Search results for "fission products"
showing 10 items of 63 documents
Total absorption γ -ray spectroscopy of the β -delayed neutron emitters Br87 , Br88 , and Rb94
2017
We investigate the decay of 87,88Br and 94Rb using total absorption γ -ray spectroscopy. These important fission products are β-delayed neutron emitters. Our data show considerable βγ intensity, so far unobserved in high-resolution γ -ray spectroscopy, from states at high excitation energy. We also find significant differences with the β intensity that can be deduced from existing measurements of the β spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the r…
New Neutron-Rich Nuclei and Isomers Produced in Symmetric Fisson
1990
The novel method for rapid on-line mass separation, the IGISOL, is described. The method has been shown applicable to mass separation of short-lived proton-induced fission products without any chemical dependence on radionuclide. Recent results on isomeric states with half-lives of the order of milliseconds produced directly in proton-induced fission of 238U and separated with the IGISOL are presented. The future plans for connection of the new K-130 cyclotron of the University of Jyvaskyla with the IGISOL are reviewed.
Total absorption spectroscopy study of the β decay of Br86 and Rb91
2017
The beta decays of 86Br and 91Rb have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the IGISOL facility in Jyvaskyla and further purified using the JYFLTRAP. 86Br and 91Rb are considered high priority contributors to the decay heat in reactors. In addition 91Rb was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decay was well known from high-resolution measurements. Our results shows that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized.
TAGS measurements of $^{100}$Nb ground and isomeric states and $^{140}$Cs for neutrino physics with the new DTAS detector
2016
V. Guadilla et al. -- 4 pags., 6 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Measurement of fission products β decay properties using a total absorption spectrometer
2013
In a nuclear reactor, the decay of fission fragments is at the origin of decay heat and antineutrino flux. These quantities are not well known while they are very important for reactor safety and for our understanding of neutrino physics. One reason for the discrepancies observed in the estimation of the decay heat and antineutrinos flux coming from reactors could be linked with the Pandemonium effect. New measurements have been performed at the JYFL facility of Jyvaskyla with a Total Absorption Spectrometer (TAS) in order to circumvent this effect. An overview of the TAS technique and first results from the 2009 measurement campaign will be presented. © Owned by the authors, published by E…
Mass and charge distributions in the very asymmetric mass region of the neutron induced fission of
2001
Abstract The mass-separator Lohengrin was used to measure the yields of the light fission products with A=74−85 and their nuclear charge and kinetic energy distributions from the odd- Z compound nucleus 239 Np ∗ formed by double capture of thermal neutrons. The mass yield distribution reveals an influence of the fragment shell with N=50 affecting also the nuclear charge and kinetic energy distributions. An odd–even effect for protons is found in the very asymmetric mass division, increasing from 4% to 35% with increasing fission asymmetry. This is in contrast to findings in normal asymmetric fission (region of high fission yields) where no odd–even effect for protons was observed. An odd–ev…
Neutron and fragment yields in proton-induced fission of 238U at intermediate energies
2001
The primary fission fragment mass and kinetic energy distributions, and neutron multiplicities as function of fragment mass have been measured in the proton-induced fission of 238 U at energies Ep ¼ 20, 35, 50 and 60 MeV using time-of-flight technique. Pre-scission and post-scission neutron multiplicities have been extracted from double differential distributions. The fragment mass dependence of the post-scission neutron multiplicities reveals the gross nuclear shell structure effect even at the higher proton energies we measured. The yields ofneutron-rich fission products in the fission of 238 U by 25 MeV protons were measured using an ion guide-based isotope separator technique. The resul…
Level lifetimes in neutron-rich Ru isotopes
1995
The neutron-rich Ru isotopes are situated between the strongly deformed Sr-Zr region with axial deformation of f l _ 0.40 [1] and the spherical Cd-Sn region. Evidence for triaxiality of even-even Ru isotopes has been presented in [2-5], and lifetimes of some of their 2 + states have been measured in fission studies [6-9]. It seems, however, that in these experiments the nearly identical energies of the 2 + ---* 0 + transitions in l~ and 11~ could not be separated. Therefore, high-resolution measurements are required in order to perceive the evolution of deformation with increasing neutron number. So far only few measurements by the delayed-coincidence method [10] have been performed on chem…
New results with stored exotic nuclei at relativistic energies
2004
Recently, much progress has been made with stored exotic nuclei at relativistic velocities ( v c = 0.7 ) . Fragments of 208Pb and 209Bi projectiles and fission products from 238U ions were produced, separated in flight with the fragment separator FRS, and injected into the storage-cooler ring ESR for precision measurements. 114 new masses of neutron-deficient isotopes in the lead region have been measured with time-resolved Schottky Mass Spectrometry (SMS). A new isospin dependence of the pairing energy was observed due to the improved mass accuracy of typically 1.5×10-7 (30 keV). New masses of short-lived neutron-rich fission fragments have been obtained with Isochronous Mass Spectrometry …
Systematics of neutron emission probabilities from delayed neutron precursors
1973
A simple correlation based on the gross theory ofβ-decay is derived between the neutron emission probabilitiesPn of delayed neutron precursors, theirβ-decay energies and the neutron binding energies of the daughter nuclei. The correlation is shown to be valid for delayed neutron precursors among the fission products. ThePn-values of several expected but still unidentified neutron precursors are estimated together with their contributions to the delayed neutron groups in thermal-neutron induced fission of235U. Some aspects of theβ-strength function for transitions into highly excited states are discussed.