Search results for "nonlinear optics"
showing 10 items of 482 documents
Unusual response to environmental polarity in a nonlinear-optical benzylidene-type chromophore containing a 1,3-bis(dicyanomethylidene)indane accepto…
2017
One of the strongest known electron-accepting fragments used in the synthesis of organic dyes for applications in nonlinear optics (NLO) is 1,3-bis(dicyanomethylidene)indane (BDMI). By studying a benzylidene-type push-pull chromophore bearing a 5-carboxy-BDMI electron-acceptor and 4-(dimethylamino)aniline donor fragment, we demonstrate that this class of compounds can show unusual response to the polarity of the surrounding medium. The combined results of UV-Vis absorption spectrometry, NMR experiments and computational modeling indicate that the studied compound undergoes a geometrical transformation that involves an increase in the torsion angle ω between the aniline and indane ring syste…
Influence of Ag, Cu dopants on the second and third harmonic response of ZnO films
2009
International audience; Silver- and copper-doped ZnO films were prepared by radio-frequency (RF)-magnetron sputtering on glass and quartz substrates. The influence of dopants content on the microstructural evolution and optical as well as nonlinear optical (NLO) properties were investigated. It has been found that the grain sizes were enlarged with increasing of Ag, Cu dopants amount in ZnO films. The Ag or Cu doping leads to the optical band gap narrowing. Besides, the second-order NLO response of Ag- and Cu-doped ZnO films is lower than that of undoped ZnO film. The second harmonic generation (SHG) efficiency of the ZnO:Ag film was found to be higher than that of the ZnO:Cu film at the si…
Non-critically phase-matched cascaded THG at 440 nm in KTiOP1−yAsyO4 crystals
1995
Abstract We report the relative nonlinear optical properties of flux-grown KTiOP 1− y As y O 4 crystals ( y =0, y =0.03 and y =0.12). The non-critical phase-matching temperatures along the x -axis for blue generation by type II indirect third harmonic generation from 1318.8 nm and 1320 nm are measured. The phosphorus-arsenic substitution allows a “chemical tuning” of the phase-matching properties, through a birefringence variation, so that non-critical phase-matching at room temperature is possible for the previous interactions. Type II frequency doubling from 1064 nm is briefly considered.
Temperature dependence of refractive index and absorption coefficient of GaSe at 633 nm
1995
Abstract Measurements of the ordinary refractive index and the absorption coefficient ( E /t] to c axis ) of gallium selenide at 633 nm, in the temperature range [20,100] °C, are reported. Useful analytical approximations obtained after a least squares fitting process are provided, as well. These results are basic for any theoretical model of nonlinear and bistable optical devices based on GaSe.
Nonlinear Disorder Mapping via Three Wave Mixing in Poled Lithium Tantalate
2010
We introduce and test a simple approach for the characterization of domain distribution in bulk quadratic ferroelectric crystals, such as periodically poled Lithium Tantalate with random mark-to space ratio.
<title>Effects of light polarization and crystal orientation on the holographic recording efficiency in doped LiNbO<formula><inf>&l…
2008
The holographic recording efficiency in doped LiNbO3 crystals has been studied both experimentally and theoretically depending on the type of dope, on the recording geometry and on the polarizations of the recording and readout light.. The studied crystals can be arranged in the following order by their efficiency: LiNbO3:Cu, LiNbO3:Fe (yet having a smaller thickness and donor concentration than LiNbO3:Cu), LiNbO3:Fe+Cu, LiNbO3:Fe+Ti, LiNbO3:Ti. It was found that the recording geometry with the holographic grating vector along the optical axis is much more efficient than in the perpendicular configuration.This fact is in accordance with the photorefraction theory based on photogalvanic and …
Two-wave mixing at 854 nm in BaTiO3:Rh planar waveguide implanted with He+
2001
Abstract Guided waves at 854 nm are observed in a BaTiO 3 :Rh waveguide fabricated by the technique of ion-beam implantation. The photorefractive interaction between two guided modes is demonstrated and characterized. The experiments reveal that the gain direction is reversed in the guiding layer in comparison with that in the bulk. A maximum gain of 24 cm −1 is achieved.
Filamentation-induced spectral broadening and pulse shortening of infrared pulses in Tellurite glass
2016
Abstract Filamentation of infrared femtosecond pulses in Tellurite glass is reported, leading to the generation of a supercontinuum generation spanning from the visible up to 4 μm. The angular distribution of the supercontinuum shows clear evidence of conical waves generation, in particular, in the visible region. Moreover, taking advantage of the spatio-temporal self-focusing effect occurring in the Tellurite glass, a twofold pulse shortening is demonstrated. Tellurite glass appears as a very convenient, versatile and promising medium for femtosecond nonlinear optics in the infrared region.
Dispersion-optimized multicladding silicon nitride waveguides for nonlinear frequency generation from ultraviolet to mid-infrared
2016
Nonlinear frequency conversion spanning from the ultraviolet to the mid-infrared (beyond 2.4 μm) is experimentally demonstrated in multicladding silicon nitride (𝑆𝑖𝑋𝑁𝑌) waveguides. By adjusting the waveguide cross-section the chromatic dispersion is flattened, which enhances both the efficiency and the bandwidth of the nonlinear conversion. How accurately the dispersion is tailored is assessed through chromatic dispersion measurements and an experiment/simulation comparison of the dispersive waves' wavelength locations. Undesirable fluctuations of both the refractive index and the dimensions of the waveguide during the fabrication process result in a dispersion unpredictability of at l…
Nonlinear optical properties of silver nanoparticles: separating thermo-optical and Kerr effects
2021
In this paper, we present a study on thermo-optical effect in core-shell silver/thiol-termination ligand nanoparticles. Nanoparticles were dissolved in Dichloromethane. Experimental measurements were carried out using a Z-scan setup. As laser sources we used two 1064 nm lasers: i) 28 ps pulse width laser with 1000 Hz pulse repetition rate; ii) 8 ns pulse width laser with changeable pulse repetition rate 200 – 40 000 Hz. To study what processes lead to refractive index changes we used the polarization-resolved Z-scan method. Comparing ps and ns results showed that response time of single pulse thermal effects for organic solvents depends on beam size while for nanoparticles it corresponds to…