Search results for "coherent control"

Spatiotemporal rotational dynamics of laser-driven molecules

2020

Molecular alignment and orientation by laser fields has attracted significant attention in recent years, mostly due to new capabilities to manipulate the molecular spatial arrangement. Molecules can now be efficiently prepared for ionization, structural imaging, orbital tomography, and more, enabling, for example, shooting of dynamic molecular movies. Furthermore, molecular alignment and orientation processes give rise to fundamental quantum and classical phenomena like quantum revivals, Anderson localization, and rotational echoes, just to mention a few. We review recent progress on the visualization, coherent control, and applications of the rich dynamics of molecular rotational wave pack…

Control of the coupling strength and linewidth of a cavity magnon-polariton

2020

The full coherent control of hybridized systems such as strongly coupled cavity photon-magnon states is a crucial step to enable future information processing technologies. Thus, it is particularly interesting to engineer deliberate control mechanisms such as the full control of the coupling strength as a measure for coherent information exchange. In this work, we employ cavity resonator spectroscopy to demonstrate the complete control of the coupling strength of hybridized cavity photon-magnon states. For this, we use two driving microwave inputs which can be tuned at will. Here, only the first input couples directly to the cavity resonator photons, whilst the second tone exclusively acts …

Coherent control of stimulated emission inside one-dimensional photonic crystals

2004

In this paper, the quasinormal mode (QNM) theory is applied to discuss the quantum problem of an atom embedded inside a one-dimensional (1D) photonic band gap (PBG) cavity pumped by two counterpropagating laser beams. The e.m. field is quantized in terms of the QNMs in the 1D PBG and the atom modeled as a two-level system is assumed to be weakly coupled to just one of the QNMs. The main result of the paper is that the decay time depends on the position of the dipole inside the cavity, and can be controlled by the phase difference of the two laser beams.

Intensity Invariance of Strong-Field Two-Photon Absorption

2010

We demonstrate experimentally and theoretically the intensity-invariant scaling formula of coherent control of two-photon absorption as a function of pulse-shape parameters of ultrafast laser field in the strong-interaction regime.

Control of Quantum Dynamics by Laser Pulses: Adiabatic Floquet Theory

2003

Temporal phase control of bound-bound and bound-free two-photon transitions in NO with two time-delayed cross-polarized pulses

2001

0953-4075; Temporal phase control over the multi-photoionization of NO is investigated experimentally The coherent excitation of the molecular system is achieved by a sequence of two phase-related non-Fourier-transform-limited laser pulses delivered by a nanosecond dye laser, The phase-locked pulses are produced by making use of an actively stabilized interferometer with a tunable pathlength difference. As the coherence time of the laser is comparable with the inhomogenous dephasing time of the medium, the measurements are performed with temporally overlapped pulses. In order to avoid the modulation of the ionic signal coming from optical interference, the linear polarizations of the two pu…

Triply resonant coherent four-wave mixing in silicon nitride microresonators

2015

The generation of multiple tones using four-wave mixing (FWM) has been exploited for many applications, ranging from wavelength conversion to frequency comb generation. FWM is a coherent process, meaning that its dynamics strongly depends on the relative phase among the waves involved. The coherent nature of FWM has been exploited for phase-sensitive processing in different waveguide structures, but it has never been studied in integrated microresonators. Waveguides arranged in a resonant way allow for an effective increase in the wavelength conversion efficiency (at the expense of a reduction in the operational bandwidth). In this letter, we show that phase shaping of a three-wave pump pro…

Coherent control via weak measurements in P31 single-atom electron and nuclear spin qubits

2018

The understanding of weak measurements and interaction-free measurements has greatly expanded the conceptual and experimental toolbox to explore the quantum world. Here we demonstrate single-shot variable-strength weak measurements of the electron and nuclear spin states of a P31 single-atom donor in silicon. We first show how the partial collapse of the nuclear spin due to measurement can be used to coherently rotate the spin to a desired pure state. We explicitly demonstrate that phase coherence is preserved with high fidelity throughout multiple sequential single-shot weak measurements and that the partial state collapse can be reversed. Second, we use the relation between measurement st…

On-chip entangled D-level photon states – scalable generation and coherent processing

2018

Exploiting a micro-cavity-based quantum frequency comb, we demonstrate the on-chip generation of high-dimensional entangled quantum states with a Hilbert-space dimensionality larger than 100, and introduce a coherent control approach relying on standard telecommunications components.

Harmonic Generation and Nonlinear Propagation: When Secondary Radiations Have Primary Consequences

2014

In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultraintense pulse unexpectedly modify the nonlinear properties of the medium and lead to a strong modification of the propagation dynamics. This result is in contrast with all current state-of-the-art propagation model predictions, in which secondary radiations, such as third harmonic, are expected to have a negligible action upon the fundamental pulse propagation. By analyzing full three-dimensional ab initio quantum calculations describing the microscopic atomic optical response, we have identified a fundamental mechanism resulting from interfere…