Search results for "bistability"
showing 10 items of 124 documents
Sub-nanosecond nonlinear pulse shaping in microfiber resonators
2009
Thanks to their small size and large index contrast allowing for tight field confinement, optical microfibers are of great interest in nonlinear optics. Their properties have recently been exploited in various devices for supercontinuum generation, pulse compression [1] and third-harmonic generation [2]. Combining field confinement and field enhancement in a loop or knot resonator can result in low-threshold non-linear microfibre devices, in which pulse shaping effects and bistability can be obtained. Such a behaviour has already been observed at a power level of ten milliwatts with millisecond time response, in the case of thermally-induced non-linearity in silica microfibres [3]. In contr…
Slow and fast nonlinearities in microfiber resonators
2008
Nonlinear optical properties of microfiber resonators are investigated. First, a miniature optical resonator standing in air is realized out of a silica microfiber, and measurements of the intensity transfer function show a wide variety of hysteresis cycles obtained at low scanning frequency of the input power. The results are satisfactorily interpreted through the action of thermally-induced nonlinear phase shifts. Secondly, we discuss the conditions under which the fast Kerr nonlinearity can be used efficiently in microfiber resonators under pulsed optical operation.
Near-field control of optical bistability in a nanocavity
2009
Micro- and nanocavities allow for strong light confinement in very small volume [1]. They give opportunities for new experiments such as cavity quantum electrodynamics, waveguiding, light slowing or trapping…[2] The increase of the electromagnetic (EM) field in the cavity enhances the interaction between light and matter, resulting in the possible observation of nonlinear effects [3]. Several studies have recently been published on the observation and characterisation of nonlinear silicon cavities [4]. As a step further, we propose and demonstrate the feasibility of an innovative way to mechanically control the bistable operating regime of a nanovavity. Using a near-field tip, we switch the…
Bistable Device based on the Kerr Effect in a Microfiber Resonator
2007
We propose a bistable device based on the Kerr effect in a microfiber resonator. Our simulations show that low switching powers (in the order of a few tens of mW) are expected with tellurite microfibers.
Étude et manipulation de modes résonants en champ proche optique
2010
Within the quick nano-fabrication techniques evolution and the increasing needs in low space and energy opto-electronic functions on-chip integration, studies and control of electromagnetic resonances of sub-micrometric objects are crucial issues. One aim of this work was then to improve our knowledge of the light-matter interaction. To this end, optical near-field experiments and complementary numerical development of models have been performed to study electromagnetic resonances due to light-matter interaction in sub-micrometric resonators. As an introduction, the first part of the manuscript presents the main phenomena involved in near-field optical microscopy and the used SNOM operation…
Theoretical study of microfiber resonator devices exploiting a phase shift
2008
Phase shifts within microfiber resonators can be exploited to demonstrate compact and fast-responding devices. Two examples, a sensor and a bistable device, where the origins of the phase shift are fundamentally different, are investigated. In the sensor the phase change originates from the change of refractive index of the medium surrounding the microfiber ring. This is a linear mechanism which translates into a change of resonance wavelength. Calculations of a silica microfiber ring immersed in an aqueous solution and operating at a wavelength of 1550 nm show that with a fiber 550 nm in diameter the sensitivity approaches a maximal value of about 1137 nm/RIU. In contrast to the sensitivit…
Towards low-energy-light-driven bistable photoswitches : ortho-fluoroaminoazobenzenes
2021
AbstractThermally stable photoswitches that are driven with low-energy light are rare, yet crucial for extending the applicability of photoresponsive molecules and materials towards, e.g., living systems. Combined ortho-fluorination and -amination couples high visible light absorptivity of o-aminoazobenzenes with the extraordinary bistability of o-fluoroazobenzenes. Herein, we report a library of easily accessible o-aminofluoroazobenzenes and establish structure–property relationships regarding spectral qualities, visible light isomerization efficiency and thermal stability of the cis-isomer with respect to the degree of o-substitution and choice of amino substituent. We rationalize the exp…
Scalable Electro-Optic Control of Localized Bistable Switching in Broad-Area VCSELs Using Reconfigurable Funnel Waveguides
2017
We demonstrate a steplike optical modulation based on the activation and deactivation of a bistable localized structure using a photoinduced and reconfigurable miniaturized 30 × 30 μm electroactivated funnel waveguide. Control of a single 10-μm-diameter spot in a 200-μm-diameter vertical-cavity surfaceemitting laser at 980 nm is achieved modulating the phase of an exciting beam in the specific position of the spot in the cavity. This localized on-off response can be scaled into arrays and offer a possible route to fast integrated optical logical functions and memory at low intensities at near-infrared wavelengths.
Downsizing of Nanocrystals While Retaining Bistable Spin Crossover Properties in Three-Dimensional Hofmann-Type {Fe(pz)[Pt(CN)4]}–Iodine Adducts
2021
Mastering nanostructuration of functional materials into electronic devices is presently an essential task in materials science. This is particularly relevant for spin crossover (SCO) compounds, whose properties are extremely sensitive to size reduction. Indeed, the search for materials displaying strong cooperative hysteretic SCO properties operative at the nanoscale close near room temperature is extremely challenging. In this context, we describe here the synthesis and characterization of 20-30 nm surfactant-free nanocrystals of the FeII Hofmann-type polymer {FeII(pz)[PtII,IVIx(CN)4]} (pz = pyrazine), which affords the first example of a robust three-dimensional coordination polymer, sub…