Search results for "plasmon"

Novel prospects in hyperbolic metamaterials: Dyakonov-like surface waves

2014

Hot electrons and nonlinear optical nanoantennas

2017

The large field enhancement generated at the surface of a resonant plasmonic nanoparticle, or optical antennas, is the key mechanism that eventually led to the development of nonlinear plasmonics [1-2]. While the resonance may boost the nonlinear yield of an adjacent structure or surrounding medium, it was soon realized that optical antennas possess nonlinear coefficients comparable or exceeding those of standard nonlinear optical materials [3]. We discuss here two nonlinear optical processes — incoherent multi-photon luminescence (MPL) and coherent second-harmonic generation (SHG) — emitted from gold rod optical antennas upon local illumination with a tightly focused femtosecond near-infra…

Variational theory of soliplasmon resonances

2013

We present a first-principles derivation of the variational equations describing the dynamics of the interaction of a spatial soliton and a surface plasmon polariton (SPP) propagating along a metal/dielectric interface. The variational ansatz is based on the existence of solutions exhibiting differentiated and spatially resolvable localized soliton and SPP components. These states, referred to as soliplasmons, can be physically understood as bound states of a soliton and a SPP. Their respective dispersion relations permit the existence of a resonant interaction between them, as pointed out in Ref.[1]. The existence of soliplasmon states and their interesting nonlinear resonant behavior has …

Soliton-plasmon resonances as Maxwell nonlinear bound states

2012

We demonstrate that soliplasmons (soliton–plasmon bound states) appear naturally as eigenmodes of nonlinear Maxwell’s equations for a metal/Kerr interface. Conservative stability analysis is performed by means of finite element numerical modeling of the time-independent nonlinear Maxwell equations. Dynamical features are in agreement with the presented nonlinear oscillator model.

Plasmon-driven Bessel beams

2012

We report on subwavelength diffraction-free beams with grazing propagation in metal-dielectric devices. The nondiffracting beams are resonantly transmitted through the nanostructured medium leading to light confinement and wave amplification around the beam axis.

Analysis of the plasmonic excitations in assemblies of three-dimensional electron clusters

2020

In the quest to built novel metamaterials with unique optical properties, three-dimensional assemblies of metal clusters and nanoparticles are gathering significant attention. Organized geometries, such as tetrahedra and icosahedra, can be built, for example, by using DNA strands or virus capsids as templates. Here we use the jellium model and time-dependent density functional theory to study the plasmonic resonances in different arrangements of eight-electron clusters from the electronic perspective. A charge transfer ratio index based on the induced transition densities is used to quantify the charge transfer nature of the excitations at different energies. We vary the size, shape, and in…

Plasmonic Focusing Reduces Ensemble Linewidth

2012

In this chapter I present an effect the coating of gold nanorods with a silver shell is evocating: a reduction of the ensemble plasmon linewidth by changing the plasmon-shape relation, which connects the particle shape with its plasmon resonance wavelength. This change, we term “plasmonic focusing” (Sect. 10.2), leads to less variation of resonance wavelengths for the same particle size distribution. Section 10.3 explains the effect of increasing single particle linewidth during the coating process, which is therefore not the reason for the observed ensemble linewidth decrease. This is rather a result from a change in the plasmon-shape relation explained in Sect. 10.4. Using a simple model,…

Photon bunching of the nonlinear photoluminescence emitted by plasmonics metals

2021

International audience; In this report, we investigate the statistical temporal distribution of nonlinear upconverted photoluminescence emitted by gold and silver nanostructures excited by focused near-infrared laser pulses. We systematically observe a clear signature of photon bunching regardless of the nano-object's geometry, material's crystalline arrangement, and electronic band structure. The similarity of the data obtained across very different plasmonic objects confirms that these types of nonlinear radiation share a common chaotic origin and result from a collection of emitters. The correlation of photons at a picosecond time scale released by nanoscale nonlinear sources of broadban…

Multi-frequency super-scattering from sub-wavelength graphene-coated nanotubes

2019

A cylindrical multilayered structure with three coupled graphene shells is shown to behave as a dual-band super-scatterer at mid-infrared frequencies. Under the 2D plasmonic nature of graphene material, multiple scattering resonances are attained in the deep subwavelength regime using an isotropic material. In the proposed structure, we efficiently exploit the existing three plasmonic resonances in each scattering channel. These resonances are tailored by dispersion engineering, which is simply displayed through the Bohr model applied to the associated planar structure. For the super-scatterer design, it is essential that the resonances of multiple channels coincide in a single frequency. H…

Surface Plasmons for Chiral Sensing

2021

Chiral sensitive techniques have been used to probe the fundamental symmetries of the universe, study biomolecular structures, and even develop safe drugs. The traditional method for the measurement of chirality is through optical activity, however, chiroptical signals are inherently weak and often suppressed by large backgrounds. Different techniques have been proposed to overcome the limitations of traditionally used optical polarimetry, such as cavity- and/or nanophotonic-based schemes. In this chapter we demonstrate how surface plasmon resonance can be employed as a new research tool for chiral sensing, which we term here as CHIral Surface Plasmon Resonance (CHISPR). We present how surf…