Search results for "boundary layer"

Dust emissions in the West African heat trough the role of the diurnal cycle and of extratropical disturbances

2008

The summertime West African heat trough (HT) is one of the most active dust sources in the world. A detailed case study during May/June 2006 based upon analyses from the European Centre for Medium-Range Weather Forecasts and a new Meteosat dust product illustrates two important mechanisms of dust emissions in this region: (1) The dry continental-scale HT circulation exhibits a strong diurnal cycle characterized by nocturnal low-level jets and downward mixing of momentum to the surface during the build-up of the planetary boundary layer in the morning. This leads to strong gusty surface winds and dust emission, mostly along the northern side of the HT, but also within the southerly monsoon f…

Airborne survey of trace gases and aerosols over the Southern Baltic Sea: from clean marine boundary layer to shipping corridor effect

2020

The influence of shipping on air quality over the Southern Baltic Sea was investigated by characterizing the horizontal and vertical distribution of aerosols and trace gases using airborne measurements in the summer of 2015. Generally, continental and anthropogenic emissions affected the vertical distribution of atmospheric pollutants, leading to pronounced stratification in and above the marine boundary layer and controlling the aerosol extinction. Marine traffic along the shipping corridor “Kadet Fairway” in the Arkona Basin is shown to influence the presence and properties of both trace gases and aerosol particles in the lowest atmospheric layer. Total particle number concentration and N…

2008

Abstract. Measurements of the submicron fraction of the atmospheric aerosol in the marine boundary layer were performed from January to March 2007 (Southern Hemisphere summer) onboard the French research vessel Marion Dufresne in the Southern Atlantic and Indian Ocean (20° S–60° S, 70° W–60° E). We used an Aerodyne High-Resolution-Time-of-Flight AMS to characterize the chemical composition and to measure species-resolved size distributions of non-refractory aerosol components in the submicron range. Within the "standard" AMS compounds (ammonium, chloride, nitrate, sulfate, organics) "sulfate" is the dominant species in the marine boundary layer with concentrations ranging between 50 ng m−3 …

Arctic low-level boundary layer clouds: in situ measurements and simulations of mono- and bimodal supercooled droplet size distributions at the top l…

2015

Abstract. Aircraft borne optical in situ size distribution measurements were performed within Arctic boundary layer clouds with a special emphasis on the cloud top layer during the VERtical Distribution of Ice in Arctic clouds (VERDI) campaign in April and May 2012. An instrumented Basler BT-67 research aircraft operated out of Inuvik over the Mackenzie River delta and the Beaufort Sea in the Northwest Territories of Canada. Besides the cloud particle and hydrometeor size spectrometers the aircraft was equipped with instrumentation for aerosol, radiation and other parameters. Inside the cloud, droplet size distributions with monomodal shapes were observed for predominantly liquid-phase Arct…

The effects of different radiation parametrizations on cloud evolution

1997

With the use of the microphysical stratus model (MISTRA), investigations into the effects of variations in the radiative-transfer parametrizations on cloud development have been undertaken. Two radiative-transfer schemes were coupled with the microphysical-thermodynamical section of MISTRA, one based on the exponential sumfitting method and the other based on the correlated k-distribution method of determining gaseous absorption properties. Model runs were initiated with parameter values in accordance with measurements made over the North Sea and comparisons made between model runs where only the radiation schemes were altered. Results indicated that differences between the two schemes had …

A numerical model of the cloud-topped planetary boundary-layer: Radiation, turbulence and spectral microphysics in marine stratus

1996

A numerical model of the cloud-topped planetary boundary-layer is presented. The model is one-dimensional with special emphasis on a detailed description of cloud microphysical processes. Aerosols and cloud droplets are treated in a two-dimensional particle-distribution whereby the activation of aerosols is calculated explicitly by solving the droplet-growth equation at all relative humidities. Atmospheric radiation is determined with a δ-two-stream radiation scheme. Turbulent fluxes are parametrized as a function of the turbulent kinetic energy. Numerical results are presented which are obtained by utilizing measurements made over the North Sea. The interaction between radiation, turbulenc…

Toward Parametrization of Precipitating Shallow Cumulus Cloud Organization via Moisture Variance

2021

The influence of the initial vertical moisture profile on precipitating shallow cumulus cloud organization in terms of the column‐averaged moisture variance is investigated using large‐eddy simulations. Five idealized simulations based on the Rain in Cumulus over the Ocean field experiment with different initial moisture profiles are investigated. All cases simulate precipitating shallow cumulus convection in a marine sub‐tropical region under large‐scale subsidence. The results show that the moisture variance is mainly generated through the interaction of the moisture flux and the moisture gradient in the gradient production term at the top of the boundary layer. The development is charact…

Temperature effect on phase state and reactivity controls atmospheric multiphase chemistry and transport of PAHs

2017

Atmospheric refrigerator increases the global transport and health risks of carcinogenic PAHs.

2017

Abstract. Ozone (O3) is an important atmospheric oxidant, a greenhouse gas, and a hazard to human health and agriculture. Here we describe airborne in situ measurements and model simulations of O3 and its precursors during tropical and extratropical field campaigns over South America and Europe, respectively. Using the measurements, net ozone formation/destruction tendencies are calculated and compared to 3-D chemistry–transport model simulations. In general, observation-based net ozone tendencies are positive in the continental boundary layer and the upper troposphere at altitudes above  ∼  6 km in both environments. On the other hand, in the marine boundary layer and the middle tropospher…

Airborne observation of mixing across the entrainment zone during PARADE 2011

2016

This study presents the analysis of the structure and air mass characteristics of the lower atmosphere during the field campaign PARADE (PArticles and RAdicals: Diel observations of the impact of urban and biogenic Emissions) on Mount Kleiner Feldberg in southwestern Germany during late summer 2011. We analysed measurements of meteorological variables (temperature, moisture, pressure, wind speed and direction) from radio soundings and of chemical tracers (carbon dioxide, ozone) from aircraft measurements. We focus on the thermodynamic and dynamic properties that control the chemical distribution of atmospheric constituents in the boundary layer. We show that the evolution of tracer profiles…