Search results for "nuclear reaction"
showing 10 items of 449 documents
Nuclear Forensics: A methodology applicable to Nuclear Security and to Non-Proliferation
2011
Nuclear Security aims at the prevention and detection of and response to, theft, sabotage, unauthorized access, illegal transfer or other malicious acts involving nuclear material". Nuclear Forensics is a key element of nuclear security. Nuclear Forensics is defined as a methodology that aims at re-establishing the history of nuclear material of unknown origin. It is based on indicators that arise from known relationships between material characteristics and process history. Thus, nuclear forensics analysis includes the characterization of the material and correlation with production history. To this end, we can make use of parameters such as the isotopic composition of the nuclear material…
A study of a helium-jet ion guide for an on-line isotope separator
1981
Abstract A new method based on helium-jet techniques permits primary recoil ions, produced in radioactive decay or in nuclear reactions to be run directly through a mass separator. Results obtained with a 227 Ac source promise qualities complementary with those obtained with conventional ion sources and indicate an overall efficiency of the order of 10%. Preliminary results with 20 Na recoils from the 20 Ne(p,n)-reaction indicate that most of the ionic species transported out from the target chamber are negatively charged.
Beta decay of neutron-rich cobalt and nickel isotopes
1998
We report on the first β-γ spectroscopy measurements of the neutron-rich 68–70Co and 70–74Ni nuclei, produced in proton-induced fission of 238U and ionized in a laser ion guide coupled to an on-line mass separator. Several γ lines from the decay of these nuclei have been identified, half-lives determined and production cross sections deduced. The derived level schemes for the copper and nickel isotopes show that the occupation of the ν(1g9/2) state has a strong influence on the structure of these neutron-rich nuclei. This may have a clear impact on the predicted structure and decay properties of doubly-magic 78Ni.
Smooth terminating bands inTe112: Particle-hole induced collectivity
2007
The Gammasphere spectrometer, in conjunction with the Microball charged-particle array, was used to investigate high-spin states in Te-112 via Ni-58(Ni-58, 4p gamma) reactions at 240 and 250 MeV. Several smooth terminating bands were established, and lifetime measurements were performed for the strongest one using the Doppler-shift attenuation method. Results obtained in the spin range 18-32h yield a transition quadrupole moment of 4.0 +/- 0.5eb, which corresponds to a quadrupole deformation epsilon(2)=0.26 +/- 0.03; this value is significantly larger than the ground-state deformation of tellurium isotopes. It was also possible to extract a transition quadrupole moment for the yrast band in…
Editorial: The Future of Nuclear Structure: Challenges and Opportunities in the Microscopic Description of Nuclei
2021
The past two decades have witnessed tremendous progress in the microscopic description of atomic nuclei. The Topical Review `The Future of Nuclear Structure' aims at summarizing the current state-of-the-art microscopic calculations in Nuclear Theory and to give a useful reference for young researches who wish to learn more about this exciting discipline.
Improvement of ESR dosimetry for thermal neutron beams through the addition of gadolinium.
2007
In this paper, the addition of gadolinium is proposed as a useful tool to enhance the electron spin resonance (ESR) sensitivity of organic compounds to thermal neutrons. The target of this work is the detection, through the ESR technique, of the thermal neutron fluence in a mixed field of photons and neutrons. Gadolinium was chosen because it has a very high capture cross section to thermal neutrons; its nuclear reaction with thermal neutrons induces complex inner shell transitions that generate, besides other particles, Auger electrons, which in turn release their energy in the neighborhood (only several nanometers) of the place of reaction. Gadolinium was added to two organic molecules: a…
Submillisecond On-Line Mass Separation of Nonvolatile Radioactive Elements: An Application of Charge Exchange and Thermalization Processes of Primary…
1985
Transportation of thermalized primary recoil ions from nuclear reactions by helium flow has been investigated as a means of injecting short-lived radioactive nuclides into an on-line isotope separator. Several short-lived radioactive isotopes of highly nonvolatile elements such as B, Sc, Nb, and W have been separated. The efficiency for heavy nuclides with half-lives above 1 ms is between 1 and 10%. The shortest-lived activity identified in an on-line separation is the 182-\ensuremath{\mu}s isomeric state in $^{207}\mathrm{Bi}$.
Helium-jet ion guide for an on-line isotope separator
1981
Abstract A new method based on helium-jet techniques permits primary recoil ions produced in radioactive decay or in nuclear reactions to be run directly through a mass separator. Test results with a 227 Ac source give promise of qualities complementary to those obtained with conventional ion sources. This, 69 ± 5 per cent of the recoil particles transported with pure, commercial helium are positive ions, and 66 ± 5 per cent of them are mass separated. Nearly equal efficiencies are expected for most chemical elements and compounds. The mass spectra are remarkably free from groups caused by impurities. The shortest achievable separation time is estimated to be of the order of one millisecond.
The Szilard–Chalmers effect in macrocyclic ligands to increase the specific activity of reactor-produced radiolanthanides: Experiments and explanatio…
2012
Abstract Successful utilization of medical isotopes in the radiolabeling reactions to a significant degree depends on the technically achievable specific activity. In this respect, the Szilard-Chalmers effect is considered in detail as a radiochemical tool to increase the specific activity of radionuclides produced by direct nuclear reactions. In the present study, a physico-chemical model is described utilizing the specific aspects of thermodynamically and kinetically stabilised metal-ligand complexes. The approach is applied as a proofof- principle study to increase the specific activity of 166Ho, produced via the (n, γ) nuclear reaction. As a target material, 165Ho-DOTA is used. In this …
Single-neutron orbits near 78 Ni: Spectroscopy of theN=49isotope 79 Zn
2015
Single-neutron states in the Z=30, N=49isotope 79Zn have been populated using the 78Zn(d,p)79Zn transfer reaction at REX-ISOLDE, CERN. The experimental setup allowed the combined detection of protons ejected in the reaction, and of γrays emitted by 79Zn. The analysis reveals that the lowest excited states populated in the reaction lie at approximately 1MeV of excitation, and involve neutron orbits above the N=50shell gap. From the analysis of γ-ray data and of proton angular distributions, characteristic of the amount of angular momentum transferred, a5/2+configuration was assigned to a state at 983keV. Comparison with large-scale-shell-model calculations supports a robust neutron N=50shell…