Search results for "nuclide"
showing 10 items of 397 documents
Recent results on heavy-ion induced reactions of interest for neutrinoless double beta decay at INFN-LNS
2019
Abstract The NUMEN project aims at accessing experimentally driven information on Nuclear Matrix Elements (NME) involved in the half-life of the neutrinoless double beta decay (0νββ). In this view measurements of Heavy Ion (HI) induced Double Charge Exchange (DCE) reaction cross sections are performed with high-accuracy. In particular, the (18O,18Ne) and (20Ne,20O) reactions are used as tools for β+β+ and β-β- decays, respectively. In the experiments, performed at INFN - Laboratory Nazionali del Sud (LNS) in Catania, the beams are accelerated by the Superconducting Cyclotron (CS) and the reaction ejectiles are detected the MAGNEX magnetic spectrometer. The measured cross sections are challe…
Recent results on Heavy-Ion induced reactions of interest for 0νββ decay
2019
An updated overview of recent results on Heavy-Ion induced reactions of interest for neutrinoless double beta decay is reported in the framework of the NUMEN project. The NUMEN idea is to study heavy-ion induced Double Charge Exchange (DCE) reactions with the aim to get information on the nuclear matrix elements for neutrinoless double beta (0νββ) decay. Moreover, to infer the neutrino average masses from the possible measurement of the half- life of 0νββ decay, the knowledge of the nuclear matrix elements is a crucial aspect. Uma visão geral atualizada dos resultados recentes sobre reações induzidas por íons pesados de interesse para o decaimento beta duplo sem neutrinos é relatada na es…
Thorium-234 derived information on particle residence times and sediment deposition in shallow waters of the south-western Baltic Sea
2009
Abstract Activities of the naturally occurring, short-lived and highly particle-reactive radionuclide tracer 234 Th in the dissolved and particulate phase were measured at three shallow-water stations (maximum water depths: 15.6, 22.7 and 30.1 m) in Mecklenburg Bay (south-western Baltic Sea) to constrain the time scales of the dynamics and the depositional fate of particulate matter. Activities of particle-associated (> 0.4 μm) and total (particulate + dissolved) 234 Th were in the range of 0.08–0.11 dpm L − 1 and 0.11–0.20 dpm L − 1 , respectively. The activity ratio of total 234 Th and its long-lived and conservative parent nuclide 238 U was well below unity (range: 0.09–0.19) indicating …
Validating the use of caesium-137 measurements to estimate soil erosion rates in a small drainage basin in Calabria, Southern Italy
2001
Recent concern for problems of soil degradation and the offsite impacts of accelerated erosion has highlighted the need for improved methods of estimating rates and patterns of soil erosion by water. The use of environmental radionuclides, particularly caesium-137 (137Cs), as a means of estimating rates of soil erosion and deposition is attracting increasing attention and the approach has now been recognised as possessing several important advantages. However, one important uncertainty associated with the use of 137Cs measurements to estimate soil erosion rates is the need to employ a calibration relationship to convert the measured 137Cs inventory to an estimate of the erosion rate. Existi…
Validating erosion rate estimates provided by caesium-137 measurements for two small forested catchments in Calabria, southern Italy
2003
Increasing concern for problems of soil degradation and the off-site impacts of accelerated erosion has generated a need for improved methods of estimating rates and patterns of soil erosion by water. The use of environmental radionuclides, particularly 137 Cs, to estimate erosion rates has attracted increased attention and the approach has been shown to possess several important advantages. However, the use of 137 Cs measurements to estimate erosion rates introduces one important uncertainty, namely, the need to employ a conversion model or relationship to convert the measured reduction in the 137 Cs inventory to an estimate of the erosion rate. There have been few attempts to validate the…
Emission tomography with a large-hole collimator (CACAO): a possible new way to improve radionuclide imaging.
2002
This work aims to improve the quality of scintigraphy. It evaluates the use of a large-hole collimator, the Computer Aided Collimation Gamma Camera Project (CACAO), in SPECT. Acquisition data from the same object were simulated for CACAO and for a conventional collimator. Better signal-to-noise ratios were found for CACAO images, whatever the number of emitted photons. This work demonstrates that high-resolution images may be obtained with large-hole collimators. The combination of CACAO and pixilated detectors may further improve radionuclide imaging.
Decomposition studies of group 6 hexacarbonyl complexes. Part 1: Production and decomposition of Mo(CO)6 and W(CO)6
2015
Abstract Chemical studies of superheavy elements require fast and efficient techniques, due to short half-lives and low production rates of the investigated nuclides. Here, we advocate for using a tubular flow reactor for assessing the thermal stability of the Sg carbonyl complex – Sg(CO)6. The experimental setup was tested with Mo and W carbonyl complexes, as their properties are established and supported by theoretical predictions. The suggested approach proved to be effective in discriminating between the thermal stabilities of Mo(CO)6 and W(CO)6. Therefore, an experimental verification of the predicted Sg–CO bond dissociation energy seems to be feasible by applying this technique. By in…
Laser spectroscopy of neutron deficient lead and thallium isotopes: Systematics of nuclear radii in the Z = 82 region
1989
Publisher Summary The high sensitivity achievable in laser spectroscopic methods allows the extraction of nuclear quantities even of artificially produced short-lived nuclides far off from nuclear stability. By analyzing the hyperfine structure and the isotope shift magnetic dipole moments, the electric quadrupole moments and the change of the nuclear charge radius can be studied. This chapter describes an experiment that was carried out at the GSI on-line mass separator using collinear fast atomic-beam laser spectroscopy. Radioactive lead and thallium isotopes were produced by bombarding natural tungsten targets with oxygen beams. For the lighter thallium isotopes, a tantalum target was us…
Rapid continous radiochemical separations by thermochromatography in connection with a gas-jet recoil-transport system
1980
Abstract A combination of a gas-jet recoil-transport system with a thermochromatographic system has been studied as a technique for rapid, continuous radiochemical separations. Fission products were used as a model for complex mixtures of elements. A nitrogen gas-jet containing potassium chloride clusters was applied to transport nuclides produced in a reactor from the target area to the thermochromatographic column. Conversion of the reaction products carried by the gas-jet volatile species was achieved by stopping the clusters in a quartz-wool plug located in the column and kept at high temperatures and feeding a reactive gas into the column. Several reactive gases producing volatile chlo…
Chemical reactions in a gas-jet recoil-transport system: Continuous separation procedure for selenium and tellurium from fission products
1978
Abstract Chemical selectivity in a gas-jet recoil-transport system can be achieved by chemical reactions with the carrier gas. This is demonstrated for an ethylene-nitrogen jet in which volatile species of selenium and tellurium are formed by passing the gas through a reaction zone heated to 860°C. Rapid continuous separation procedures for selenium and tellurium from fission products based on this effect are described and some decay data of the neutron-rich nuclides 85–88Se and 135–137Te obtained with these methods are given.