Search results for "fission products"
showing 10 items of 63 documents
Separation of fission products by the ion guide fed isotope separator, IGISOL
1987
Abstract The performance of the ion guide method in the on-line mass separation of fission products has been investigated. Activity was produced by bombarding nat. U targets with a beam of 20 MeV protons. All the mass chains from A = 95 through A = 120 have been scanned using conventional methods of nuclear spectroscopy. No chemical selectivity in the separation was observed; isotopes of highly nonvolatile elements from yttrium to palladium were produced with efficiencies equal to those for the more volatile ones. The boundary of known neutron-rich nuclides was reached throughout the mass region from A = 106 to A = 118. During the course of this preliminary study the new isotope 116 Rh was …
High-accuracy mass spectrometry of fission products with Penning traps
2012
Mass measurements of fission products based on Penning-trap technique are reviewed in this article. More than 300 fission products have been measured with JYFLTRAP, ISOLTRAP, CPT, LEBIT and TITAN Penning traps with a typical precision of δm/m ≈ 10−7 − 10−8. In general, the results agree well with each other. The new data provide a valuable source of information and a challenge for the future development of theoretical mass models as well as for obtaining a deeper insight into microscopic properties of atomic nuclei as measured, for example, via key mass differentials. Shape transitions around N = 60, subshell closure at N = 40 and shell closures at N = 50 and N = 82 have been investigated i…
Benchmark of a multi-physics Monte Carlo simulation of an ionguide for neutron-induced fission products
2022
AbstractTo enhance the production of medium-heavy, neutron-rich nuclei, and to facilitate measurements of independent yields of neutron-induced fission, a proton-to-neutron converter and a dedicated ion guide for neutron-induced fission have been developed for the IGISOL facility at the University of Jyväskylä. The ion guide holds the fissionable targets, and the fission products emerging from the targets are collected in helium gas and transported to the downstream experimental stations. A computer model, based on a combination of MCNPX for modeling the neutron production, the fission code GEF, and GEANT4 for the transport of the fission products, was developed. The model will be used to i…
Summation Calculations for Reactor Antineutrino Spectra, Decay Heat and Delayed Neutron Fractions Involving New TAGS Data and Evaluated Databases
2018
9 pags., 3 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Applications of the total absorption technique to improve reactor decay heat calculations: study of the beta decay of [sup 102,104,105]Tc
2009
The decay heat of the fission products plays an important role in predicting the heat‐up of nuclear fuel after reactor shutdown. This form of energy release is calculated as the sum of the energy‐weighted activities of all fission products P(t) = ΣEiλiNi(t), where Ei is the decay energy of nuclide i (gamma and beta component), λi is the decay constant of nuclide i and Ni(t) is the number of nuclide i at cooling time t. Even though the reproduction of the measured decay heat has improved in recent years, there is still a long standing discrepancy at t∼1000 s cooling time for some fuels. A possible explanation for this disagreement can been found in the work of Yoshida et al. [1], who demonst…
β-decay data requirements for reactor decay heat calculations: study of the possible source of the gamma-ray discrepancy in reactor heat summation ca…
2007
The decay heat of fission products plays an important role in predictions of the heat up of nuclear fuel in reactors. The released energy is calculated as the summation of the activities of allfission products P(t) = Ei λi Ni(t), where Ei is the decay energy of nuclide i (gamma and beta component), λi is the decay constant of nuclide i and Ni(t) is the number of nuclide i at cooling time t. Even though the reproduction of the measured decay heat has improved in recent years, there is still a long standing discrepancy in the t ∼ 1000s cooling time for some fuels. A possible explanation to this improper description has been found in the work of Yoshida et al. (1), where it has been shown that…
Improvements on Decay Heat Summation Calculations by Means of Total Absorption Gamma-ray Spectroscopy Measurements
2011
The decay heat of fission products plays an important role in predictions of the heat released by nuclear fuel in reactors. In this contribution we present results of the analysis of the measurement of the beta decay of some refractory isotopes that were considered possible important contributors to the decay heat in reactors. The measurements presented here were performed at the IGISOL facility of the University of Jyvaeskylae, Finland. In our measurements we have combined for the first time a Penning trap (JYFLTRAP), which was used as a high resolution isobaric separator, with a total absorption spectrometer. The results of the measurements as well as their consequences for decay heat sum…
Independent yields of neutron-rich nuclei in charged-particle induced fission
1997
Abstract Yields of fission products have been studied at the recently upgraded IGISOL facility in Jyvaskyla using 50 MeV H2+ beam (Ep = 25 MeV) and thin natTh and natU targets. The independent yields of fission products in the mass regions A = 99−112 (elements Y, Nb and Tc) and A = 127−134 (elements Sn, Sb and Te) have been obtained. Comparisons of the experimental isotopic distributions with theoretical ones are presented. Enhancement of the production rate of the doubly magic 132Sn is observed in the experimental yield curve.
Fission product yields at intermediate energy
1998
The results of experimental and theoretical studies of fission product yields in proton-induced fission of 238U are presented. The yields of neutron-rich Ni, Cu, Zn, Ga and Ge—isotopes were measured by 25 MeV protons and the ion guide-based isotope separator technique. The pre-neutron emission fragment mass distributions were measured by protons at energies Ep=20, 35, 50 and 60 MeV using time-of-flight method. The results indicate enhancement for superasymmetric mass division at intermediate excitation energy of the fissioning nucleus. A model calculation of fission products yields for fission of 238U by protons and neutrons is presented which predicts the formation cross sections for neutr…
Levels in104Ru populated by the ??-decay of104Tc
1978
Theβ− — andγ-activities of 18.4 min104Tc have been studied with singles and coincidence measurements. Sources were prepared by chemical separation of technetium from the fission products of thermal-neutron-induced fission of235U. A revised level scheme of104Ru up to an excitation energy of 4.26 MeV is proposed. Fromβ-γ coincidence measurements, aQβ-value of 5.62±0.07 MeV has been obtained.