Search results for "nuclide"
showing 10 items of 397 documents
Miss Piggy, a californium-252 fission fragment source as a generator of short-lived radionuclides
2003
Abstract Carrier-free short-lived nuclides are employed in many different fields of modern nuclear chemistry. The two main production strategies are either thermal neutron-induced fission of 235U or 239Pu at nuclear reactors or spallation neutron sources or charged particle-induced nuclear reactions at accelerator facilities. An alternative method is to use a spontaneously fissioning nuclide. A facility applying this technique (“Miss Piggy”) was built at the University of Berne (Switzerland). Californium-252 (252Cf), which has a 3% fission branch and a half-life of 2.645 a, is used for the production of short-lived fission products that are stopped in an adjacent recoil chamber. Short-lived…
The limits of the nuclear landscape
2012
In 2011, 100 new nuclides were discovered. They joined the approximately 3,000 stable and radioactive nuclides that either occur naturally on Earth or are synthesized in the laboratory. Every atomic nucleus, characterized by a specific number of protons and neutrons, occupies a spot on the chart of nuclides, which is bounded by 'drip lines' indicating the values of neutron and proton number at which nuclear binding ends. The placement of the neutron drip line for the heavier elements is based on theoretical predictions using extreme extrapolations, and so is uncertain. However, it is not known how uncertain it is or how many protons and neutrons can be bound in a nucleus. Here we estimate t…
New nuclideHa263
1992
A new nuclide $^{263}\mathrm{Ha}$ was produced in the bombardment of a $^{249}\mathrm{Bk}$ target with 93-MeV $^{18}\mathrm{O}$ ions. It was detected via spontaneous fission counting and was shown to have a half-life of about 0.5 min. This activity was also separated from the reaction products by automated rapid chemical separations using cation-exchange chromatography in 0.05M \ensuremath{\alpha}-hydroxyisobutyric acid. After chemical separation, $^{263}\mathrm{Ha}$ was found to decay by spontaneous fission (${57}_{\mathrm{\ensuremath{-}}15}^{+13}$%) and by \ensuremath{\alpha} emission (${\mathit{E}}_{\mathrm{\ensuremath{\alpha}}}$=8.35 MeV, 43%) with a half-life of ${27}_{\mathrm{\ensurem…
α-Decay branching ratios measured by γ-ray tagging
2008
Abstract The nuclides 168–170Pt were produced by bombarding isotopically enriched 92,94Mo targets with 336, 348 MeV 78Kr ions. Prompt γ rays were detected at the target position and provided a selection criterion for the 168–170Pt nuclei. This technique enables the problem of the background from higher-energy α decays in the spectrum to be circumvented. The Pt nuclei were separated in flight using the gas-filled separator RITU and implanted into the GREAT spectrometer, which was used to study subsequent α decays. The α -decay branching ratios of 164–166Os were deduced from the fraction of selected 168–170Pt nuclei correlated with α decays of 164–166Os. The resulting branching ratios agree w…
Experimental study of fragmentation products in the reactions112Sn+112Snand124Sn+124Snat 1AGeV
2011
Production cross sections and longitudinal velocity distributions of the projectilelike residues produced in the reactions ${}^{112}\text{Sn}+{}^{112}\text{Sn}$ and ${}^{124}\text{Sn}+{}^{124}\text{Sn}$, both at an incident beam energy of 1$A$ GeV, were measured with the high-resolution magnetic spectrometer, the Fragment Separator of GSI. For both reactions the characteristics of the velocity distributions and nuclide production cross sections were determined for residues with atomic number $Z\ensuremath{\ge}10$. A comparison of the results of the two reactions is presented.
Studies of Weak Beta-Delayed Protons Emitted in the Decay of Odd-Z, Tz = -3/2 Nuclei
1983
Radioactive decay of Tz = - 3/2 nuclides, 27P and 31Cl, predicted to be weak β-delayed proton precursors, have been looked for. Two proton groups having energies of 989 ± 15 and 1528 ± 20 keV and a half-life of 150 ± 25 ms were associated with the decay of 31Cl. The search for 27P is still under way, but the first qualitative results are briefly discussed.
Decays of new nuclides and isomers beyond the proton drip line - The influence of neutron configurations
2008
Bozok University;Erciyes University;et al.;Istanbul University;Nigde University;The Turkish Atomic Energy Authority (TAEK)
Measurement of radionuclide activities induced in target components of an IBA CYCLONE 18/9 by gamma-ray spectrometry with HPGe and LaBr3: Ce detector…
2014
Cyclotrons are used worldwide to produce radiopharmaceuticals by proton irradiation of a suitable target. The intense secondary neutron beam generated by proton interactions with the target induce high radionuclide activities in the target assembly parts that may result in an exposure to high dose levels of the operators during maintenance. The main goal of this work is to evaluate gamma-emitting radionuclide activities induced in Havar foils and titanium windows of a target assembly and carousel stripper forks of an IBA CYCLONE 18/9 cyclotron. The knowledge of radionuclide inventory for each component is required by many companies to assess risk for operators before waste handling and disp…
First observation ofγrays emitted from excited states south-east ofSn132: Theπg9/2−1⊗νf7/2multiplet ofIn83132
2016
For the first time, the γ decay of excited states has been observed in a nucleus situated in the quadrant south-east of doubly magic Sn132, a region in which experimental information so far is limited to ground-state properties. Six γ rays with energies of 50, 86, 103, 227, 357, and 602 keV were observed following the β-delayed neutron emission from Cd85133, populated in the projectile fission of a U238 beam at the Radioactive Isotope Beam Factory at RIKEN within the EURICA project. The new experimental information is compared to the results of a modern realistic shell-model calculation, the first one in this region very far from stability, focusing in particular on the π0g9/2-1 - ν1f7/2 pa…
Time-separated oscillatory fields for high-precision mass measurements on short-lived Al and Ca nuclides
2008
High-precision Penning trap mass measurements on the stable nuclide 27Al as well as on the short-lived radionuclides 26Al and 38,39Ca have been performed by use of radiofrequency excitation with time-separated oscillatory fields, i.e. Ramsey's method, as recently introduced for the excitation of the ion motion in a Penning trap, was applied. A comparison with the conventional method of a single continuous excitation demonstrates its advantage of up to ten times shorter measurements. The new mass values of 26,27Al clarify conflicting data in this specific mass region. In addition, the resulting mass values of the superallowed beta-emitter 38Ca as well as of the groundstate of the beta-emitte…