Search results for "nonlinear optics"
showing 10 items of 482 documents
Second harmonic generation in selenium-metal structures
2009
The article examines the processes of second harmonic generation (SHG) when selenium-metal (Cu) film structures are illuminated by femtosecond radiation (180 fs, 80 MHz) at wavelength 800 – 1000 nm. Selenium-copper structures were obtained by successive thermal evaporation of selenium and copper onto the glass substrate in vacuum. Microanalysis of the film composition was performed to determine amount of copper in thin films. The as-evaporated selenium-copper structures were crystallised by annealing in inert atmosphere at temperature 85°C. Just evaporated as well as annealed thin films were explored. The experiment was performed by confocal microscope [1] where the femtosecond radiation fr…
Tellurites fibers for infrared supercontinuum sources : opto-geometric profiles and extrinsic absorptions management
2016
This PhD thesis work focuses on the synthesis and purification of vitreous materials used for the development of waveguides with varied profiles, dedicated to supercontinuum (SC) generation between 1 and 5 μm.Concerning the purification of tellurite glasses, several leads were followed, but best results are obtained for the purification of the TeO2-ZnO-Na2O glassy system by the means of zinc fluoride. Attenuation measurements performed on several meter-long single-index fiber samples reveal the nearly complete elimination of water-related absorptions between 3 and 4 μm (OH ions concentration lower than 1 ppm mass.). Such water-purified glasses were firstly dedicated to microstructured optic…
Polarization Modulation Instability in All-Normal Dispersion Microstructured Optical Fibers With Quasi-Continuous Pump
2019
We report the experimental observation of the polarization modulation instability (PMI) effect in all-normal dispersion (ANDi) microstructured optical fibers (MOFs) with quasi-continuous pumping. The small unintentional birefringence (~10-5), that any realistic non-polarization maintaining MOF exhibits, contributes to this nonlinear effect. PMI can produce two sidebands whose polarization state is orthogonal to the polarization of the pump. In this work, only one type of PMI process is observed, i.e., when the pump is polarized along the slow axis of the fiber and sidebands are generated in the fast axis mode. This PMI process was studied experimentally in two ANDi fibers with different dis…
Novel second-order nonlinear optical polymer materials containing indandione derivativatives as a chromophore
2006
Second order non linear optical (NLO) properties of sPMMA based host-guest systems containing eight dimethylaminobenzylidene -1, 3 - indandione (DMABI) related chromophores have been investigated by means of quantum chemical calculations and SHG experimental characterization. Ab initio calculations with basis set 6-31G were used for molecular geometry determination as well as in the calculations of molecular hyperpolarizability by FF approach. Influence of the chromophore concentration on the host-guest film NLO performance was obtained by SHG Maker fringe experiments. The highest value of d53233 =80 pm/V (frequency corrected value d033 =12 pm/V) at chromophore concentration 15 %wt have bee…
About the role of hamiltonian singularities in controlled systems : applications in quantum mechanics and nonlinear optics
2012
This thesis has two goals: the first one is to improve the control techniques in quantum mechanics, and more specifically in NMR, by using the tools of geometric optimal control. The second one is the study of the influence of Hamiltonian singularities in controlled systems. The chapter about optimal control study three classical problems of NMR : the inversion problem, the influence of the radiation damping term, and the steady state technique. Then, we apply the geometric optimal control to the problem of the population transfert in a three levels quantum system to recover the STIRAP scheme.The two next chapters study Hamiltonian singularities. We show that they allow to control the polar…
A fiber-based limiter at 170 Gbit/s for all-optical regeneration
2009
We report the numerical and experimental studies of a spectrally filtered fiber-based optical limiter at 170 Gbit/s. The device, including less than 1 km-long of highly nonlinear optical fiber and a 3 nm-width filter, exhibits good performance at an average input power of 14.5 dBm. No power penalty has been observed and a strong robustness against optical noise has been demonstrated.
Spatial beam cleaning in quadratic nonlinear medium
2018
We show experimentally that a laser beam scrambled by propagation in a short segment of multimode fiber may be cleaned by the nonlinear propagation in KTP cristal with type-II second-harmonic generation.
Wave dynamics and turbulence in multimode optical systems
2021
The subject of this thesis essentially focuses on the experimental and theoretical study of optical turbulence in different types of nonlinear media. The first part of the manuscript is devoted to the study of thermalization and condensation of optical waves during their propagation in graded-index multimode fibers. The analysis based on the wave turbulence theory reveals that the disorder inherent to light propagation in an optical fiber induces a significant acceleration of the process of optical thermalization, which can clarify the mechanism of certain regimes of spatial beam cleaning recently reported in the literature. We show experimentally that the optical field relaxes during its p…
Second- and third-harmonic generation as a local probe for nanocrystal-doped polymer materials with a suppressed optical breakdown threshold
2003
Abstract Second- and third-harmonic generation processes are shown to allow the detection of absorptive agglomerates of nanocrystals in transparent materials and the visualization of optical breakdown in nanocomposite materials. Correlations between laser-induced breakdown and the behavior of the second- and third-harmonic signals produced in SiC/PMMA nanocomposite films are studied. The potential of second- and third-harmonic generation for the on-line visualization of laser breakdown in nanocomposite polymer materials is revealed, with the ablative material removal being monitored by the decay of the second- and third-harmonic signals. The second and third harmonics generated around the o…
Optical characterization of YCa4O(BO3)3 and Nd:YCa4O(BO3)3 crystals
2007
International audience; We report a complete optical characterization of YCa4O(BO3)3 and Nd:YCa4O(BO3)3 crystals. We studied the relative orientation between the dielectric and the crystallographic frames as a function of the wavelength and performed accurate phase-matching angles measurements for second harmonic generation, using a single crystal cut as a sphere. We also recorded polarized luminescence spectra of Nd:YCOB along the principal axes of the dielectric frame. For both crystals, we measured the gray-tracking and the thermo-optic properties as a function of temperature and wavelength using oriented slabs. Finally, we measured all their dielectric and electro-optic coefficients, as…