Search results for "fission products"
showing 10 items of 63 documents
Fission studies at IGISOL/JYFLTRAP: Simulations of the ion guide for neutron-induced fission and comparison with experimental data
2020
For the production of exotic nuclei at the IGISOL facility, an ion guide for neutron-induced fission has been developed and tested in experiments. Fission fragments are produced inside the ion guide and collected using a helium buffer gas. Meanwhile, a GEANT4 model has been developed to simulate the transportation and stopping of the charged fission products. In a recent measurement of neutron-induced fission yields, implantation foils were located at different positions in the ion guide. The gamma spectra from these foils and the fission targets are compared to the results from the GEANT4 simulation. In order to allow fission yield measurements in the low yield regions, towards the tails a…
Odd-Even Effects in the Reaction 241Am(2n,f)
1992
Fission yields of the light fission products in the reaction 241Am(2n,f) have been measured. The results indicate an odd-even proton effect in the yield distribution of this odd nucleus with Z=95.
Rapid chemical separation procedures
1976
Fast, discontinuous separation procedures are described for zirconium, niobium, technetium and antimony from fission products. Other rapid separation methods from aqueous solutions are summarized. The combination of a gas jet recoil transport system with a continuous solvent extraction technique and with a thermochromatographic separation method is presented. The application of such procedures to the investigation of new and already known short-lived nuclides is illustrated by some examples.
New antineutrino energy spectra predictions from the summation of beta decay branches of the fission products
2012
In this paper, we study the impact of the inclusion of the recently measured beta decay properties of the $^{102;104;105;106;107}$Tc, $^{105}$Mo, and $^{101}$Nb nuclei in an updated calculation of the antineutrino energy spectra of the four fissible isotopes $^{235, 238}$U, and $^{239,241}$Pu. These actinides are the main contributors to the fission processes in Pressurized Water Reactors. The beta feeding probabilities of the above-mentioned Tc, Mo and Nb isotopes have been found to play a major role in the $\gamma$ component of the decay heat of $^{239}$Pu, solving a large part of the $\gamma$ discrepancy in the 4 to 3000\,s range. They have been measured using the Total Absorption Techni…
Rapid continous radiochemical separations by thermochromatography in connection with a gas-jet recoil-transport system
1980
Abstract A combination of a gas-jet recoil-transport system with a thermochromatographic system has been studied as a technique for rapid, continuous radiochemical separations. Fission products were used as a model for complex mixtures of elements. A nitrogen gas-jet containing potassium chloride clusters was applied to transport nuclides produced in a reactor from the target area to the thermochromatographic column. Conversion of the reaction products carried by the gas-jet volatile species was achieved by stopping the clusters in a quartz-wool plug located in the column and kept at high temperatures and feeding a reactive gas into the column. Several reactive gases producing volatile chlo…
Chemical reactions in a gas-jet recoil-transport system: Continuous separation procedure for selenium and tellurium from fission products
1978
Abstract Chemical selectivity in a gas-jet recoil-transport system can be achieved by chemical reactions with the carrier gas. This is demonstrated for an ethylene-nitrogen jet in which volatile species of selenium and tellurium are formed by passing the gas through a reaction zone heated to 860°C. Rapid continuous separation procedures for selenium and tellurium from fission products based on this effect are described and some decay data of the neutron-rich nuclides 85–88Se and 135–137Te obtained with these methods are given.
Transport of recoil atoms in a stream of liquid-air-cooled pure helium
1974
Abstract Pure commercial helium cooled down to the temperature of liquid air (80 K) has been used for rapid transportation of recoil atoms over distances as long as 10 m. Transport efficiencies of several tens of per cent have been obtained for recoil atoms resulting from alpha decay or from decay by fission. The angle of divergence of the beam of recoil atoms at the exit of the transport capillary is measured to be (11±2)° for particles of mass number A = 211. Experimental results are discussed in terms of thermal diffusion. The elimination of carrier vapors will probably simplify the use of the helium-jet technique in on-line mass separators.
New accurate measurements of neutron emission probabilities for relevant fission products
2017
We have performed new accurate measurements of the beta-delayed neutron emission probability for ten isotopes of the elements Y, Sb, Te and I. These are fission products that either have a significant contribution to the fraction of delayed neutrons in reactors or are relatively close to the path of the astrophysical r process. The measurements were performed with isotopically pure radioactive beams using a constant and high efficiency neutron counter and a low noise beta detector. Preliminary results are presented for six of the isotopes and compared with previous measurements and theoretical calculations. peerReviewed
Implementation of an aerodynamic lens for TRIGA-SPEC
2016
Abstract We report on the optimization of the gas-jet system employed to couple the TRIGA-SPEC experiment to the research reactor TRIGA Mainz. CdI2 aerosol particles suspended in N2 as carrier gas are used for an effective transport of fission products from neutron induced 235 U fission from the target chamber to a surface ion source. Operating conditions of the gas-jet were modified to enable the implementation of an aerodynamic lens, fitting into the limited space available in front of the ion source. The lens boosts the gas-jet efficiency by a factor of 4–10. The characterization of the gas-jet system as well as the design of the aerodynamic lens and efficiency studies are presented and …
In-beam spectroscopy using the JYFL gas-filled magnetic recoil separator RITU
2003
The techniques of recoil-gating and recoil-decay tagging have been employed at Jyvaskyla to perform in-beam γ-ray and electron spectroscopy studies of heavy nuclei. The JUROSPHERE γ-ray array and the SACRED electron spectrometer have been placed at the target position of the JYFL gas-filled recoil separator recoil ion transport unit (RITU). The RITU separator has been used to collect the recoils of interest and separate them from beam particles and fission products. At the focal plane a detector system consisting of time-of-flight and implantation detectors has been used for further event identification. The method and some highlights from the results in the lead region close to the proton …