Search results for "second-harmonic"
showing 10 items of 121 documents
Parabolic pulse generation through passive reshaping of gaussian pulses in a normally dispersive fiber
2007
We numerically and experimentally demonstrate that a Gaussian pulse can be reshaped into a pulse with a stable parabolic intensity profile during propagation in normally dispersive nonlinear fibers.
High third and second order non linearities of chalcogenide glasses and fibers for compact infrared non linear devices.
2008
Due to their intrinsic nature, chalcogenide glasses present attractive nonlinearities from third and second order, with values reaching between 10 and 1000 times those of silica. We present a study of their properties and their shaping with the purpose to reach efficient devices in the near-mid infrared.
Nonlinear optical fiber polarization tracking at 200 krad/s
2011
International audience; We demonstrate endless nonlinear polarization stabilization with a standard telecom fiber at a tracking speed of 200 krads/s. We provide a simple analytical estimate for the response time of nonlinear polarization control
Optical Cavity-Less 40-GHz Picosecond Pulse Generator in the Visible Wavelength Range
2019
International audience; High-repetition-rate optical frequency-comb sources emitting picosecond pulses play important roles in variousscientific researches and industrial applications. Such ultrafast pulse sources are mostly generated in opticalcavities or microresonators. By means of the wavelength-conversion techniques, it is possible to transfer thecavity-based near-IR robust and compact sources to the mid-IR or to the visible wavelength regions [1-2], forwhich there is an increasing demand, for biophotonics and other applications. Here we demonstrate the generationof high-repetition-rate picosecond pulses in the visible wavelength range by using a fully optical cavity-lessconfiguration.…
Temporal coherence in mirrorless optical parametric oscillators
2012
International audience; One of the unique features of mirrorless optical parametric oscillators based on counterpropagating three-wave interactions is the narrow spectral width of the wave generated in the backward direction. In this work, we in- vestigate experimentally and numerically the influence that a strong phase modulation in the pump has on the spectral bandwidths of the parametric waves and on the efficiency of the nonlinear interaction. The effects of group-velocity mismatch and group-velocity dispersion are elucidated. In particular, it is shown that the substan- tial increase in temporal coherence of the backward-generated wave can be obtained even for pumping with a temporally…
Residual Phase Noise Measurement of Optical Second Harmonic Generation in PPLN Waveguides
2017
We report on the characterization, including residual phase noise and fractional frequency instability, of fiber-coupled PPLN non-linear crystals. These components are devoted to frequency doubling 871 nm light from an extended-cavity diode laser to produce a 435.5 nm beam, corresponding to the ytterbium ion electric quadrupole clock transition. We measure doubling efficiencies of up to 117.5 %/W. Using a Mach-Zehnder interferometer and an original noise rejection technique, the residual phase noise of the doublers is estimated to be lower than ${\rm -35\, dBrad^2/Hz}$ at 1 Hz, making these modules compatible with up-to-date optical clocks and ultra-stable cavities. The influence of externa…
Nonlinear optical properties of diaromatic stilbene, butadiene and thiophene derivatives
2021
Series of highly polar stilbene (1a–e), diphenylbutadiene (2a–c) and phenylethenylthiophene (3a–c) derivatives were prepared via Horner–Wadsworth–Emmons method with a view to produce new and efficient materials for second harmonic generation (SHG) in the solid-state. The single-crystal X-ray structures of compounds 1–3 reveal extensive polymorphism and a peculiar photodimerization of the 2-chloro-3,4-dimethoxy-4′-nitrostilbene derivative 1a to afford two polymorphs of tetra-aryl cyclobutane 4. The stilbene congeners 2-chloro-3,4-dimethoxy-4′-nitrostilbene (1a·non-centro), 5-bromo-2-hydroxy-3-nitro-4′-nitrostilbene (1b) and 4-dimethylamino-4′-nitrostilbene (1e), as well as 4′-fluoro-4′′-nitr…
Second harmonic generation in self-assembled alternating multilayers of hemicyanine containing polymers and polyvinylamine
1995
Abstract Assembly of noncentrosymmetric multilayers is a facile technique for preparing noncentrosymmetric films avoiding electrical poling procedures and problems from subsequent relaxation of the induced orientational order. A maximum Xzzz of 13 × 10−9 esu was achieved for the assembly of up to six layers. Current problems are the long-term hydrolysation of the hemicyanine nonlinear optical chromophores and the reduction of polar orientation with increasing layer thickness.
Poling dynamics of an EO active material using parallel-plate electrodes
2017
We describe the sample preparation and experimental setup for second harmonic generation measurement of electro-optical (EO) chromophore/polymer system at the time of contact-poling. Different types of spacers for avoiding electric breakdown due to avalanche multiplication are compared. Electric field threshold values for second harmonic generation are observed in all samples.
Electron crystallography and organic materials with non-linear optical properties
1999
Results of electron microscopic studies of crystal structures of a number of bis-benzylidene cyclohexanones are presented. It is shown that some of these compounds are efficient crystalline non-linear optically active (NLO) chromophores with second harmonic generation (SHG) properties. Appropriately functionalized chromophores of this type can be used as a polycondensation comonomer to produce partly crystalline main-chain NLO-active polymers. Electron diffraction crystal structural data, obtained for very small crystals, allowed us to get reasonable estimations of macroscopic crystal NLO-coefficients, relating quantum-chemically calculated molecular first hyperpolarizability components to …