Search results for "liquid"
showing 10 items of 4351 documents
A Wind Tunnel Study of Turbulence Effects on the Scavenging of Aerosol Particles by Water Drops
2001
Abstract Laboratory experiments are described where the effects of turbulence on the impaction scavenging of aerosol particles by water drops were investigated. During the experiments the drops were freely suspended at their terminal velocities in the Mainz vertical wind tunnel. Turbulence in the tunnel airstream was produced by placing a needle obstruction upstream of the floating drop. The energy dissipation rates e were between 0.03 and 0.5 m2 s−3. The power spectrum covered a range of k values between 102 and 3 × 103 m−1, agreeing with atmospheric observations within this range. Collector drops of 346-μm, 1.68-mm, and 2.88-mm radius were exposed to indium acetylacetonate aerosol particl…
3-D imaging and quantification of graupel porosity by synchrotron-based micro-tomography
2011
The air bubble structure is an important parameter to determine the radiation properties of graupel and hailstones. For 3-D imaging of this structure at micron resolution, a cryo-stage was developed. This stage was used at the tomography beamline of the Swiss Light Source (SLS) synchrotron facility. The cryo-stage setup provides for the first time 3-D-data on the individual pore morphology of ice particles down to infrared wavelength resolution. In the present study, both sub-mm size natural and artificial ice particles rimed in a wind tunnel were investigated. In the natural rimed ice particles, Y-shaped air-filled closed pores were found. When kept for half an hour at −8 °C, this morpholo…
The effects of different radiation parametrizations on cloud evolution
1997
With the use of the microphysical stratus model (MISTRA), investigations into the effects of variations in the radiative-transfer parametrizations on cloud development have been undertaken. Two radiative-transfer schemes were coupled with the microphysical-thermodynamical section of MISTRA, one based on the exponential sumfitting method and the other based on the correlated k-distribution method of determining gaseous absorption properties. Model runs were initiated with parameter values in accordance with measurements made over the North Sea and comparisons made between model runs where only the radiation schemes were altered. Results indicated that differences between the two schemes had …
Comparison of ERA40 cloud top phase with POLDER-1 observations
2008
[1] A detailed grid-point-based comparison of the cloud top phase derived from the 40-year reanalyses (ERA40) of the European Centre for Medium-Range Weather Forecasts (ECMWF) with satellite measurements is presented. For this purpose an algorithm is implemented to extract a two-dimensional “satellite-like” field of the cloud top phase from ERA40 data. This field is compared with cloud top phase data from the Polarization and Directionality of the Earth Reflectances (POLDER-1) instrument which was in orbit from November 1996 to June 1997. The thermodynamic cloud phase in ERA40 data is parameterized as a function of temperature with pure liquid clouds above 0°C, pure ice clouds below −23°C a…
A multi-model assessment of the impact of sea spray geoengineering on cloud droplet number
2012
Artificially increasing the albedo of marine boundary layer clouds by the mechanical emission of sea spray aerosol has been proposed as a geoengineering technique to slow the warming caused by anthropogenic greenhouse gases. A previous global model study (Korhonen et al., 2010) found that only modest increases (< 20%) and sometimes even decreases in cloud drop number (CDN) concentrations would result from emission scenarios calculated using a windspeed dependent geoengineering flux parameterisation. Here we extend that work to examine the conditions under which decreases in CDN can occur, and use three independent global models to quantify maximum achievable CDN changes. We find that dec…
Reproducing cloud microphysical and irradiance measurements using three 3D cloud generators
2007
Using three cloud generators, three-dimensional (3D) cloud fields are reproduced from microphysical cloud data measured in situ by aircraft. The generated cloud fields are used as input to a 3D radiative transfer model to calculate the corresponding fields of downward and upward irradiance, which are then compared with airborne and ground-based radiation measurements. One overcast stratocumulus scene and one broken cumulus scene were selected from the European INSPECTRO field experiment, which was held in Norwich, UK, in September 2002. With these data, the characteristics of the three different cloud reproduction techniques are assessed. Besides vertical profiles and histograms of measured…
Effects of 20–100 nm particles on liquid clouds in the clean summertime Arctic
2016
Abstract. Observations addressing effects of aerosol particles on summertime Arctic clouds are limited. An airborne study, carried out during July 2014 from Resolute Bay, Nunavut, Canada, as part of the Canadian NETCARE project, provides a comprehensive in situ look into some effects of aerosol particles on liquid clouds in the clean environment of the Arctic summer. Median cloud droplet number concentrations (CDNC) from 62 cloud samples are 10 cm−3 for low-altitude cloud (clouds topped below 200 m) and 101 cm−3 for higher-altitude cloud (clouds based above 200 m). The lower activation size of aerosol particles is ≤ 50 nm diameter in about 40 % of the cases. Particles as small as 20 nm ac…
Control of solute concentrations in cloud and fog water by liquid water content
2000
We measured the concentrations of Cl^−, NO_3^−, and SO_4^(2−) in atmospheric cloudwater collected with a passive collector from a remote marine site and the concentrations of Cl^−, NO_3^−, SO_4^(2−), Na^+ and NH_4^+ in cloudwater from a continental site. At the continental site, an active rotating arm collector was employed for cloudwater collection. At both locations, we observed an inverse relationship between the measured ion concentrations and the liquid water content of the clouds. The product of the observed concentrations and the liquid water content, the cloudwater loading, was found to be nearly constant. A study of published cloudwater data showed that at the majority of the exami…
Airborne investigation of the aerosols–cloud interactions in the vicinity and within a marine stratocumulus over the North Sea during EUCAARI (2008)
2013
Abstract Within the European Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) project, the Meteo France research aircraft ATR-42 was operated from Rotterdam (Netherlands) airport during May 2008, to perform scientific flights dedicated to the investigation of aerosol–cloud interactions. The objective of this study is to illustrate the impact of cloud processing on the aerosol particle physical and chemical properties. The presented results are retrieved from measurements during flight operation with two consecutive flights, first from Rotterdam to Newcastle (United Kingdom) and subsequently reverse along the same waypoints back to Rotterdam using data measured with compact Time …
Characterization of methyl orange and its photocatalytic degradation products by HPLC/UV–VIS diode array and atmospheric pressure ionization quadrupo…
2002
Abstract HPLC/UV–VIS diode array and HPLC/MS techniques were successfully applied to the analysis of sulfonated molecules present in samples coming from the photocatalytic degradation of the azo dye indicator, methyl orange. The substrate was chosen as a simple model for the study of reactions involving the more complex commercial products used for the dyeing of textile fibers. Unexpected MS fragmentation path was observed, due to the very stable methyl orange molecular structure. The chromatographic information were combined with the obtained MS, MS/MS data and the UV–VIS diode array spectra and allowed to rationalize the molecular structures attributable to the various degradation product…