Search results for "harmonic generation"
showing 10 items of 217 documents
Control of the high harmonic generation spectra by changing the molecule-laser field relative orientation
2010
The time dependent Schrodinger equation of a homonuclear diatomic molecule in the presence of a linearly polarized laser field is numerically solved by means of a split-operator parallel code. The calculations are carried out by assuming a single active electron model with fixed nuclei; a simplified two-dimensional model of the system is used. The highly nonlinear response of the electron wave function to the laser electric field stimulates the molecule to emit electromagnetic radiation consisting of a wide plateau of odd harmonics of the laser field. It is shown that the emitted spectrum can be finely controlled by changing the angle between the laser electric field and the molecular axis;…
Pulse-duration dependence of the isotopic effect in simple molecular ions driven by strong laser fields
2011
In this paper we discuss isotopic effects in simple molecular ions subjected to strong laser fields. We show that the intensity of the emitted spectra strongly depends upon both the nuclear mass of the molecular ions and the laser pulse duration. In particular, for short pulse duration [up to 8 optical cycles (o.c.)], we confirm the trend described in the most studied case in which the high-order harmonic generation is more efficient for heavier isotopes; in contrast, an interesting physical phenomenon is predicted for pulses longer than 16 o.c. characterized by an inverse effect in which lighter molecular species are responsible for higher-order harmonic emission.
Ferroelectric liquid crystalline polysiloxanes designed for high second-order nonlinear susceptibilities
1994
Ferroelectric liquid crystalline (FLC) copolysiloxanes containing suitable comonomers («NLO-chromophores») for second harmonic generation (SHG) have been prepared. Their important feature is a donor-acceptor x-system sited perpendicular to the long axis of the side-group moieties in order to adopt the polar ordering of the ferroelectric LC phase. The influcences of the mesogen structure and of the content of NLO-chromophores on the liquid crystalline and ferroelectric properties are studied. The desired chiral smectic C * phase is retained up to 30 mol-% of chromophore. Also, first measurements of second harmonic generation have been performed
Dynamic clock generator and memory mass device using a quantum ring driven by three-color laser fields
2021
We study the behaviour and applications of a quantum ring (QR) under a three-color laser field. In particular we study the emission of harmonics and their temporal evolution through wavelets. These results suggest the use of QR for three important applications: (1) generation of single short pulses, (2) creation of a variable clock generator, (3) a memory mass device through the angular momentum acquired by the electron.
Quantum Control in Atomic Systems
1999
We review a series of recent experiments demonstrating quantum control of atomic processes and products induced by the interaction of the atom with coherent bichromatic electromagnetic fields. Since the effects under consideration are electromagnetically induced, control is established through the field parameters i.e. frequency, amplitude and phase. The controlled processes include resonant and non resonant multiphoton ionization, autoionization, radiative decay in multiple continua (ionization branching ratios) and third harmonic generation.
Parametric self-trapping in the presence of randomized quasi phase matching
2010
We report on experimental evidence of parametric spatial solitons in a quadratic crystal with randomized periodic ferroelectric poling. Two-color self-focusing via quadratic cascading overcomes the diffractive nature of both fundamental and frequency-doubled beams.
Ultraviolet quasi-phase-matched second harmonic generation in surface periodically poled lithium niobate optical waveguides
2007
The compatibility of low concentration (alpha-phase) proton exchange channel waveguides with electric field surface periodic poling of congruent lithium niobate (SPPLN) crystals has been experimentally demonstrated. With such waveguides, we obtained ultraviolet second harmonic generation (SHG) by first order quasi-phase-matching (QPM), a result made possible by the fabrication, on Z-cut LN crystals, of periodic structures with a pitch down to 750 nm. Nonlinear copropagating QPM-SHG measurements have been carried out on such structures. The pump source was a Ti:sapphire laser with a tunability range of 700-980 nm and a 40 GHz linewidth. We have measured UV continuous wave light at 390 nm by …
Tuning the high-order harmonic lines of a Nd:Glass laser for soft x-ray laser seeding
2010
Taking advantage of the non-adiabatic blue-shift of high-order harmonics generated by a fixed frequency Nd:Glass laser system, we are able to report more than 50 % coverage of the XUV spectral range between 18 nm and 35 nm. The generated harmonic lines are capable of seeding Ni-like Y, Zr and Mo soft x-ray lasers and others.
Stable and long-time operation of a soft x-ray laser for user applications experiments
2011
LASERIX is a high-power laser facility leading to High-repetition-rate XUV laser pumped by Titanium:Sapphire laser. The aim of this laser facility is to offer Soft XRLs in the 30-7 nm range and auxiliary IR beam that could also be used to produce synchronized XUV sources. This experimental configuration highly enhances the scientific opportunities of the facility, giving thus the opportunity to realize both X-ray laser experiments and more generally pump/probe experiments, mixing IR and XUV sources. In this contribution, the main results concerning both the development of XUV sources(X-Ray lasers and HHG sources) and their use for applications are presented.
Ultrafast optics in coherently spinning molecules
2020
This thesis reports on the study of unidirectional rotation of molecules and focuses on the rotational Doppler effect occuring in the course of third-harmonic generation in coherently spinning molecules.The rotational Doppler effect appears when a circularly polarized wave interacts with an anisotropic rotating object. During the interaction, an exchange of angular momentum and energy between the field and the object occurs, leading to a frequency shift of the wave. In this work, the frequency shift of the third-harmonic generated in unidirectionaly rotating molecules has been observed. An anlytical model developped in the mansucript forsees four kinds of frequency shifts depending on the m…