Search results for "goals"
showing 10 items of 643 documents
Size-And Wavelength-Dependent Two-Photon Absorption Cross-Section of CsPbBr3 Perovskite Quantum Dots
2017
All-inorganic colloidal perovskite quantum dots (QDs) based on cesium, lead, and halide have recently emerged as promising light emitting materials. CsPbBr3 QDs have also been demonstrated as stable two-photon-pumped lasing medium. However, the reported two photon absorption (TPA) cross sections for these QDs differ by an order of magnitude. Here we present an in-depth study of the TPA properties of CsPbBr3 QDs with mean size ranging from 4.6 to 11.4 nm. By using femtosecond transient absorption (TA) spectroscopy we found that TPA cross section is proportional to the linear one photon absorption. The TPA cross section follows a power law dependence on QDs size with exponent 3.3 +- 0.2. The …
Red Spectral Forms of Chlorophylls in Green Plant PSI - A Site-Selective and High-Pressure Spectroscopy Study
2003
One of the special spectroscopic characteristics of photosystem I (PSI) complexes is that they possess absorption and emission bands at lower energy than those of the reaction center. In this paper, the red pigment pools of PSI-200, PSI-core, and LHCI complex from Arabidopsis thaliana have been characterized at low temperatures by means of spectrally selective (hole-burning and fluorescence line-narrowing) and high-pressure spectroscopic techniques. It was shown that the green plant PSI-200 complex has at least three red pigment pools, from which two are located in the PSI-core and one, in the peripheral light-harvesting complex I (LHCI). All of the red pigment pools are characterized by st…
Frequency Range Selection Method for Vibrational Spectra
2018
Theoretical calculations of vibrational properties are widely used to explain and predict experimental spectra. However, with standard quantum chemical methods all molecular motions are considered, which is rather time-consuming for large molecules. Because typically only a specific spectral region is of experimental interest, we propose here an efficient method that allows calculation of only a selected frequency interval. After a computationally cheap low-level estimate of the molecular motions, the computational time is proportional to the number of normal modes needed to describe this frequency range. Results for a medium-sized molecule show a reduction in computational time of up to 1 …
Test of a separable approximation to a local soft-core potential in the three-body system
1975
Three-nucleon observables below the break-up threshold are calculated employing the pole approximation to the soft-core Malfliet-Tjon potentials. The results are compared in detail to those obtained with the local potentials and to those calculated with the usual Yamaguchi interactions.
Taming conformational heterogeneity in and with vibrational circular dichroism spectroscopy
2019
Chemical science 10, 7680 -7689 (2019). doi:10.1039/C9SC02866H
Search for the decay B0→a1±ρ∓
2006
We present a search for the rare B-meson decay B-0 -> a(1)(+/-)rho(-/+) with a(1)(+/-)->pi(+)pi(-)pi(+/-). We use (110 +/- 1.2)x10(6) Upsilon(4S)-> B (B) over bar decays collected with the BABAR detector at the PEP-II asymmetric-energy B Factory at SLAC. We obtain an upper limit of 30x10(-6) (90%C.L.) for the branching fraction product B(B-0 -> a(1)(+/-)rho(-/+))B(a(1)(+/-)->pi(+)pi(-)pi(+/-)), where we assume that the a(1)(+/-) decays exclusively to rho(0)pi(+/-).
Precision measurement of the Λ+c baryon mass
2005
The $\Lambda_c^+$ baryon mass is measured using $\Lambda_c^+\to\Lambda K^0_S K^+$ and $\Lambda_c^+\to\Sigma^0 K^0_S K^+$ decays reconstructed in 232 fb$^{-1}$ of data collected with the BaBar detector at the PEP-II asymmetric-energy $e^+e^-$ storage ring. The $\Lambda_c^+$ mass is measured to be $2286.46\pm0.14\mathrm{MeV}/c^2$. The dominant systematic uncertainties arise from the amount of material in the tracking volume and from the magnetic field strength.
Tri/Bi-maximal lepton mixing and leptogenesis
2009
In models with flavour symmetries added to the gauge group of the Standard Model the CP-violating asymmetry necessary for leptogenesis may be related with low-energy parameters. A particular case of interest is when the flavour symmetry produces exact Tri-Bimaximal lepton mixing leading to a vanishing CP-violating asymmetry. In this paper we present a model-independent discussion that confirms this always occurs for unflavoured leptogenesis in type I see-saw scenarios, noting however that Tri-Bimaximal mixing does not imply a vanishing asymmetry in general scenarios where there is interplay between type I and other see-saws. We also consider a specific model where the exact Tri-Bimaximal mi…
Dispersion relation formalism for virtual Compton scattering of the proton
2001
We present in detail a dispersion relation formalism for virtual Compton scattering (VCS) off the proton from threshold into the $\Delta(1232)$-resonance region. Such a formalism can be used as a tool to extract the generalized polarizabilities of the proton from both unpolarized and polarized VCS observables over a larger energy range. We present calculations for existing and forthcoming VCS experiments and demonstrate that the VCS observables in the energy region between pion production threshold and the $\Delta(1232)$-resonance show an enhanced sensitivity to the generalized polarizabilities.
Phenomenological consequences of the seesaw mechanism in S-4 based models
2009
Reference [1] proposed a flavor model based on the symmetry group S-4, managing to describe fermion masses and mixings. The Weinberg operator has been used in order to provide the smallness of the neutrino masses, while a set of scalar fields, getting nonvanishing vacuum expectation values, spontaneously breaks down S-4 and provides the tri-bimaximal pattern as the lepton mixing matrix. Restricting to this setting, in this paper we analyze possible origins for the effective terms: the type I seesaw mechanism is the best known approach, but type II and III are also discussed. The phenomenology related to these models is various and future experiments could in principle discriminate among the…