Search results for "ice crystals"

In-line holography of cloud volumes applied to the measurement of raindrops and snowflakes

1998

Abstract The ground-based HODAR (HOlographic Droplet and Aerosol Recording) of the University of Mainz has been operational since 1989 on the Kleiner Feldberg Mountain Observatory near Frankfurt/Main, Germany, in a `small volume' configuration. With this setup an air volume of approximately 1 l can be in situ recorded, which allows it to image all aerosol particles and droplets with diameter larger than 6 μm contained in the sample volume in situ. Recently the beam diameter and optical path length of the inline system have been enlarged such that large cloud volumes (approximately 500 l) can be recorded on single holograms. During the holographic image reconstruction step in the laboratory,…

2020

Abstract. An ice cloud chamber was developed at the Johannes Gutenberg University of Mainz for generating several thousand data points for mass and sedimentation velocity measurements of ice crystals with sizes less than 150 µm. Ice nucleation was initiated from a cloud of supercooled droplets by local cooling using a liquid nitrogen cold finger. Three-dimensional tracks of ice crystals falling through the slightly supersaturated environment were obtained from the reconstruction of sequential holographic images, automated detection of the crystals in the hologram reconstructions, and particle tracking. Through collection of the crystals and investigation under a microscope before and after …

Ice supersaturations and cirrus cloud crystal numbers

2009

Upper tropospheric observations outside and inside of cirrus clouds indicate water vapour mixing ratios sometimes exceeding water saturation. Relative humidities over ice (RHice) of up to and more than 200% have been reported from aircraft and balloon measurements in recent years. From these observations a lively discussion continues on whether there is a lack of understanding of ice cloud microphysics or whether the water measurements are tainted with large uncertainties or flaws. Here, RHice in clear air and in ice clouds is investigated. Strict quality-checked aircraft in situ observations of RHice were performed during 28 flights in tropical, mid-latitude and Arctic field experiments in…

Environmental scanning electron microscopy (ESEM) as a new technique to determine the ice nucleation capability of individual atmospheric aerosol par…

2007

Abstract Heterogeneous ice nucleation on synthetic silver iodide, natural kaolinite and montmorillonite particles via condensation, freezing and deposition modes was studied by environmental scanning electron microscopy (ESEM) in the temperature range of 250–270 K. By increasing the H2O pressure in the sample chamber at constant temperature, ice formation can be studied in situ and can be related to the chemical composition of the particles that can be determined simultaneously. For silver iodide and kaolinite, supersaturation values of first ice formation are in good agreement (1–2% absolute) with diffusion chamber experiments. For both substances, threshold temperatures for the condensati…

A laboratory study of the effects of a kerosene-burner exhaust on ice nucleation and the evaporation rate of ice crystals

1998

Abstract Laboratory experiments are described during which the influence of gases and particles from the exhaust of a kerosene burner on microphysical processes were studied. In one experimental investigation the evaporation rates of ice crystals polluted with the kerosene-burner exhaust were compared with the evaporation rates of pure ice crystals. During another experimental investigation the ice nucleating ability of the exhaust particles was studied in terms of the efficiency of the exhaust particles to act as deposition and condensation freezing nuclei, as immersion freezing nuclei, and as contact nuclei. The results of our experiments showed that the evaporation rate of ice crystals p…

Comparing irradiance fields derived from Moderate Resolution Imaging Spectroradiometer airborne simulator cirrus cloud retrievals with solar spectral…

2007

[1] During the Cirrus Regional Study of Tropical Anvils and Cirrus Layers–Florida Area Cirrus Experiment, the Moderate Resolution Imaging Spectroradiometer (MODIS) airborne simulator (MAS) and the solar spectral flux radiometer (SSFR) operated on the same aircraft, the NASA ER-2. While MAS provided two-dimensional horizontal fields of cloud optical thickness and effective ice particle radius, the SSFR measured spectral irradiance in the visible to near-infrared wavelength range (0.3–1.7 μm). The MAS retrievals, along with vertical profiles from a combined radar/lidar system on board the same aircraft were used to construct three-dimensional cloud fields, which were input into Monte Carlo ra…

New investigations on homogeneous ice nucleation: the effects of water activity and water saturation formulations

2022

Laboratory measurements at the AIDA cloud chamber and airborne in-situ observations suggest that the homogeneous freezing thresholds at low temperatures are possibly higher than expected from the so-called “Koop-line”. This finding is of importance, because the ice onset relative humidity affects the cirrus cloud coverage and, at the very low temperatures of the tropical tropopause layer, together with the number of ice crystals also the transport of water vapor into the stratosphere. Both, the appearance of cirrus clouds and the amount of stratospheric water feed back to the radiative budget of the atmosphere. In order to explore the enhanced ice onset humidities, we re-examine…

Arctic low-level boundary layer clouds: in situ measurements and simulations of mono- and bimodal supercooled droplet size distributions at the top l…

2015

Abstract. Aircraft borne optical in situ size distribution measurements were performed within Arctic boundary layer clouds with a special emphasis on the cloud top layer during the VERtical Distribution of Ice in Arctic clouds (VERDI) campaign in April and May 2012. An instrumented Basler BT-67 research aircraft operated out of Inuvik over the Mackenzie River delta and the Beaufort Sea in the Northwest Territories of Canada. Besides the cloud particle and hydrometeor size spectrometers the aircraft was equipped with instrumentation for aerosol, radiation and other parameters. Inside the cloud, droplet size distributions with monomodal shapes were observed for predominantly liquid-phase Arct…

A laboratory study on the uptake of HCl, HNO3, and SO2 gas by ice crystals and the effect of these gases on the evaporation rate of the crystals

1998

The results of our new and earlier laboratory studies on the uptake of gases by ice crystals are summarized in terms of (1) the equilibrium phase diagram for a system gas/H2O, (2) the effect of these gases on the evaporation rate of ice crystals, and (3) in terms of the uptake of the gases by water drops. It is shown that the intrinsic quasi-liquid layer significantly affects the uptake of a gas by an ice surface in that, depending on the gas phase concentration, the layer thickness may be considerably increased by depressing the equilibrium freezing point causing additional surface melting. It is further shown that the evaporation rate of ice particles previously exposed to a gas may becom…

Effects of ice crystal habit on thermal infrared radiative properties and forcing of cirrus

2007

[1] The impact of assumed ice crystal morphology on thermal infrared (IR) radiative properties of subtropical cirrus is quantified. In particular, the crystal-shape-dependent profiles of downwelling and upwelling thermal IR (broadband and spectral) irradiances and the radiative forcing of cirrus (at the top and bottom of the atmosphere) are investigated. For this purpose, airborne measurements of ice crystal size distribution (in terms of ice crystal maximum dimension) from the CRYSTAL-FACE campaign and a recently published library of thermal IR optical properties of nonspherical ice crystal habits are implemented into radiative transfer simulations. Two cirrus cases are studied in detail: …