Search results for "polymerointi"

showing 2 items of 2 documents

Highly Syndiotactic or Isotactic Polyhydroxyalkanoates by Ligand-Controlled Yttrium-Catalyzed Stereoselective Ring-Opening Polymerization of Function…

2017

International audience; Reported herein is the first stereoselective controlled ROP of a specific family of racemic functional β-lactones, namely 4-alkoxymethylene-β-propiolactones (BPL(OR) s). This process is catalyzed by an yttrium complex stabilized by a nonchiral tetradentate amino alkoxy bisphenolate ligand _ONOO(R'2) ₍2-) , which features both a good activity and a high degree of control over the molar masses of the resulting functional poly(3-hydroxyalkanoate)s. A simple modification of the R' substituents in ortho and para position on the ligand platform allows for a complete reversal from virtually pure syndioselectivity (Ps up to 0.91 with R'=cumyl) to very high isoselectivity (Pi…

esteritStereochemistryring-opening polymerizationchemistry.chemical_element010402 general chemistry01 natural sciencesRing-opening polymerizationCatalysisCatalysispolymerointiTacticity[CHIM]Chemical SciencesYttriumpolymeeritta116β-lactonespolymersMolar mass010405 organic chemistryLigand[CHIM.ORGA]Chemical Sciences/Organic chemistrystereoselective catalysisGeneral MedicineGeneral ChemistryYttrium0104 chemical scienceschemistrykatalyysiAlkoxy groupStereoselectivitybeta-lactonesAngewandte Chemie International Edition
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The Effect of Mechanocatalytic Pretreatment on the Structure and Depolymerization of Willow

2020

In this study, the effect of a mechanocatalytic pretreatment on the structure of willow and sugar release from pretreated willow was explored. In the mechanocatalytic approach, the pretreatment consists of solvent-free impregnation with sulfuric acid and a mechanical treatment with ball milling. Willow sawdust and pretreated samples were analyzed with field emission scanning electron microscope and X-ray diffraction. The products in the sugar solution were determined as the total reducing sugars with the 3,5-dinitrosalicylic acid method and monosaccharides with capillary electrophoresis. According to the results, milling increased the sugar production, depending on the sulfuric acid load. T…

rikkihappo020209 energyselluloosaWillow sawdustpajut02 engineering and technology010501 environmental sciencesXyloseesikäsittelylcsh:Chemical technologycomplex mixtures01 natural sciencesCatalysisHydrolysatepolymerointilcsh:ChemistryBall millingchemistry.chemical_compoundlignocellulose0202 electrical engineering electronic engineering information engineeringmechanocatalytic pretreatmentMonosaccharidelcsh:TP1-1185Physical and Theoretical ChemistrySugarBall mill0105 earth and related environmental scienceschemistry.chemical_classificationDepolymerizationSulfuric acidsulfuric aciddigestive oral and skin physiologytechnology industry and agriculturefood and beveragesSulfuric acidwillow sawdustlcsh:QD1-999chemistryvisual_artvisual_art.visual_art_mediumball millingSawdustLignocelluloseMechanocatalytic pretreatmentNuclear chemistryCatalysts
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