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showing 10 items of 2224 documents

Ultra-broad spectral photo-response in FePS3 air-stable devices

2021

Van der Waals materials with narrow energy gaps and efficient response over a broadband optical spectral range are key to widen the energy window of nanoscale optoelectronic devices. Here, we characterize FePS as an appealing narrow-gap p-type semiconductor with an efficient broadband photo-response, a high refractive index, and a remarkable resilience against air and light exposure. To enable fast prototyping, we provide a straightforward guideline to determine the thickness of few-layered FePS nanosheets extracted from the optical transmission characteristics of several flakes. The analysis of the electrical photo-response of FePS devices as a function of the excitation energy confirms a …

Materials scienceFísica de la Materia CondensadaSpectral photo-response02 engineering and technology010402 general chemistrymedicine.disease_cause01 natural sciences7. Clean energysymbols.namesakeUltra-broadBroadbandmedicineGeneral Materials SciencePhotodetectors; FePS3; Ab-initio theory;Materials of engineering and construction. Mechanics of materialsQD1-999MaterialsFePS3PhotocurrentRange (particle radiation)business.industryMechanical EngineeringGeneral ChemistryAir-stable devices021001 nanoscience & nanotechnologyCondensed Matter Physics0104 chemical sciencesChemistrySemiconductorMechanics of MaterialsTA401-492symbolsOptoelectronicsvan der Waals forceElectrònica Aparells i instruments0210 nano-technologybusinessRefractive indexUltravioletExcitation
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High-pressure synthesis of CO and syngas from CO2 reduction using Ni-N-doped porous carbon electrocatalyst

2022

Abstract Electrochemical conversion of CO2 to CO or syngas (CO/H2 mixture) is considered one of the most promising approaches to valorise waste-CO2. To develop the process on industrial scale, it would be necessary to use selective and inexpensive electrodes and to obtain high productivities with low energy consumption. In this frame, Ni−NC catalysts are considered among the most interesting ones because of their relatively low cost, high faradaic efficiency in CO ( F E C O ), and high stability. However, up to now, quite low productivities were obtained as a result of low current densities achieved in aqueous electrolytes. In this work, we have evaluated the performances of a Ni−NC electro…

Materials scienceGeneral Chemical EngineeringDopingCO reductionGeneral ChemistrySettore ING-IND/27 - Chimica Industriale E TecnologicaElectrochemistryElectrocatalystSyngasIndustrial and Manufacturing EngineeringCatalysisCOHigh pressureChemical engineeringCO2 reductionElectrodeEnvironmental ChemistryNi−NC electrocatalystCurrent densityFaraday efficiencySyngas
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ZnO/ZnS heterostructures for hydrogen production by photoelectrochemical water splitting

2016

This work studies the photoelectrochemical behavior of novel ZnO/ZnS heterostructures obtained by means of anodization in water and glycerol/water/NH4F electrolytes with different Na2S additions under controlled hydrodynamic conditions. For this purpose different techniques such as Field Emission Scanning Electronic Microscopy (FE-SEM) with EDX, Raman spectroscopy and photoelectrochemical water splitting tests under standard AM 1.5 conditions have been carried out. The obtained results showed that the hydrodynamic conditions promoted an ordered nanotubular morphology which facilitates electron-hole separation and consequently, the photoelectrochemical activity for water splitting is enhance…

Materials scienceGeneral Chemical EngineeringInorganic chemistry02 engineering and technologyElectrolyte010402 general chemistry01 natural sciencesINGENIERIA QUIMICAsymbols.namesakeZINCRAMAN-SPECTROSCOPYANODIZATIONTIO2 NANOTUBESHydrogen productionAnodizingELECTROLYTESPHOTOCATALYTIC ACTIVITYHeterojunctionGeneral Chemistry021001 nanoscience & nanotechnologyHYDRODYNAMIC CONDITIONSEVOLUTION0104 chemical sciencesARRAYSElectroquímicaField electron emissionsymbolsWater splitting0210 nano-technologyRaman spectroscopySENSITIZED ZNODark current
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In situ investigation of sacrificial behaviour of hot dipped AlSi coating in sulphate and chloride solutions

2013

Abstract The electrochemical behaviour of the cut-edge of hot-dipped aluminium–silicon-based alloy coated steel is studied in immersed conditions in sulphate and in chloride media. Preliminary studies performed on steel-pure Al bi-electrode demonstrate that a significant galvanic current can develop at short times (t

Materials scienceGeneral Chemical EngineeringMetallurgyAlloyGeneral Chemistryengineering.materialElectrochemistryChlorideCorrosionCoatingengineeringGalvanic cellmedicineGeneral Materials ScienceCurrent (fluid)Anodic protectionmedicine.drugCorrosion Science
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Investigation of self-healing mechanism on galvanized steels cut edges by coupling SVET and numerical modeling

2008

Local cathodic inhibition has been observed on the cut-edge of galvanized steel immersed in 0.03 M NaCl solution using the scanning vibrating electrode technique. The current distribution results indicate that cathodic inhibition occurs in a limited spatial zone located between the cathodic sites on the steel and the anodic sites on the exposed zinc surface. The experimental current distributions are compared with the results of numerical simulations that show the specific diagnostic features for the detection of cathodic inhibition from scanning vibrating electrode technique (SVET) data so as to distinguish the zero current regions from experimental artifacts due to the lateral resolution …

