Search results for "spontaneous emission"
showing 10 items of 145 documents
Solvatochromism Unravels the Emission Mechanism of Carbon Nanodots
2016
High quantum yield, photoluminescence tunability, and sensitivity to the environment are hallmarks that make carbon nanodots interesting for fundamental research and applications. Yet, the underlying electronic transitions behind their bright photoluminescence are strongly debated. Despite carbon-dot interactions with their environment should provide valuable insight into the emitting transitions, they have hardly been studied. Here, we investigate these interactions in a wide range of solvents to elucidate the nature of the electronic transitions. We find remarkable and systematic dependence of the emission energy and kinetics on the characteristics of the solvent, with strong response of …
Manipulating spontaneous emission of the CsPbI3 Perovskite NCs using hybrid (HMM-Mie resonator) structures
2021
Entanglement trapping in structured environments
2008
The entanglement dynamics of two independent qubits each embedded in a structured environment under conditions of inhibition of spontaneous emission is analyzed, showing entanglement trapping. We demonstrate that entanglement trapping can be used efficiently to prevent entanglement sudden death. For the case of realistic photonic band-gap materials, we show that high values of entanglement trapping can be achieved. This result is of both fundamental and applicative interest since it provides a physical situation where the entanglement can be preserved and manipulated, e.g. by Stark-shifting the qubit transition frequency outside and inside the gap.
Spontaneous emission of an atom in a dynamical photonic crystal
2014
A structured environment such as a photonic crystal can strongly affect radiative properties of an atomic system, for example the spontaneous emission process. Recently there has been also an increasing interest on dynamical photonic crystal, that is photonic crystals whose dielectric properties change on time. We consider the spontaneous emission of an atom placed inside a photonic crystal with time-dependent properties (dynamical photonic crystal). We investigate the atomic spontaneous emission in two different regimes, weak and strong coupling, assuming a small, periodic and adiabatic perturbation of the crystal. In the weak coupling case, we analytically obtain the spontaneous emission …
Several Derivatives of 6-(Tert-Butyl)-4H-Pyran-4-Ylidene Malononitrile with Different Amorphous Phase Promoting Substituents for Light-Amplification …
2019
A series of glassy 6-(tert-butyl)-4H-pyran-4-ylidene malononitrile (DCM) derivatives with covalently attached amorphous state promoting bulky 1,1,1-triphenylmethyl (trityl) moieties through several chemical design approaches have been synthesized and investigated for suitability in organic solid state laser applications. Results showed that the bonding type of such functional groups had a considerable influence on glass structure forming dye thermal properties and a slight influence on their optical properties. Thermal stability up to 346 °C was achieved with glass transitions in the range from 39 to 138 °C. Incorporation of bulky triphenyl substituents via ester groups showed remarkable am…
Cavités plasmoniques et nanosources optiques
2013
Optical microcavities exhibit high resonance quality, so that, they are of key interest for the design of low-threshold lasers or for achieving strong coupling regime. But, such systems support modes whose the volume remain diffraction limited.In this manuscript, we are interested in their plasmonic counterparts because they support confined modes at the sub-wavelength scale. First, we study an in-plane plasmonic cavity which is the transposition of 1D optical cavity to surface wave. We characterize the cavity by measuring the fluorescence lifetime of dye molecules deposited inside.Then, we are interested in 3-dimension mode confinement achieved by spherical metal nanoparticles. We discuss …
An experimental analysis of self-Q-switching via stimulated Brillouin scattering in an ytterbium doped fiber laser
2013
An experimental study of self-Q-switching (SQS) in an ytterbium doped fiber laser (YDFL) arranged using a twin-core GTWave assembly is reported. The main mechanisms that initiate, amplify, and limit SQS pulses in amplitude are revealed to be stimulated Brillouin and Raman scattering (SBS/SRS) and Yb3+ amplified spontaneous emission. The parameters featuring SQS oscillation in terms of efficiency and stability of pulsing are found to be intra-cavity loss and feedback strength. An analysis of the YDFL SQS regime?s features?pulsing time series, optical and RF spectra, amplitude and timing jitter?is provided for the two experimental situations: (i) when SQS pulsing stochastically intermits with…
Ytterbium-doped fiber laser as pulsed source of narrowband amplified spontaneous emission
2019
AbstractWe report random noise pulsed regime of an ytterbium-doped fiber laser arranged in common Fabry-Perot configuration. We show that the laser output obeys the photon statistics inherent to narrowband amplified spontaneous emission and that the noise pulsing is properly addressed in terms of probability density and autocorrelation functions. Our novel approach reveals, in particular, that the regime’s coherence time dramatically shortens, from few ns to tens ps, with increasing laser power.
Implementation of single-qubit quantum gates by adiabatic passage and static laser phases
2006
International audience; We propose and analyse experimentally feasible implementations of single-qubit quantum gates based on stimulated Raman adiabatic passage (STIRAP) between magnetic sublevels in atoms coupled by elliptically polarized pulsed laser fields, in part based on a proposal by Kis and Renzoni [Z. Kis, F. Renzoni, Phys. Rev. A 65 (2002) 032318]. These techniques require only the control of the relative phase of the driving fields but do not involve any dynamical or geometric phases, which makes it independent of the other interaction details: detuning, pulse shapes, pulse areas and pulse durations. The suggested techniques are immune to spontaneous emission since the qubit mani…
Rains of Solitons in a Fiber Laser
2009
We report a novel and intriguing nonlinear dynamics observed in a fiber laser cavity, in which soliton pulses are created from an extended noisy background and drift until they reach a condensed phase comprising several tens of aggregated solitons. This soliton flow can be adjusted with manual cavity tuning, and can even be triggered by the injection of an external low-power cw laser.