Search results for "circular"
showing 10 items of 856 documents
Electronic, magnetic, and structural properties of the ferrimagnet Mn2CoSn
2011
The magnetic ground state of the Heusler compound Mn${}_{2}$CoSn was predicted to be nearly half-metallic ferrimagnetic with a high spin polarization by ab initio electronic structure calculations. Mn${}_{2}$CoSn was synthesized, and the magnetic behavior of the compound was studied using a superconducting quantum interference device and x-ray magnetic circular dichroism. The experimental values were found to be in fair accordance with the theoretical predictions. The electronic structure and the crystal structure of Mn${}_{2}$CoSn were characterized comprehensively using x-ray powder diffraction, $^{119}\mathrm{Sn}$ M\"ossbauer spectroscopy, nuclear magnetic resonance, and hard x-ray photo…
Symmetry of molecular properties
1993
The symmetry of coefficients in the expansion of a given molecular property are shown to be obtainable through well defined tensor methods. The analytical expansions required of various vibrational and rotational tensors are given up to the fourth degree in dynamical variables. To illustrate the method, some rovibrational properties of spherical tops are considered. The symmetry of the associated molecular constants is expressed, simultaneously, for XY4 and XY6 molecules, by algebraic relations involving the independent constants and the coupling symbols of the molecular symmetry group. To allow comparisons, some examples are given for which the symmetry of the constants has been published …
Quantum simulations of toroidal electric ring currents and magnetic fields in linear molecules induced by circularly polarized laser pulses
2008
Circularly polarized laser pulses may excite state selective unidirectional toroidal electric ring currents around the axis of oriented linear molecules. These in turn induce state selective magnetic fields. Quantum simulations for AlCl show that these effects are about one or even more than three orders of magnitudes larger than those which may be prepared in oriented planar molecules such as Mg-porphyrin, by means of either circularly polarized laser pulses, or by traditional magnetic fields, respectively.
Element-specific magnetic moments and spin-resolved density of states in CoFeMnZ(Z=Al, Ga; Si, Ge)
2011
Using circular dichroism in x-ray-absorption spectroscopy (XAS/XMCD), we determined element-specific magnetic moments and spin-resolved unoccupied densities of states (DOS) for Co, Fe, and Mn in the quaternary Heusler compounds CoFeMn$Z$ ($Z=\text{Al}$, Ga; Si, Ge). These compounds belong to a class of highly spin-polarized materials with cubic LiMgPdSn-type structure. Different structure models for the sublattice occupation leading to similar average magnetization values can be distinguished by comparison of element-specific moments with theory. We find that the compounds form similar structures, where Co, Fe, Mn, and $Z$ occupy the $X$, ${X}^{\ensuremath{'}}$, $Y$, and $Z$ sublattice of t…
Hyperfine Paschen-Back regime in alkali metal atoms: consistency of two theoretical considerations and experiment
2013
Simple and efficient "\lambda-method" and "\lambda/2-method" (\lambda is the resonant wavelength of laser radiation) based on nanometric-thickness cell filled with rubidium are implemented to study the splitting of hyperfine transitions of 85Rb and 87Rb D_1 line in an external magnetic field in the range of B = 0.5 - 0.7 T. It is experimentally demonstrated from 20 (12) Zeeman transitions allowed at low B-field in 85Rb (87Rb) spectra in the case of \sigma+ polarized laser radiation, only 6 (4) remain at B > 0.5 T, caused by decoupling of the total electronic momentum J and the nuclear spin momentum I (hyperfine Paschen-Back regime). The expressions derived in the frame of completely uncoupl…
Complete nonlinear polarization control in an optical fiber system.
2010
International audience; We consider the counterpropagating interaction of a signal and a pump beam in an isotropic optical fiber. On the basis of recently developed mathematical techniques, we show that an arbitrary state of polarization of the signal beam can be converted into any other desired state of polarization. On the other hand, an unpolarized signal beam may be repolarized into two specific states of polarization, without loss of energy. Both processes of repolarization and polarization conversion may be controlled by adjusting the polarization state of the backward pump.
Sodium vapor cell laser guide star experiments for continuous wave model validation
2016
Recent numerical simulations and experiments on sodium Laser Guide Star (LGS) have shown that a continuous wave (CW) laser with circular polarization and re-pumping should maximize the fluorescent photon return flux to the wavefront sensor for adaptive optics applications. The orientation and strength of the geomagnetic field in the sodium layer also play an important role affecting the LGS return ux. Field measurements of the LGS return flux show agreement with the CW LGS model, however, fluctuations in the sodium column abundance and geomagnetic field intensity, as well as atmospheric turbulence, induce experimental uncertainties. We describe a laboratory experiment to measure the photon …
LES of the flow around two cylinders in tandem
2008
The flow around an arrangement of two-in-tandem cylinders exhibits a remarkably\ud complex behaviour that is of interest for many engineering problems, such as environmental\ud flows or structural design. In the present paper, a Large Eddy Simulation using a staggered\ud Cartesian grid has been performed for the flow around two-in-tandem cylinders of diameter\ud D=20mm and height H=50mm submerged in an open channel with height h=60 mm. The two\ud axes have a streamwise spacing of 2D. The Reynolds number is 1500, based on the cylinder\ud diameter and the free-stream velocity u�. The results obtained show that no vortex shedding\ud occurs in the gap between the two cylinders where the separat…
Spontaneous polarization induced by natural thermalization of incoherent light
2008
We analyze theoretically the polarization properties of a partially coherent optical field that propagates in a nonlinear Kerr medium. We consider the standard model of two resonantly coupled nonlinear Schrödinger equations, which account for a wave-vector mismatch between the orthogonal polarization components. We show that such a phase-mismatch is responsible for the existence of a spontaneous repolarization process of the partially incoherent optical field during its nonlinear propagation. The repolarization process is characterized by an irreversible evolution of the unpolarized beam towards a highly polarized state, without any loss of energy. This unexpected result contrasts with the …
Electronic States, Absorption Spectrum and Circular Dichroism Spectrum of the Photosynthetic Bacterial LH2 Antenna of Rhodopseudomonas acidophila as …
1999
A new approach that uses a combination of semiempirical configuration interaction method and exciton theory to calculate electronic energies, eigenstates, absorption spectrum and circular dichroism (CD) spectrum of the LH2 antenna of Rhodopseudomonas acidophila is introduced. A statistical simulation that uses experimental homogeneous line widths was used to account for the inhomogeneous line width of the observed spectrum. Including the effect of orbital overlap of the close-lying pigments of the B850 ring and the effect of the pigment protein interaction in the B800 ring allowed a successful simulation of the experimental absorption and CD spectra of the antenna at room temperature. Two e…