Search results for "defect"

showing 10 items of 879 documents

Experimental evidence of E’_gamma centers generation from oxygen vacancies in a-SiO2

2007

Abstract We report on the thermal treatment effects in a γ-ray irradiated oxygen deficient amorphous silicon dioxide (a-SiO2) containing Al impurities. We observed that by thermal treatments the intensity of the 7.6 eV optical absorption band, associated to an oxygen deficient center, and the EPR signal amplitude of irradiation induced [AlO4]0 centers gradually decrease. During these thermal treatments, the E γ ′ centers concentration is found to increase in a correlated way to the decrease of the 7.6 eV absorption amplitude. These results are interpreted assuming an hole-transfer process from the [AlO4]0 centers to the diamagnetic oxygen vacancies, resulting in the generation of E γ ′ cent…

ChemistryAnalytical chemistryOptical spectroscopychemistry.chemical_elementSilicaThermal treatmentCondensed Matter PhysicsOxygenElectronic Optical and Magnetic Materialslaw.inventionAbsorptionlawAbsorption bandImpurityElectron spin resonanceMaterials ChemistryCeramics and CompositesDiamagnetismDefectsIrradiationAtomic physicsElectron paramagnetic resonanceAbsorption (electromagnetic radiation)
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First‐principles modelling of defects in advanced nuclear fuels

2007

In this paper we present and discuss the results of first first-principle modelling of point defects in nitride nuclear fuels. Calculations have been performed using the VASP computer code combined with supercells containing up to 250 atoms. The effective atomic charges, the electronic density redistribution, atomic displacements around U and N vacancies and their formation energies are discussed. (© 2007 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim)

ChemistryNanotechnologyRedistribution (chemistry)Atomic chargeNitrideCondensed Matter PhysicsMolecular physicsCrystallographic defectElectronic densityphysica status solidi c
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First-principles calculations of oxygen interstitials in corundum: a site symmetry approach

2017

The authors are indebted to R. Vila, A. Popov and A. Lushchik for stimulating discussions. This work was carried out within the framework of the EUROfusion Consortium and received funding from the European Union’s Horizon 2020 Research and Innovation Programme under grant agreement 633053. The views and opinions expressed herein do not necessarily reflect those of the European Commission. Support from Latvian National Research Program IMIS2 (2014–2017) is also appreciated. Calculations were carried out using both the Marconi supercomputer system at the Computational Simulation Centre and the Computer Center of St. Petersburg State University.

ChemistryOxideGeneral Physics and AstronomyCharge (physics)02 engineering and technology010402 general chemistry021001 nanoscience & nanotechnology7. Clean energy01 natural sciences0104 chemical sciencesHybrid functionalCondensed Matter::Materials Sciencechemistry.chemical_compoundTriplet oxygenInterstitial defectAtom:NATURAL SCIENCES:Physics [Research Subject Categories]DumbbellSinglet statePhysical and Theoretical ChemistryAtomic physics0210 nano-technologyPhysical Chemistry Chemical Physics
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<title>Spatial correlation of latent image centers active in photostimulable luminescence of irradiated doped alkali halides</title>

2001

Changes in the photostimulated luminescence (PSL) spectrum of an electron irradiated KBr:Tl single crystal in relation to the A-luminescence spectrum upon direct activator ion excitation in the A-absorption band (AL) are found. Based on the view about the spatial correlation between F and activator hole centers, it is suggested that anion vacancy is an additional perturbing factor fot he activator (Tl+) excited (p-electron) state which is already subject to the dynamical Jahn-Teller effect. Dependences of the PSL efficiency on activator (In+) concentration in KBr:In samples irradiated by UV-light (6.30-6.45 eV), X-rays (30 keV or electrons (5.6 keV), are compared. The possible role of 6.45 …

ChemistryPhotostimulated luminescenceExcitonVacancy defectExcited stateActivator (phosphor)Atomic physicsLuminescenceSingle crystalIonSPIE Proceedings
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Diffusion and reactions of interstitial oxygen species in amorphous SiO2: A review

2008

This article briefly summarizes the diffusion and reactions of interstitial oxygen species in amorphous SiO 2 (a-SiO 2 ). The most common form of interstitial oxygen species is oxygen molecule (O 2 ), which is sensitively detectable via its characteristic infrared photoluminescence (PL) at 1272 nm. The PL observation of interstitial 0 2 provides key data to verify various processes related to interstitial oxygen species: the dominant role of interstitial O 2 in long-range oxygen transport in a-SiO 2 ; formation of the Frenkel defect pair (Si-Si bond and interstitial oxygen atom, 0°) by dense electronic excitation; efficient photolysis of interstitial O 2 into O° with F 2 laser light (λ= 157…

