Search results for "isolaatio"

showing 5 items of 5 documents

Raman spectroscopy and crystal-field split rotational states of photoproducts CO and H2 after dissociation of formaldehyde in solid argon

2012

Raman signal is monitored after 248 nm photodissociation of formaldehyde in solid Ar at temperatures of 9–30 K. Rotational transitions J = 2 ← 0 for para-H2 fragments and J = 3 ← 1 for ortho-H2 are observed as sharp peaks at 347.2 cm−1 and 578.3 cm−1, respectively, which both are accompanied by a broader shoulder band that shows a split structure. The rovibrational spectrum of CO fragments has transitions at 2136.5 cm−1, 2138.3 cm−1, 2139.9 cm−1, and 2149 cm−1. To explain the observations, we performed adiabatic rotational potential calculations to simulate the Raman spectrum. The simulations indicate that the splitting of rotational transitions is a site effect, where H2 molecules can resi…

Raman spektroskopiacarbon compoundstranslational statesphotodissociationmatriisi-isolaatiohydrogen neutral moleculesrotational statesrotational-vibrational statesfotodissosiaatiorotaatio-vibraatiotilatmolecule-photon collisionsRaman spectrainterstitialsorgaaniset yhdisteet
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Isolated glyoxylic acid-water 1:1 complexes in low temperature argon matrices

2015

Abstract The 1:1 hydrogen bonded complexes between glyoxylic acid (GA) and water are studied in low temperature argon matrices. Four different complex structures were found in deposited matrices. The lowest energy conformer (T1) of GA was found to form complex, where the water molecule was attached to the opposite side of the intramolecular hydrogen bond in the molecule (T1B). Interestingly, this complex was estimated to be +8.0 kJ mol −1 higher in energy than the most stable structure (T1A), where the water is inserted into the internal hydrogen bond, and also found in solid argon but in smaller abundance. For the second-lowest energy conformer of GA (T2), the two lowest-energy complex str…

Spectrophotometry InfraredHydrogenMolecular Conformationconformerschemistry.chemical_elementVibrationkonformeeritAnalytical Chemistrychemistry.chemical_compoundIsomerismComputational chemistryglyoxylic acidMoleculematriisi isolaatioArgonvärähdysspektroskopiaInstrumentationConformational isomerismta116SpectroscopyGlyoxylic acidhydrogen bondArgonglyoksyylihappoHydrogen bondMatrix isolationGlyoxylatesWatermatrix isolationHydrogen Bondinglaskennallinen kemiacomputational chemistryAtomic and Molecular Physics and OpticsCold TemperatureCrystallographychemistryIntramolecular forcevetysidosSpectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy
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Interspecific interactions and premating reproductive isolation

2008

Interspecific interactions have several evolutionary consequences: for example, two species may compete, hybridize, or behave aggressively towards each other, or there may be predator–prey interactions. One consequence of these interactions is the evolution of premating reproductive isolation between the two species. The most obvious interspecific interaction, which has an effect on reproductive isolation, is the avoidance of hybridization, or, in other words, the reinforcement process. The theory of reinforcement states that when hybridization is maladaptive, selection pressure causes a divergence in female mate preference and/or in male secondary sexual characters. It is often assumed tha…

aggressiivisuusLisääntymisisolaatioZoologyReproductive isolationInterspecific competitionBiologykilpailusaalistus
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Do allopatric male Calopteryx virgo damselflies learn species recognition?

2012

There is a growing amount of empirical evidence that premating reproductive isolation of two closely related species can be reinforced by natural selection arising from avoidance of maladaptive hybridization. However, as an alternative for this popular reinforcement theory, it has been suggested that learning to prefer conspecifics or to discriminate heterospecifics could cause a similar pattern of reinforced premating isolation, but this possibility is much less studied. Here, we report results of a field experiment in which we examined (i) whether allopatric Calopteryx virgo damselfly males that have not encountered heterospecific females of the congener C. splendens initially show discri…

reinforcementsudenkorennotlisääntymisisolaatiopremating reproductive isolationoppiminenOdonataspeciationeducation1181 Ecology evolutionary biologylajiutuminenspecies discriminationOriginal Research
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Sexual and postmating reproductive isolation between allopatric Drosophila montana populations suggest speciation potential

2011

Background - Widely distributed species with populations adapted to different environmental conditions can provide valuable opportunities for tracing the onset of reproductive incompatibilities and their role in the speciation process. Drosophila montana, a D. virilis group species found in high latitude boreal forests in Nearctic and Palearctic regions around the globe, could be an excellent model system for studying the early stages of speciation, as a wealth of information concerning this species' ecology, mating system, life history, genetics and phylogeography is available. However, reproductive barriers between populations have hereto not been investigated. Results - We report both pr…

speciationisolaatiopremating isolationlajiutuminenpostmating isolationlisääntyminen
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