Search results for "electrons"
showing 10 items of 1325 documents
Characterization of a sucrose/starch matrix through positron annihilation lifetime spectroscopy: unravelling the decomposition and glass transition p…
2010
The triplet state of positronium, o-Ps, is used as a probe to characterize a starch-20% w/w sucrose matrix as a function of temperature (T). A two-step decomposition (of sucrose, and then starch) starts at 440 K as shown by a decrease in the o-Ps intensity (I(3)) and lifetime (τ(3)), the latter also disclosing the occurrence of a glass transition. Upon sucrose decomposition, the matrix acquires properties (reduced size and density of nanoholes) that are different from those of pure starch. A model is successfully established, describing the variations of both I(3) and τ(3) with T and yields a glass transition temperature, T(g) = (446 ± 2) K, in spite of the concomitant sucrose decomposition…
Band-selective third-harmonic generation in superconducting MgB$_2$: Possible evidence for Higgs amplitude mode in the dirty limit
2020
We report on time-resolved linear and nonlinear terahertz spectroscopy of the two-band superconductor MgB$_2$ with the superconducting transition temperature $T_c \approx 36$ K. Third-harmonic generation (THG) is observed below $T_c$ by driving the system with intense narrowband THz pulses. For the pump-pulse frequencies $f=$ 0.3, 0.4, and 0.5 THz, temperature-dependent evolution of the THG signals exhibits a resonance maximum at the temperatures with the resonance conditions $2f=2\Delta_\pi(T)$ fulfilled, for the dirty-limit superconducting gap $2\Delta_\pi$. In contrast, for $f=$ 0.6 and 0.7 THz with $2f>2\Delta_\pi(T\rightarrow0)=1.03$ THz, the THG intensity increases monotonically with …
A Ni-based Superconductor: the Heusler Compound ZrNi$_2$Ga
2008
This work reports on the novel Heusler superconductor ZrNi2Ga. Compared to other nickel-based superconductors with Heusler structure, ZrNi2Ga exhibits a relatively high superconducting transition temperature of Tc=2.9 K and an upper critical field of 1.5 T. Electronic structure calculations show that this relatively high transition temperature is caused by a van Hove singularity, which leads to an enhanced density of states at the Fermi energy. The van Hove singularity originates from a higher order valence instability at the L-point in the electronic structure. The enhanced density of states at the Fermi level was confirmed by specific heat and susceptibility measurements. Although many He…
Superconductivity provides a giant enhancement to the spin battery effect
2021
We develop a theory of the spin battery effect in superconductor/ferromagnetic insulator (SC/FI) systems taking into account the magnetic proximity effect. We demonstrate that the spin-energy mixing enabled by the superconductivity leads to the enhancement of spin accumulation by several orders of magnitude relative to the normal state. This finding can explain the recently observed giant inverse spin Hall effect generated by thermal magnons in the SC/FI system. We suggest a non-local electrical detection scheme which can directly probe the spin accumulation driven by the magnetization dynamics. We predict a giant Seebeck effect converting the magnon temperature bias into the non-local volt…
Chiral pair density wave states generated by spin supercurrents
2021
We report that spin supercurrents in magnetic superconductors and superconductor/ferromagnetic insulator bilayers can induce the Dzyaloshinskii-Moriya interaction which strength is proportional to the superconducting order parameter amplitude. This effect leads to the existence of inhomogeneous parity-breaking ground states combining the chiral magnetic helix and the pair density wave orders. The formation of such states takes place via the penetration of chiral domain walls at the threshold temperature below the superconducting transition. We find regimes with both the single and the re-entrant transitions into the inhomogeneous states with decreasing temperature. The predicted hybrid chir…
Enhanced Superconductivity and Suppression of Charge-density Wave Order in 2H-TaS$_2$ in the Two-dimensional Limit
2017
As superconductors are thinned down to the 2D limit, their critical temperature $T_c$ typically decreases. Here we report the opposite behavior, a substantial enhancement of $T_c$ with decreasing thickness, in 2D crystalline superconductor 2H-TaS$_2$. Remarkably, in the monolayer limit, $T_c$ increases to 3.4 K compared to 0.8 K in the bulk. Accompanying this trend in superconductivity, we observe suppression of the charge-density wave (CDW) transition with decreasing thickness. To explain these trends, we perform electronic structure calculations showing that a reduction of the CDW amplitude results in a substantial increase of the density of states at the Fermi energy, which contributes t…
Low-Frequency Imaginary Impedance at the Superconducting Transition of 2H-NbSe2
2019
The superconducting transition leads to a sharp resistance drop in a temperature interval that can be a small fraction of the critical temperature T$_c$. A superconductor exactly at T$_c$ is thus very sensitive to all kinds of thermal perturbations, including the heat dissipated by the measurement current. We show that the interaction between electrical and thermal currents leads to a sizeable imaginary impedance at frequencies of order of tens of Hz at the resistive transition of single crystals of the layered material 2H-NbSe$_2$. We explain the result using models developed for transition edge sensors. By measuring under magnetic fields and at high currents, we find that the imaginary im…
Giant negative magnetoresistance driven by spin-orbit coupling at the LAO/STO interface
2014
The LAO/STO interface hosts a two-dimensional electron system that is unusually sensitive to the application of an in-plane magnetic field. Low-temperature experiments have revealed a giant negative magnetoresistance (dropping by 70\%), attributed to a magnetic-field induced transition between interacting phases of conduction electrons with Kondo-screened magnetic impurities. Here we report on experiments over a broad temperature range, showing the persistence of the magnetoresistance up to the 20~K range --- indicative of a single-particle mechanism. Motivated by a striking correspondence between the temperature and carrier density dependence of our magnetoresistance measurements we propos…
Tuning interchain ferromagnetic instability in A2Cr3As3 ternary arsenides by chemical pressure and uniaxial strain
2020
We analyze the effects of chemical pressure induced by alkali metal substitution and uniaxial strain on magnetism in the A2Cr3As3 (A = Na, K, Rb, Cs) family of ternary arsenides with quasi-one dimensional structure. Within the framework of the density functional theory, we predict that the non-magnetic phase is very close to a 3D collinear ferrimagnetic state, which realizes in the regime of moderate correlations, such tendency being common to all the members of the family with very small variations due to the different interchain ferromagnetic coupling. We uncover that the stability of such interchain ferromagnetic coupling has a non-monotonic behavior with increasing the cation size, bein…
Dynamics of Collective Modes in an unconventional Charge Density Wave system BaNi$_{2}$As$_{2}$
2021
AbstractBaNi2As2 is a non-magnetic analogue of BaFe2As2, the parent compound of a prototype pnictide high-temperature superconductor, displaying superconductivity already at ambient pressure. Recent diffraction studies demonstrated the existence of two types of periodic lattice distortions above and below the triclinic phase transition, suggesting the existence of an unconventional charge-density-wave (CDW) order. The suppression of CDW order upon doping results in a sixfold increase in the superconducting transition temperature and enhanced nematic fluctuations, suggesting CDW is competing with superconductivity. Here, we apply time-resolved optical spectroscopy to investigate collective d…