Search results for "high-spin"

showing 7 items of 7 documents

Cooperative phenomena and light-induced bistability in iron(II) spin-crossover compounds

1999

In iron(II) spin-crossover compounds, the transition from the 1A1 low-spin state at low temperatures to the 5T2 high-spin state at elevated temperatures is accompanied by a large increase in metal-ligand bond lengths. The resulting elastic interactions may be pictured as an internal pressure which is proportional to the concentration of the low-spin species. Because pressure stabilises the low-spin state relative to the high-spin state this results in a positive feedback. Thermal transition curves in neat iron(II) spin-crossover compounds are thus invariable much steeper than in diluted mixed crystals, and the high-spin→low-spin relaxation following the light-induced population of the high-…

Phase transitioneducation.field_of_studyCooperative effectsCondensed matter physicsBistabilityChemistryRelaxation (NMR)PopulationInternal pressureIron(II) coordination compoundsLIESSTInorganic ChemistryChemical physicsSpin crossoverddc:540Materials ChemistryHigh-spinlow-spin relaxationCondensed Matter::Strongly Correlated ElectronsBistabilityPhysical and Theoretical ChemistrySpin-crossoverGround stateeducationCoordination Chemistry Reviews
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High-spin states beyond the proton drip-line: Quasiparticle alignments in 113 Cs

2014

Abstract Excited states have been studied in the deformed proton emitter 113Cs. Gamma-ray transitions have been unambiguously assigned to 113Cs by correlation with its characteristic proton decay, using the method of recoil-decay tagging. Two previously identified rotational bands have been observed and extended to tentative spins of 45/2 and 51 / 2 ħ , with excitation energies over 8 MeV above the lowest state. These are the highest angular momenta and excitation energies observed to date in any nucleus beyond the proton drip-line. Transitions in the bands have been rearranged compared to previous work. A study of aligned angular momenta, in comparison to the predictions of Woods–Saxon cra…

PhysicsNuclear and High Energy PhysicsProtonSpin statesSpinsta114Proton decayNuclear Theoryrecoil decay taggingProton decayQuasiparticle alignmentsgamma ray spectroscopylcsh:QC1-999High-spin statesExcited stateQuasiparticleRecoil-decay taggingGamma spectroscopyGamma-ray spectroscopyAtomic physicsNuclear ExperimentExcitationlcsh:PhysicsPhysics Letters B
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High-spin states of $^{218}$Th

2020

Abstract High-spin states in the N = 128 nucleus 218Th have been investigated following fusion–evaporation reactions, using the recoil-decay tagging technique. Due to the short-lived nature of the ground state of 218Th prompt γ rays have been correlated with the α decay of the daughter nucleus 214Ra. The level scheme representing the decay of excited states has been extended to (16+) with the observation of six previously unreported transitions. The observations are compared with the results of shell model calculations and within the context of the systematics of neighbouring nuclei.

PhysicsNuclear and High Energy PhysicsSpin states010308 nuclear & particles physicsSHELL modelThoriumchemistry.chemical_elementContext (language use)01 natural sciencesNuclear physicsmedicine.anatomical_structurehigh-spin stateschemistryExcited stateNuclear Physics - Theory0103 physical sciencesmedicinenuclear and particle physicsydinfysiikka010306 general physicsGround stateNuclear ExperimentNucleus
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Angular momentum population in fragmentation reactions

2009

Neutron-deficient nuclei with N = 126 have been populated following projectile fragmentation of a 238U beam with energy 1 GeV/A. The decay of several previously reported isomers has been measured. This will allow us to calculate high-spin isomeric ratios and compare them with model calculations to allow a better understanding of the reaction mechanism. Algora, Alejandro, Alejandro.Algora@ific.uv.es ; Molina Palacios, Francisco Manuel, Francisco.Molina@ific.uv.es ; Rubio Barroso, Berta, Berta.Rubio@ific.uv.es

UNESCO::FÍSICA::Física molecular:FÍSICA [UNESCO]:FÍSICA::Física molecular [UNESCO]UNESCO::FÍSICANeutron-deficient nucleiProjectile fragmentationHigh-spin isometric ratiosNeutron-deficient nuclei ; Projectile fragmentation ; High-spin isometric ratios ; Reaction mechanismReaction mechanism
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Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements in Hg-184,Hg-186 and two-state mixing calculations

2014

Abstract: The neutron-deficient mercury isotopes, 184 , 186 Hg, were studied with the recoil distance Doppler-shift method using the Gammasphere array and the K ̈ oln plunger device. The differential decay curve method was employed to determine the lifetimes of the yrast states in 184 , 186 Hg. An improvement on previously measured values of yrast states up to 8 + is presented as well as first values for the 9 3 state in 184 Hg and 10 + state in 186 Hg. B ( E 2) values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia model, allowing for extraction of spin-dependent mixing strengths and amplitudes. peerReviewed

high-spin stateslight mercury isotopesdecay curve method
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High-spin states beyond the proton drip-line: Quasiparticle alignments in Cs-113

2015

Excited states have been studied in the deformed proton emitter 113Cs. Gamma-ray transitions have been unambiguously assigned to 113Cs by correlation with its characteristic proton decay, using the method of recoil-decay tagging. Two previously identified rotational bands have been observed and extended to tentative spins of 45/2 and 51/2 h¯, with excitation energies over 8 MeV above the lowest state. These are the highest angular momenta and excitation energies observed to date in any nucleus beyond the proton drip-line. Transitions in the bands have been rearranged compared to previous work. A study of aligned angular momenta, in comparison to the predictions of Woods–Saxon cranking calcu…

proton decayhigh-spin statesNuclear Theoryrecoil decay taggingNuclear Experimentquasiparticle alignmentsgamma ray spectroscopy
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First identification of rotational band structures in Re-166(75)91

2015

Excited states in the odd-odd, highly neutron-deficient nucleus 166Re have been investigated via the 92Mo(78Kr, 3p1n) 166Re reaction. Prompt γ rays were detected by the JUROGAM II γ -ray spectrometer, and the recoiling fusion-evaporation products were separated by the recoil ion transport unit (RITU) gas-filled recoil separator and implanted into the Gamma Recoil Electron Alpha Tagging spectrometer located at the RITU focal plane. The tagging and coincidence techniques were applied to identify the γ -ray transitions in 166Re, revealing two collective, strongly coupled rotational structures, for the first time. The more strongly populated band structure is assigned to the πh11/2[514]9/2− ⊗ ν…

total data readouthigh-spinsignature inversionnucleimass regionshape coexistenceNuclear Experimentspectrocopy
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