ChemistryRadicalPhotodissociationDangling bondOxygen transportchemistry.chemical_elementCondensed Matter PhysicsPhotochemistryOxygenChemical reactionElectronic Optical and Magnetic MaterialsMaterials ChemistryCeramics and CompositesFrenkel defectMoleculeJournal of Non-Crystalline Solids
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Calculations of F centers in KNbO 3 ferroelectric crystals

1997

Semi-empirical method of the intermediate neglect of the differential overlap (INDO) combined with the supercell model is applied to the calculations of the F center optical properties in ferroelectric KNbO 3 perovskite crystals. It is shown that two electrons of the defect are weakly localized inside the O vacancy, unlike similar defects in ionic alkali halides, but are considerably spread over two nearest Nb atoms. For the orthorhombic phase stable at room temperatures three absorption bands are predicted to be at 2.72 eV, 3.04 eV and 3.11 eV, respectively. The first energy is close to the band at 2.7 eV observed in electron- irradiated crystals. In the high temperature, cubic phase only …

ChemistryVacancy defectPhase (matter)Supercell (crystal)Ionic bondingOrthorhombic crystal systemElectronAtomic physicsMolecular physicsFerroelectricityPerovskite (structure)SPIE Proceedings
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Possible relationship between micronucleated and binucleated cells induced by cisplatin in cultured CHO cells

1993

Abstract Chinese hamster ovary (CHO) cells were treated with a single dose (10 μg/ml) of cis-diammino-dichloroplatinum (II) (cisplatin) for 1 h and the effect of the drug on the kinetics of proliferation of the cultures was studied. It was found that the drug produces a delay in the proliferation rates of the treated cultures. The induction of micronuclei and binucleated cells (BC) at different times after treatment have also been studied, and the ability of these cells to undergo DNA synthesis (measured as the ability to incorporate [3H]thymidine) is shown. It was found that cisplatin induced a particular type of BC that contains one or more micronuclei rather than a pure population of BC.…

Cisplatineducation.field_of_studyDNA synthesisChinese hamster ovary cellBinucleated cellsPopulationHamsterCHO CellsBiologyToxicologycomplex mixturesMolecular biologychemistry.chemical_compoundchemistryCricetinaeMicronucleus testGeneticsmedicineAnimalsCisplatineducationThymidineCell DivisionMicronuclei Chromosome-Defectivemedicine.drugMutation Research/Environmental Mutagenesis and Related Subjects
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Magnetometry with Nitrogen-Vacancy Centers in Diamond

2016

This chapter covers magnetic sensing with nitrogen-vacancy (NV) defect centers in diamond. The NV center fundamentals are introduced and NV optically detected magnetic resonance techniques for dc and ac magnetic sensing are summarized. After reviewing some successful sensing applications, the advantages for using NV magnetometry, as well as some ongoing challenges, are enumerated.

Coherence timeMaterials scienceMagnetic noisebusiness.industrySensing applicationsMagnetometerDiamondchemistry.chemical_element02 engineering and technologyengineering.material021001 nanoscience & nanotechnology01 natural sciencesMagnetic sensingNitrogenlaw.inventionchemistrylawVacancy defect0103 physical sciencesengineeringOptoelectronics010306 general physics0210 nano-technologybusiness
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Energy loss and fluence dependency of swift‐ion‐induced hardening in LiF

2005

The depth profiles of the hardening effects of LiF irradiated with swift Au, Pb, Bi, Kr, Ni and S ions of MeV-GeV energy have been studied as a function of ion penetration depth. For all projectiles, the hardness increases scaling with the range of ions and depending on ion fluence and energy loss. Heavy ions (Au, Pb, Bi), for which the energy loss noticeably exceeds the threshold of about 10 keV/nm for severe track core damage, cause uniform increase of hardness in the entire irradiated layer. For irradiations with lighter S, Ni, Kr ions, the hardening displays strong depth dependence. Ion-induced hardening is related to pinning of dislocations by defect aggregates (possibly small Li collo…

ColloidMaterials scienceAstrophysics::High Energy Astrophysical PhenomenaIon trackVacancy defectHardening (metallurgy)IrradiationAtomic physicsPenetration depthFluenceIonphysica status solidi (c)
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Microscopic theory of colloid formation in solids under irradiation

1996

Results of the first-principles study of diffusion-controlled aggregation of Frenkel defects-interstitial atoms-under irradiation of solids are presented. Conditions of the efficient radiation-induced aggregation of vacancies and interstitials are studied and the scenario of this process is presented.

ColloidMaterials scienceCondensed matter physicsMechanics of MaterialsChemical physicsMechanical EngineeringDiffusionFrenkel defectGeneral Materials ScienceIrradiationMicroscopic theoryCondensed Matter PhysicsMaterials Science and Engineering: B
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