Search results for "rct"

Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs)

2005

International audience; A PSC was detected on 6 February 2003 in the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (~10-4cm-3) of small nitric acid (HNO3) containing particles (dTNAT, these NAT particles have the potential to grow further and to remove HNO3 from the stratosphere, thereby enhancing polar ozone loss. Interestingly, the NAT particles formed in less than a day at temperatures just slightly below TNAT (T>TNAT-3.1K). This unique measurement of PSC formation at extremely low NAT saturation ratios (SNAT?10) constrains current NAT nucleation theories. We suggest, that the NAT particles have formed heterogeneo…

Relationships between the Antarctic Oscillation, the Madden-Julian Oscillation and ENSO, and consequences for rainfall analysis

2010

Abstract The Antarctic Oscillation (AAO) is the leading mode of atmospheric variability in the Southern Hemisphere mid- and high latitudes (south of 20°S). In this paper, the authors examine its statistical relationships with the major tropical climate signals at the intraseasonal and interannual time scales and their consequences on its potential influence on rainfall variability at regional scales. At the intraseasonal time scale, although the AAO shows its most energetic fluctuations in the 30–60-day range, it is not unambiguously related to the global-scale Madden–Julian oscillation (MJO) activity, with in particular no coherent phase relationship with the MJO index. Moreover, in the hi…

2017

Abstract. Size-resolved and vertical profile measurements of single particle chemical composition (sampling altitude range 50–3000 m) were conducted in July 2014 in the Canadian high Arctic during an aircraft-based measurement campaign (NETCARE 2014). We deployed the single particle laser ablation aerosol mass spectrometer ALABAMA (vacuum aerodynamic diameter range approximately 200–1000 nm) to identify different particle types and their mixing states. On the basis of the single particle analysis, we found that a significant fraction (23 %) of all analyzed particles (in total: 7412) contained trimethylamine (TMA). Two main pieces of evidence suggest that these TMA-containing particles origi…

Observations of atmospheric chemical deposition to high Arctic snow

2017

Abstract. Rapidly rising temperatures and loss of snow and ice cover have demonstrated the unique vulnerability of the high Arctic to climate change. There are major uncertainties in modelling the chemical depositional and scavenging processes of Arctic snow. To that end, fresh snow samples collected on average every 4 days at Alert, Nunavut, from September 2014 to June 2015 were analyzed for black carbon, major ions, and metals, and their concentrations and fluxes were reported. Comparison with simultaneous measurements of atmospheric aerosol mass loadings yields effective deposition velocities that encompass all processes by which the atmospheric species are transferred to the snow. It is…

Relationship between weather regimes and atmospheric rivers in East Antarctica.

2021

25 pages; International audience; Here, we define weather regimes in the East Antarctica—Southern Ocean sector based on daily anomalies of 700 hPa geopotential height derived from ERA5 reanalysis during 1979–2018. Most regimes and their preferred transitions depict synoptic-scale disturbances propagating eastwards off the Antarctic coastline. While regime sequences are generally short, their interannual variability is strongly driven by the polarity of the Southern Annular Mode (SAM). Regime occurrences are then intersected with atmospheric rivers (ARs) detected over the same region and period. ARs are equiprobable throughout the year, but clearly concentrate during regimes associated with …

Cloud phase identification of Arctic boundary-layer clouds from airborne spectral reflection measurements: test of three approaches

2008

Abstract. Arctic boundary-layer clouds were investigated with remote sensing and in situ instruments during the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign in March and April 2007. The clouds formed in a cold air outbreak over the open Greenland Sea. Beside the predominant mixed-phase clouds pure liquid water and ice clouds were observed. Utilizing measurements of solar radiation reflected by the clouds three methods to retrieve the thermodynamic phase of the cloud are introduced and compared. Two ice indices IS and IP were obtained by analyzing the spectral pattern of the cloud top reflectance in the near infrared (1500–1800 nm wavelength) spectral range whi…

Evidence of ice crystals at cloud top of Arctic boundary-layer mixed-phase clouds derived from airborne remote sensing

2009

Abstract. The vertical distribution of ice crystals in Arctic boundary-layer mixed-phase (ABM) clouds was investigated by airborne remote-sensing and in situ measurements during the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign in March and April 2007. Information on the spectral absorption of solar radiation by ice and liquid water cloud particles is derived from airborne measurements of solar spectral radiation reflected by these clouds. It is shown by calculation of the vertical weighting function of the measurements that the observed absorption of solar radiation is dominated by the upper cloud layers (50% within 200 m from cloud top). This vertical weighti…

The Southern Annular Mode seen through weather regimes

2012

This article investigates the prominent features of the Southern Hemisphere (south of 20°S) atmospheric circulation when extracted using EOF analysis and a k-means clustering algorithm. The focus is on the southern annular mode (SAM), the nature of its recent trend, and the zonal symmetry of associated spatial patterns. The study uses the NCEP–Department of Energy Atmospheric Model Intercomparison Project II Reanalysis (NCEP-2) (period 1979–2009) to obtain robust patterns over the recent years and the Twentieth Century Reanalysis Project (period 1871–2008) to document decadal changes. Also presented is a comparison of these signals against a station-based reconstruction of the SAM index an…

Vertical profiles of light absorption and scattering associated with black carbon particle fractions in the springtime Arctic above 79° N

2020

Despite the potential importance of black carbon (BC) for radiative forcing of the Arctic atmosphere, vertically resolved measurements of the particle light scattering coefficient (σsp) and light absorption coefficient (σap) in the springtime Arctic atmosphere are infrequent, especially measurements at latitudes at or above 80∘ N. Here, relationships among vertically distributed aerosol optical properties (σap, σsp and single scattering albedo or SSA), particle microphysics and particle chemistry are examined for a region of the Canadian archipelago between 79.9 and 83.4∘ N from near the surface to 500 hPa. Airborne data collected during April 2015 are combined with gro…

Chemical composition and source attribution of sub-micrometre aerosol particles in the summertime Arctic lower troposphere

2021

Aerosol particles impact the Arctic climate system both directly and indirectly by modifying cloud properties, yet our understanding of their vertical distribution, chemical composition, mixing state, and sources in the summertime Arctic is incomplete. In situ vertical observations of particle properties in the high Arctic combined with modelling analysis on source attribution are in short supply, particularly during summer. We thus use airborne measurements of aerosol particle composition to demonstrate the strong contrast between particle sources and composition within and above the summertime Arctic boundary layer. In situ measurements from two complementary aerosol mass spectrometers, t…