Search results for "nanoscale"
showing 10 items of 752 documents
Narrow-band tunable THz detector in antiferromagnets via N\'eel spin-orbit torque and spin-transfer torque
2017
We study dynamics of antiferromagnets induced by simultaneous application of dc spin current and ac charge current, motivated by the requirement of all-electrically controlled devices in THz gap (0.1-30 THz). We show that ac electric current, via N\'eel spin orbit torques, can lock the phase of a steady rotating N\'eel vector whose precession is controlled by a dc spin current. In the phase-locking regime the frequency of the incoming ac signal coincides with the frequency of autooscillations which for typical antiferromagnets fall into the THz range. The frequency of autooscillations is proportional to the precession-induced tilting of the magnetic sublattices related to the so-called dyna…
Resonant tunneling through a macroscopic charge state in a superconducting SET transistor
1997
We predict theoretically and observe in experiment that the differential conductance of a superconducting SET transistor exhibits a peak which is a complete analogue in a macroscopic system of a standard resonant tunneling peak associated with tunneling through a single quantum state. In particular, in a symmetric transistor, the peak height is universal and equal to $e^2/2\pi \hbar$. Away from the resonance we clearly observe the co-tunneling current which in contrast to the normal-metal transistor varies linearly with the bias voltage.
Quantum Phase Slips in one-dimensional Josephson Junction Chains
2013
We have studied quantum phase-slip (QPS) phenomena in long one-dimensional Josephson junction series arrays with tunable Josephson coupling. These chains were fabricated with as many as 2888 junctions, where one sample had a tunable weak link in the middle. Measurements were made of the zero-bias resistance, $R_0$, as well as current-voltage characteristics (IVC). The finite $R_0$ is explained by QPS and shows an exponential dependence on $\sqrt{E_J/E_C}$ with a distinct change in the exponent at $R_0=R_Q=h/4e^2$. When $R_0 > R_Q$ the IVC clearly shows a remnant of the Coulomb blockade, which evolves to a zero-current state with a sharp critical voltage as $E_J$ is tuned to a smaller val…
Quantum advantage in a molecular spintronic engine that harvests thermal fluctuation energy
2022
Recent theory and experiments have showcased how to harness quantum mechanics to assemble heat/information engines with efficiencies that surpass the classical Carnot limit. So far, this has required atomic engines that are driven by cumbersome external electromagnetic sources. Here, using molecular spintronics, we propose an implementation that is both electronic and autonomous. Our spintronic quantum engine heuristically deploys several known quantum assets by having a chain of spin qubits formed by the paramagnetic Co centers of phthalocyanine (Pc) molecules electronically interact with electron-spin selecting Fe/C60 interfaces. Density functional calculations reveal that transport fluct…
Discrete saturation thickness and anomalous potential height of native ultrathin aluminum oxide tunnel barriers
2001
We have investigated planar metal - insulator - metal tunnel junctions with aluminum oxide as dielectricum. These oxide barriers were grown on an aluminum electrode in pure oxygen at room temperature till saturation. We observed discrete barrier widths separated by \Delta s \approx 0.38 nm, corresponding to the addition of one layer of oxygen atoms. The minimum thickness of s_0 \approx 0.54 nm is due to a double layer of oxygen. We found a strong and systematic dependence of the barrier height \Phi_0 on the thickness s like \Phi_0 \approx 2.5 eV / s^2(nm), which nearly coincides with the kinetic electron energy E = h^2/2ms^2 for which the deBroglie wavelength matches the width of the barrie…
Derivation of the universal decay cascade distribution
2014
A detailed derivation of the decay cascade probability distribution stated in Eqs. (4)-(6) and (11) of Phys. Rev. Lett. 104, 186805 (2010) [arXiv:0901.4102] by Kashcheyevs and Kaestner is provided. Recurrence relations are solved explicitly and connections between solutions in different limits are demonstrated.
Data mining, dashboard and statistical analysis: a powerful framework for the chemical design of molecular nanomagnets
2021
Three decades of research in molecular nanomagnets have raised their magnetic memories from liquid helium to liquid nitrogen temperature thanks to a wise choice of the magnetic ion and coordination environment. Still, serendipity and chemical intuition played a main role. In order to establish a powerful framework for statistically driven chemical design, we collected chemical and physical data for lanthanide-based nanomagnets, catalogued over 1400 published experiments, developed an interactive dashboard (SIMDAVIS) to visualise the dataset, and applied inferential statistical analysis. Our analysis showed that the Arrhenius energy barrier correlates unexpectedly well with the magnetic memo…
Strong Coupling of Coherent Phonons to Excitons in Semiconducting Monolayer MoTe$_2$
2023
The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of semiconducting monolayer 2$H$-MoTe$_2$ encapsulated with $h$BN using broadband optical pump-probe microscopy. The sub-40-fs pump pulse triggers extremely intense and long-lived coherent oscillations in the spectral region of the A' and B' exciton resonances, up to $\sim$20% of the maximum transient signal, due to the displacive excitation of the out-of-plane $A_{1g}$ phonon. Ab-initio calculations reveal a dramatic rearrangement of the optical absorption of…
Origin of the spin Seebeck effect probed by temperature dependent measurements in Gd$_{3}$Fe$_{5}$O$_{12}$
2014
We probe the spin Seebeck effect in Gd$_{3}$Fe$_{5}$O$_{12}$/Pt hybrid structures as a function of temperature and observe two sign changes of the spin Seebeck signal with decreasing temperature. A first sign change occurs at a temperature close to the Gd$_{3}$Fe$_{5}$O$_{12}$ magnetic compensation point at around 280 K. There the spin Seebeck signal changes sign abruptly with unaltered amplitude, indicating that the spin current is mainly caused by the magnetic Fe sub-lattices, which reorient their directions at this temperature. A second, more gradual sign change takes place around the ordering temperature of the Gd sub-lattice in the range of 65-85 K, showing that the Gd magnetic sub-lat…
Multiorbital exciton formation in an organic semiconductor
2023
Harnessing the optoelectronic response of organic semiconductors requires a thorough understanding of the fundamental light-matter interaction that is dominated by the excitation of correlated electron-hole pairs, i.e. excitons. The nature of these excitons would be fully captured by knowing the quantum-mechanical wavefunction, which, however, is difficult to access both theoretically and experimentally. Here, we use femtosecond photoemission orbital tomography in combination with many-body perturbation theory to gain access to exciton wavefunctions in organic semiconductors. We find that the coherent sum of multiple electron-hole pair contributions that typically make up a single exciton c…