on the use of the multicrossing Landau-Zener model. In the temperature range of the present experiment, 428-451 K, the computed cross sections vary little, from 2.09x10^-14 cm^2 to 2.04x10^-14 cm^2, and agree well with the value 1.8(8)x10^-14 cm^2, which is the average of the corresponding experimental results.

Atomic Physics (physics.atom-ph)FOS: Physical sciencesPhysics - Atomic Physics
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