Materials scienceGeneral Chemical EngineeringMetallurgyOxidechemistry.chemical_elementZincGalvanizationAnodeCathodic protectionchemistry.chemical_compoundsymbols.namesakechemistrySelf-healingElectrochemistrysymbolsCoupling (piping)Composite materialCurrent (fluid)Electrochimica Acta
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Mechanical properties and corrosion behaviour after scratch and tribological tests of electrodeposited Co-Mo/TiO2 nano-composite coatings

2019

International audience; The micro-mechanical (Young’s modulus and hardness) and tribological properties, as well as the scratch resistance of Co-Mo/TiO2 nano-composite coatings were investigated. The coating was found to be harder and stiffer than the substrate (pure cobalt). Low residual stresses were also derived from Stoney’s equation (type I stress). The corrosion behaviour after tribological and scratch tests was studied in Ringer’s solution. Dry sliding of the coating against an alumina ball at the load of 1 N or 2 N over the same distance had nearly no influence onthe anodic branch of the polarisation curves. By contrast, the current density in the cathodic branch (oxygen reduction r…

Materials scienceGeneral Physics and Astronomy02 engineering and technologyengineering.material010402 general chemistry01 natural sciencesCathodic protectionCorrosionCoatingResidual stressComposite materialcomputer.programming_language[PHYS.MECA]Physics [physics]/Mechanics [physics]Surfaces and InterfacesGeneral ChemistryTribology021001 nanoscience & nanotechnologyCondensed Matter Physics0104 chemical sciencesSurfaces Coatings and FilmsAnodeScratchengineering0210 nano-technologyCurrent densitycomputerApplied Surface Science
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Magnetic field effect on electrodeposition of cobalt dendrites

2012

International audience; We are studying the effect of a magnetic field on cobalt dendrites grown by electrodeposition in thin cell. Several electrochemical parameters like pH, current density, initial concentration, are known to affect the crystalline structure of electrodeposited cobalt. Here we analyze, for two values of the pH, the effect of a high magnetic field (6 T) on the growth direction of the dendrites with respect to the crystalline axis of the structure.

Materials scienceGeneral Physics and Astronomychemistry.chemical_elementCrystal structureMagnetic field effectequipment and suppliesElectrochemistry01 natural sciencesmagnetic field effecteye diseases010305 fluids & plasmasMagnetic fieldchemistryChemical engineering0103 physical scienceselectrodeposition[PHYS.COND.CM-MS]Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci]sense organsElectrical and Electronic Engineeringhuman activitiesCobaltCurrent density
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Aqueous synthesis of Z-scheme photocatalyst powders and thin-film photoanodes from earth abundant elements

2018

Riga Technical University supported the preparation of this manuscript from the Scientific Research Project Competition for Young Researchers No. ZP 2017/8

Materials scienceHematiteNanoparticle02 engineering and technology010402 general chemistry01 natural sciences7. Clean energy:NATURAL SCIENCES:Physics [Research Subject Categories]Chemical Engineering (miscellaneous)Thin filmWaste Management and DisposalPhotocurrentProcess Chemistry and TechnologyPhotocatalystHeterojunction021001 nanoscience & nanotechnologyPollution0104 chemical sciencesAmorphous solidChemical engineeringZ-schemePhotoelectrochemical propertiesPhotocatalysisWater splitting0210 nano-technologyPhotoanodeVisible spectrumJournal of Environmental Chemical Engineering
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AC impedance behavior of the Ti4Ni2Oy and Ti3.5Zr0.5Ni2Oy type metal hydride electrodes

1999

The hydrogen storage alloy electrodes of the type Ti4Ni2Oy (y=0, 0.3 and 0.6) and Ti3.5Zr0.5Ni2Oy (y=0.15 and 0.3) were investigated by impedance spectroscopy for potential application as negative electrode in alkaline secondary nickel-metal hydride (MH) batteries. The phase Ti4Ni2O0.30 was found to be electrochemically more stable during the cycling. The addition of copper or nickel powder as current collector improved the electrochemical behavior of the electrodes. It was possible in this way to decrease the charge transfer resistance. These additions have a negligible influence on the stability of electrode material during cycling.

Materials scienceHydrideGeneral Chemical EngineeringInorganic chemistryGeneral EngineeringGeneral Physics and Astronomychemistry.chemical_elementCurrent collectorElectrochemistryCopperDielectric spectroscopyNickelHydrogen storagechemistryElectrodeGeneral Materials Science
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Comparison of resistance to damage of unalloyed carbon steels under the influence of hydrogen

2018

One of the most commonly used construction material in industry is unalloyed steel S235 and S355. These types of steel are used for construction of ships, bridges, coastal construction, welded tanks, and in buildings. Due to the operating conditions, these types of steel may undergo hydrogen degradation in the process of manufacturing of welded structures or when operating the structures. This paper presents the results of study into resistance of selected types of non-alloy structural steels to hydrogen degradation. Tests were carried out to determine changes in mechanical properties in the static trials of stretching without hydrogen, and after saturation with hydrogen. Parallel fractogra…

Materials scienceHydrogenMetallurgychemistry.chemical_elementWeldingElectrochemistrylaw.inventionchemistrylcsh:TA1-2040lawDegradation (geology)Arsenic oxideElectric currentlcsh:Engineering (General). Civil engineering (General)Saturation (chemistry)CarbonMATEC Web of Conferences
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